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The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

Statistical Mechanics · Physics 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

We describe a new approach to precision NMR with hyperpolarized gases designed to mitigate NMR frequency shifts due to the alkali spin exchange field. The electronic spin polarization of optically pumped alkali atoms is square-wave…

Atomic Physics · Physics 2015-12-23 Anna Korver , Daniel Thrasher , Mike Bulatowicz , Thad Walker

Diffractive deep neural network (DNNet) is a novel machine learning framework on the modulation of optical transmission. Diffractive network would get predictions at the speed of light. It's pure passive architecture, no additional power…

Machine Learning · Computer Science 2019-12-24 Yingshi Chen , Jinfeng Zhu

The control of nuclear spins in quantum dots is essential to explore their many-body dynamics and exploit their prospects for quantum information processing. We present a unique combination of dynamic nuclear spin polarization and…

Mesoscale and Nanoscale Physics · Physics 2015-12-16 Florian Forster , Max Mühlbacher , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…

Quantum Physics · Physics 2022-12-07 Zhu-yao Jin , Jia-shun Yan , Jun Jing

Over recent decades, the value of conducting experiments at lower frequencies and in inhomogeneous and/or time-variable fields has grown. For example, an interest in the nanoscale heterogeneities of hydration dynamics demands increasingly…

Chemical Physics · Physics 2022-11-23 Alec A. Beaton , Alexandria Guinness , John M. Franck

Periodic driving of quantum dots is analyzed as a basis for developing dynamic switching devices. We study transport through periodically modulated energy levels which are coupled to leads via tunneling coefficients. Utilizing Floquet…

Mesoscale and Nanoscale Physics · Physics 2025-09-10 Jan Mathis Giesen , Daniel Weber , Sebastian Eggert

The optimization of dynamical decoupling and quantum error correction for a particular qubit realization is based on a detailed knowledge of the noise properties. Spectroscopy of single-axis noise using dynamical decoupling pulse sequences…

Quantum Physics · Physics 2014-01-22 Daniel K. Park , Jonathan Baugh

A broad effort is underway to improve the sensitivity of nuclear magnetic resonance through the use of dynamic nuclear polarization. Nitrogen-vacancy (NV) centers in diamond offer an appealing platform because these paramagnetic defects can…

Sensing the internal dynamics of individual nuclear spins or clusters of nuclear spins has recently become possible by observing the coherence decay of a nearby electronic spin: the weak magnetic noise is amplified by a periodic,…

Quantum Physics · Physics 2016-01-05 J. E. Lang , Ren-Bao Liu , T. S. Monteiro

The nitrogen-vacancy (NV) centre in diamond has emerged as a candidate to non-invasively hyperpolarise nuclear spins in molecular systems to improve the sensitivity of nuclear magnetic resonance (NMR) experiments. Several promising proof of…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 A. J. Healey , L. T. Hall , G. A. L. White , T. Teraji , M. -A. Sani , F. Separovic , J. -P. Tetienne , L. C. L. Hollenberg

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 E. Evers , T. Kazimierczuk , F. Mertens , D. R. Yakovlev , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer , A. Greilich

We propose a new method for dynamic nuclear polarisation in a quasi one-dimensional quantum wire utilising the spin-orbit interaction, the hyperfine interaction, and a finite source-drain potential difference. In contrast with current…

Mesoscale and Nanoscale Physics · Physics 2008-03-05 V. Tripathi , A. C. H. Cheung , N. R. Cooper

The dynamics of the coupled electron-nuclear spin system is studied in an ensemble of singly-charged (In,Ga)As/GaAs quantum dots (QDs) using periodic optical excitation at 1 GHz repetition rate. In combination with the electron-nuclei…

Mesoscale and Nanoscale Physics · Physics 2021-08-11 E. Evers , N. E. Kopteva , I. A. Yugova , D. R. Yakovlev , M. Bayer , A. Greilich

In this paper, we numerically optimize broadband pulse shapes that maximize Hahn echo amplitudes. Pulses are parameterized as neural networks (NN), nonlinear amplitude limited Fourier series (FS), and discrete time series (DT). These are…

Chemical Physics · Physics 2025-05-01 Eric R. Lowe , Stefan Stoll , J. P. Kestner

$^1$H nuclear spin-lattice relaxation and Dynamic Nuclear Polarization (DNP) have been studied in amorphous samples of trehalose sugar doped with TEMPO radicals by means of mechanical milling, in the 1.6 K $\div$ 4.2 K temperature range.…

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

Quantum Physics · Physics 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

We report bulk, room-temperature hyperpolarization of 13C nuclear spins observed via high-field nuclear magnetic resonance (NMR). The hyperpolarization is achieved by optical pumping (OP) of nitrogen vacancy defect centers in diamond…

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

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