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Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
Extremely fast qubit controls can greatly reduce the calculation time in quantum computation, and potentially resolve the finite-time decoherence issues in many physical systems. Here, we propose and experimentally demonstrate pico-second…
Adiabatic protocols are employed across a variety of quantum technologies, from implementing state preparation and individual operations that are building blocks of larger devices, to higher-level protocols in quantum annealing and…
We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…
This theoretical paper presents numerical calculations for photoassociation of ultracold cesium atoms with a chirped laser pulse and detailed analysis of the results. In contrast with earlier work, the initial state is represented by a…
We systematically characterize the dynamical evolution of time-parity (PT )-symmetric two-level systems with spin-dependent dissipations. If the control parameters of the gap are linearly tuned with time, the dynamical evolution can be…
Pulsed lasers offer significant advantages over CW lasers in the coherent control of qubits. Here we review the theoretical and experimental aspects of controlling the internal and external states of individual trapped atoms with pulse…
We introduce a geometric framework for efficient few-parameter pulse optimization in multi-level quantum systems, enabling high-fidelity state transfer beyond the adiabatic limit. Our method interpolates smoothly between adiabatic and…
We show that a counter-intuitive pulse sequence leads to adiabatic passage between the vibrational levels of three harmonic potentials through parallel dark states in adiabatic approximation. However, the adiabatic assumptions break down…
This work focuses on the incoherent and coherent combination of pulsed laser beams, building on previous research [1] that addressed the combination of continuous-wave laser beams. For the pulsed combination, we have focused on the temporal…
In the pursuit of scalable superconducting quantum computing, tunable couplers have emerged as a pivotal component, offering the flexibility required for complex quantum operations of high performance. In most current architectures of…
The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear…
Shortcut to adiabaticity in various quantum systems has attracted much attention with the wide applications in quantum information processing and quantum control. In this paper, we concentrate on stimulated Raman shortcut-to-adiabatic…
The interaction of a molecule with the quantized electromagnetic field of a nano-cavity gives rise to light-induced conical intersections between polaritonic potential energy surfaces. We demonstrate for a realistic model of a polyatomic…
We present a comprehensive computational framework for simulating nonadiabatic molecular dynamics with explicit inclusion of geometric phase (GP) effects. Our approach is based on a generalized two-level Hamiltonian model that can represent…
Efficient control schemes that enable fast, high-fidelity operations are essential for any practical quantum computation. However, current optimization protocols are intractable due to stringent requirements imposed by the microscopic…
We present an implementation of optimal control theory for the first-principles non-adiabatic Ehrenfest Molecular Dynamics model, which describes a condensed matter system by considering classical point-particle nuclei, and quantum…
We present a method to control photodissociation by manipulating the bond softening mechanism occurring in strong shaped laser fields, by varying the chirp sign and magnitude of an ultra-short laser pulse. Manipulation of bond-softening is…
The ability to control spins in semiconductors is important in a variety of fields including spintronics and quantum information processing. Due to the potentially fast dephasing times of spins in the solid state [1-3], spin control…
Photon echo (PE) techniques offer a promising approach to optical quantum memory, yet their implementation in conventional platforms, such as rare-earth-ion-doped crystals, is hindered by limited bandwidths. Semiconductor quantum dot (QD)…