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Predicting the structure of quantum many-body systems from the first principles of quantum mechanics is a common challenge in physics, chemistry, and material science. Deep machine learning has proven to be a powerful tool for solving…

Nuclear Theory · Physics 2023-04-05 Yilong Yang , Pengwei Zhao

This paper investigates efficient deep neural networks (DNNs) to replace dense unstructured weight matrices with structured ones that possess desired properties. The challenge arises because the optimal weight matrix structure in popular…

Machine Learning · Computer Science 2024-03-11 Changwoo Lee , Hun-Seok Kim

Performance optimization is the art of continuous seeking a harmonious mapping between the application domain and hardware. Recent years have witnessed a surge of deep learning (DL) applications in industry. Conventional wisdom for…

Distributed, Parallel, and Cluster Computing · Computer Science 2019-11-27 Guoping Long , Jun Yang , Wei Lin

Finding new materials with previously unknown atomic structure or materials with optimal set of properties for a specific application greatly benefits from computational modeling. Recently, such screening has been dramatically accelerated…

Materials Science · Physics 2025-04-11 Ethan Berger , Mohammad Bagheri , Hannu-Pekka Komsa

Traditional simulations on High-Performance Computing (HPC) systems typically involve modeling very large domains and/or very complex equations. HPC systems allow running large models, but limits in performance increase that have become…

Designing architectures for deep neural networks requires expert knowledge and substantial computation time. We propose a technique to accelerate architecture selection by learning an auxiliary HyperNet that generates the weights of a main…

Machine Learning · Computer Science 2017-08-18 Andrew Brock , Theodore Lim , J. M. Ritchie , Nick Weston

We present a general framework for training deep neural networks without backpropagation. This substantially decreases training time and also allows for construction of deep networks with many sorts of learners, including networks whose…

Machine Learning · Statistics 2017-06-09 Chris Hettinger , Tanner Christensen , Ben Ehlert , Jeffrey Humpherys , Tyler Jarvis , Sean Wade

Molecular property calculations are the bedrock of chemical physics. High-fidelity \textit{ab initio} modeling techniques for computing the molecular properties can be prohibitively expensive, and motivate the development of…

Machine Learning · Computer Science 2022-11-28 Hatem Helal , Jesun Firoz , Jenna Bilbrey , Mario Michael Krell , Tom Murray , Ang Li , Sotiris Xantheas , Sutanay Choudhury

In comparison to classical shallow representation learning techniques, deep neural networks have achieved superior performance in nearly every application benchmark. But despite their clear empirical advantages, it is still not well…

Machine Learning · Computer Science 2022-01-11 Calvin Murdock , George Cazenavette , Simon Lucey

Amorphous materials exhibit unique properties that make them suitable for various applications in science and technology, ranging from optical and electronic devices and solid-state batteries to protective coatings. However, data-driven…

Materials Science · Physics 2024-02-02 Hui Zheng , Eric Sivonxay , Max Gallant , Ziyao Luo , Matthew McDermott , Patrick Huck , Kristin A. Persson

Two of the most widely used electronic structure theory methods, namely Hartree-Fock and Kohn-Sham density functional theory, both requires the iterative solution of a set of Schr\"odinger-like equations. The speed of convergence of such…

Chemical Physics · Physics 2024-06-06 S. Hazra , U. Patil , S. Sanvito

Hardware accelerations of deep learning systems have been extensively investigated in industry and academia. The aim of this paper is to achieve ultra-high energy efficiency and performance for hardware implementations of deep neural…

Machine Learning · Computer Science 2018-02-20 Yanzhi Wang , Caiwen Ding , Zhe Li , Geng Yuan , Siyu Liao , Xiaolong Ma , Bo Yuan , Xuehai Qian , Jian Tang , Qinru Qiu , Xue Lin

Molecular sciences address a wide range of problems involving molecules of different types and sizes and their complexes. Recently, geometric deep learning, especially Graph Neural Networks, has shown promising performance in molecular…

Machine Learning · Computer Science 2023-11-21 Shuo Zhang , Yang Liu , Lei Xie

Despite of their success, the results of first-principles quantum mechanical calculations contain inherent numerical errors caused by various approximations. We propose here a neural-network algorithm to greatly reduce these inherent…

Data Analysis, Statistics and Probability · Physics 2007-05-23 LiHong Hu , XiuJun Wang , LaiHo Wong , GuanHua Chen

The great success of deep learning shows that its technology contains profound truth, and understanding its internal mechanism not only has important implications for the development of its technology and effective application in various…

Machine Learning · Computer Science 2018-05-23 Dian Lei , Xiaoxiao Chen , Jianfei Zhao

The fundamental quantity governing the mechanical and thermodynamic properties of a crystalline solid is its electronic charge density. Yet, its direct use for the rapid prediction of materials properties remains challenging due to its high…

Materials Science · Physics 2026-05-11 Kammampati Sai Kumar , Albert Linda , Shubham Kumar Maurya , Somnath Bhowmick

To improve predictive models for STEM applications, supplemental physics-based features computed from input parameters are introduced into single and multiple layers of a deep neural network (DNN). While many studies focus on informing DNNs…

Emerging Technologies · Computer Science 2024-09-02 Nicholus R. Clinkinbeard , Nicole N. Hashemi

Twistronics is an emerging and captivating field in condensed matter physics and material science. However, accurately and efficiently calculating the electronic structures of twisted systems remains a significant challenge. To address…

Materials Science · Physics 2026-05-27 Junxi Yu , Yichen Liu , Cheng-Cheng Liu

The Hessian of a neural network captures parameter interactions through second-order derivatives of the loss. It is a fundamental object of study, closely tied to various problems in deep learning, including model design, optimization, and…

Machine Learning · Computer Science 2021-07-02 Sidak Pal Singh , Gregor Bachmann , Thomas Hofmann