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We present here a theoretical method to determine the phononic contribution to the thermal conductance of nanoscale systems in the phase-coherent regime. Our approach makes use of classical molecular dynamics (MD) simulations to calculate…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Fabian Müller , Peter Nielaba , Juan Carlos Cuevas , Fabian Pauly

Heat transport in low-dimensional systems has attracted enormous attention from both theoretical and experimental aspects due to its significance to the perception of fundamental energy transport theory and its potential applications in the…

Chaotic Dynamics · Physics 2013-01-04 Nianbei Li , Baowen Li

In the pursuit of advanced ceramic materials with exceptional irradiation-resistance and high-temperature tolerance for nuclear applications, compositionally complex carbides (CCCs) have emerged as a highly promising class of candidate…

Machine-learned interatomic potentials enable realistic finite temperature calculations of complex materials properties with first-principles accuracy. It is not yet clear, however, how accurately they describe anharmonic properties, which…

Materials Science · Physics 2021-10-01 Carla Verdi , Ferenc Karsai , Peitao Liu , Ryosuke Jinnouchi , Georg Kresse

Phonons play a crucial role in many properties of solid state systems, such as thermal and electrical conductivity, neutron scattering and associated effects or superconductivity. Hence, it is expected that topological phonons will also…

Phonon densities of states (DOS) of bcc $\alpha$-$^{57}$Fe were measured from room temperature through the 1044K Curie transition and the 1185K fcc $\gamma$-Fe phase transition using nuclear resonant inelastic x-ray scattering. At higher…

Materials Science · Physics 2015-06-19 L. Mauger , M. S. Lucas , J. A. Muñoz , S. J. Tracy , M. Kresch , Yuming Xiao , Paul Chow , B. Fultz

Machine learning (ML) methods have become powerful tools for predicting material properties with near first-principles accuracy and vastly reduced computational cost. However, the performance of ML models critically depends on the quality,…

Materials Science · Physics 2025-11-20 Pol Benítez , Cibrán López , Edgardo Saucedo , Teruyasu Mizoguchi , Claudio Cazorla

The material dependence of phonon-polariton based in-plane thermal conductance is investigated by examining systems composed of air and several wurtzite and zinc-blende crystals. Phonon-polariton based thermal conductance varies by over an…

Materials Science · Physics 2023-10-05 Jacob D. Minyard , Thomas E. Beechem

We show that the commonly used lowest-order theory of phonon-phonon interactions frequently fails to accurately describe the anharmonic phonon decay rates and thermal conductivity ($\kappa$), even among strongly bonded crystals. Applying a…

Materials Science · Physics 2020-07-01 Navaneetha K. Ravichandran , David Broido

All phonons in a single crystal of NaBr were measured by inelastic neutron scattering at temperatures of 10, 300 and 700 K. Even at 300 K the phonons, especially the longitudinal-optical (LO) phonons, showed large shifts in frequencies, and…

Materials Science · Physics 2020-08-26 Y. Shen , C. N. Saunders , C. M. Bernal , D. L. Abernathy , M. E. Manley , B. Fultz

Phonons are quasiparticles associated with mechanical vibrations in materials. They are at the root of the propagation of sound and elastic waves, as well as of thermal phenomena, which are pervasive in our everyday life and in many…

Phonon quasi-particles have been monumental in microscopically understanding thermodynamics and transport properties in condensed matter for decades. Phonons have one-to-one correspondence with harmonic eigenstates and their energies are…

Materials Science · Physics 2024-08-27 Jaeyun Moon , Leo Zella , Lucas Lindsay

Lattice anharmonicity is thought to strongly affect vacancy concentrations in metals at high temperatures. It is however non-trivial to account for this effect directly using density functional theory (DFT). Here we develop a deep neural…

Materials Science · Physics 2019-10-02 Anton S. Bochkarev , Ambroise van Roekeghem , Stefano Mossa , Natalio Mingo

We investigate phonon transport in perovskite strontium titanate (SrTiO3) which is stable above its phase transition temperature (~105 K) by using first-principles molecular dynamics and anharmonic lattice dynamics. Unlike conventional…

Computational Physics · Physics 2015-06-09 Lei Feng , Takuma Shiga , Junichiro Shiomi

Harnessing the power of low-dimensional materials in thermal applications calls for a solid understanding of the anomalous thermal properties of such systems. We analyze thermal conduction in one-dimensional systems by determining the…

Computational Physics · Physics 2015-12-21 K. Sääskilahti , J. Oksanen , S. Volz , J. Tulkki

Phonon measurements in the A15-type superconductors were complicated in the past because of the unavailability of large single crystals for inelastic neutron scattering, e.g., in the case of Nb$_3$Sn, or unfavorable neutron scattering…

Superconductivity · Physics 2019-04-19 A. Sauer , D. A. Zocco , A. H. Said , R. Heid , A. Böhmer , F. Weber

Despite vibrational properties being critical for the ab initio prediction of the finite temperature stability and transport properties of solids, their inclusion in ab initio materials repositories has been hindered by expensive…

A previously proposed variational approach for momentum-conserving systems [J. Liu et.al., Phys. Rev. E 91, 042910 (2015)] is extended to systematically investigate general momentum-nonconserving nonlinear lattices. Two intrinsic identities…

Statistical Mechanics · Physics 2016-09-20 Junjie Liu , Baowen Li , Changqin Wu

Studying the physical properties of materials under high pressure and temperature through experiments is difficult. Theoretical simulations can compensate for this deficiency. Currently, large-scale simulations using machine learning force…

Materials Science · Physics 2022-10-05 Hao Wang , Xiao-Long Pan , Yu-Feng Wang , Xiang-Rong Chen , Yi-Xian Wang , Hua Y. Geng

Fundamental insight into lattice dynamics and phonon transport is critical to the efficient manipulation of heat flow, which is one of the appealing thermophysical problems with enormous practical implications. Phosphorene, a novel…

Materials Science · Physics 2018-01-16 Guangzhao Qin , Ming Hu
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