Related papers: A directly observable, Zeeman-insensitive nuclear …
Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the…
Nuclear spins support long lived quantum coherence due to weak coupling to the environment, but are difficult to rapidly control using nuclear magnetic resonance (NMR) as a result of the small nuclear magnetic moment. We demonstrate a fast…
We report the existence of a sizeable quantum tunnelling splitting between the two lowest electronic spin levels of mononuclear Ni complexes. The level anti-crossing, or magnetic clock transition, associated with this gap has been directly…
Hybrid qubit systems combining electronic spins with nearby ("proximate") nuclear spin registers offer a promising avenue towards quantum information processing, with even multi-spin error correction protocols recently demonstrated in…
We study the dynamics of an electron spin in a graphene quantum dot, which is interacting with a bath of less than ten nuclear spins via the anisotropic hyperfine interaction. Due to substantial progress in the fabrication of graphene…
We demonstrate the coherent control and electrical readout of the nuclear spins of ionized phosphorus donors in natural silicon. By combining pulsed illumination with coherent electron spin manipulation, we selectively ionize the donor…
Noble-gas spins feature hours long coherence times owing to their great isolation from the environment, and find practical usage in various applications. However, this isolation leads to extremely slow preparation times, relying on weak…
The ability to process and store information on surrounding nuclear spins is a major requirement for group-IV color center-based repeater nodes. We demonstrate coherent control of a ${}^{13}$C nuclear spin strongly coupled to a negatively…
The transfer of information between different physical forms is a central theme in communication and computation, for example between processing entities and memory. Nowhere is this more crucial than in quantum computation, where great…
Spins in silicon that are accessible via a telecom-compatible optical transition are a versatile platform for quantum information processing that can leverage the well-established silicon nanofabrication industry. Key to these applications…
Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…
We address the decoherence of a localized electron spin in an external magnetic field due to the hyperfine interaction with a lattice of nuclear spins. Using a completely non-perturbative method, rigorous bounds on the T_1 and T_2 coherence…
Many coherence transfer experiments in Nuclear Magnetic Resonance Spectroscopy, involving network of coupled spins, use temporary spin-decoupling to produce desired effective Hamiltonians. In this paper, we show that significant time can be…
An experiment demonstrating the quantum simulation of a spin-lattice Hamiltonian is proposed. Dipolar interactions between nuclear spins in a solid state lattice can be modulated by rapid radio-frequency pulses. In this way, the effective…
We investigate the coherence properties of individual nuclear spin quantum bits in diamond [Dutt et al., Science, 316, 1312 (2007)] when a proximal electronic spin associated with a nitrogen-vacancy (NV) center is being interrogated by…
For the realisation of scalable solid-state quantum-bit systems, spins in semiconductor quantum dots are promising candidates. A key requirement for quantum logic operations is a sufficiently long coherence time of the spin system.…
We present a new class of control pulses designed to transfer co-located ensembles without relying on frequency selectivity, thereby allowing much faster state-transitions. A geometric approach allows us to construct sequences which are…
The quantum antiferromagnet Cu2Te2O5Br2 was investigated by NMR and NQR. The 125Te NMR investigation showed that there is a magnetic transition around 10.5K at 9T, in agreement with previous studies. From the divergence of the spin-lattice…
Motivated by the recent observation that exponentially long coherence times can be achieved for edge spins in models with strong zero modes, we study the impact of level crossings in finite-length spin chains on the dynamics of the edge…
Optically addressed atomic defects in the solid-state are widely used as single-photon sources and memories for quantum network applications. The solid-state environment allows for a high density of electron and nuclear spins with the…