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A highly sensitive, general, and preferably nondestructive technique to detect polar molecules would greatly advance a number of fields, in particular quantum science with cold and ultracold molecules. Here, we propose using resonant energy…

Atomic Physics · Physics 2017-06-23 Martin Zeppenfeld

We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar…

Quantum Physics · Physics 2017-09-13 Elena Kuznetsova , Seth T. Rittenhouse , Hossein R. Sadeghpour , Susanne F. Yelin

We propose a method to sympathetically cool polar molecules with Rydberg atoms without destroying the quantum information encoded in the polar molecules. While the interactions between the two are usually state-dependent, we show how to…

Quantum Physics · Physics 2025-07-22 Jeremy T. Young , Ron Belyansky , Kang-Kuen Ni , Alexey V. Gorshkov

We present a new approach to investigating Rydberg molecules by demonstrating the formation and characterization of individual Rb$^{*}$Cs Rydberg molecules using optical tweezers. By employing single-atom detection of Rb and Cs, we observe…

Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the…

Atomic Physics · Physics 2024-08-28 Daniel K. Ruttley , Alexander Guttridge , Tom R. Hepworth , Simon L. Cornish

The ability to locally control and measure subsets of ancilla qubits in an efficient and crosstalk-free manner is a key ingredient in quantum error correction (QEC). Dual-species neutral atom arrays offer an ideal implementation of these…

We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…

Quantum Physics · Physics 2016-10-05 Elena Kuznetsova , Seth T. Rittenhouse , H. R. Sadeghpour , Susanne F. Yelin

Non-radiative energy transfer between a Rydberg atom and a polar molecule can be controlled by a DC electric field. Here we show how to exploit this control for state-resolved, non-destructive detection and spectroscopy of the molecules…

Atomic Physics · Physics 2023-11-28 Sabrina Patsch , Martin Zeppenfeld , Christiane P. Koch

We investigate the Autler-Townes splitting for Rydberg atoms dressed with linearly polarized microwave radiation, resonant with generic $S_{1/2}\leftrightarrow{P}_{1/2}$ and $S_{1/2}\leftrightarrow{P}_{3/2}$ transitions. The splitting is…

Quantum Physics · Physics 2024-04-16 M. Cloutman , M. Chilcott , A. Elliott , J. S. Otto , A. B. Deb , N. Kjærgaard

Rydberg atoms held in optical tweezer arrays combine vibrational and electronic degrees of freedom which can be coupled and manipulated at a microscopic level. This opens opportunities for the quantum simulation of artificial molecular…

Quantum Physics · Physics 2025-10-21 Simon Euchner , Igor Lesanovsky

We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…

Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of…

Among the thriving quantum computation and quantum simulation platforms based on arrays of Rydberg atoms, those using circular Rydberg atoms are particularly promising. These atoms uniquely combine the strong dipole-dipole interactions…

We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation. Quantum information is stored in long-lived hyperfine or rotational states of molecules which interact…

Quantum Physics · Physics 2022-06-07 Chi Zhang , M. R. Tarbutt

We report on our recent progress on the manipulation of single rubidium atoms trapped in optical tweezers and the generation of entanglement between two atoms, each individually trapped in neighboring tweezers. To create an entangled state…

We implement and characterize a protocol that enables arbitrary local controls in a dipolar atom array, where the degree of freedom is encoded in a pair of Rydberg states. Our approach relies on a combination of local addressing beams and…

Central spin models, where a single spinful particle interacts with a spin environment, find wide application in quantum information technology and can be used to describe, e.g., the decoherence of a qubit over time. We propose a method of…

Quantum Physics · Physics 2023-11-30 Jacek Dobrzyniecki , Michał Tomza

Divalent atoms provide excellent means for advancing control in Rydberg atom-based quantum simulation and computing, due to the second optically active valence electron available. Particularly promising in this context are circular Rydberg…

Rydberg electromagnetically induced transparency (EIT) enables realization of atom-based SI-traceable microwave (MW) sensing, imaging and communication devices by exploiting the strong microwave electric dipole coupling of highly excited…

Atomic Physics · Physics 2021-08-09 Aurélien Chopinaud , Jonathan D. Pritchard

We probe resonant dipolar interactions between ultracold $^{40}$K$^{87}$Rb molecules and Rydberg $^{87}$Rb atoms in an optically trapped ensemble. Through state-selective ionization detection of the KRb molecules, we observe resonant energy…

Atomic Physics · Physics 2025-04-10 Lingbang Zhu , Jeshurun Luke , Roy Shaham , Yi-Xiang Liu , Kang-Kuen Ni
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