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We present a computational investigation of the mechanism governing size-based particle separation in microfluidic pinched flow fractionation. We study the behavior of particles moving through a pinching gap (i.e., a constriction in the…

Fluid Dynamics · Physics 2016-05-04 Sumedh R. Risbud , German Drazer

We investigate experimentally and theoretically diffusiophoretic separation of negatively charged particles in a rectangular channel flow, driven by CO2 dissolution from one side-wall. Since the negatively charged particles create an…

Fluid Dynamics · Physics 2021-06-01 Suin Shim , Mrudhula Baskaran , Ethan H. Thai , Howard A. Stone

Water is a polar solvent and hence supports the bulk dissociation of itself and its solutes into ions, and the re-association of these ions into neutral molecules in a dynamic equilibrium, e.g., ${\rm H_2O_2}\leftrightharpoons {\rm…

Soft Condensed Matter · Physics 2016-08-17 Aidan T. Brown , Wilson C. K. Poon , Christian Holm , Joost de Graaf

The friction and diffusion coefficients of rigid spherical colloidal particles dissolved in a fluid are determined from velocity and force autocorrelation functions by mesoscale hydrodynamic simulations. Colloids with both slip and no-slip…

Soft Condensed Matter · Physics 2016-03-10 Mario Theers , Elmar Westphal , Gerhard Gompper , Roland G. Winkler

Living systems routinely consume energy to achieve motility, often using intricate biomolecular machinery. In this work, we show that active droplets can sustain indefinite self-propulsion of a spherical colloid in an otherwise homogeneous,…

Soft Condensed Matter · Physics 2026-05-01 Benjamin Sorkin , Ned S. Wingreen

In this work, we numerically investigate the impact of two-dimensional solute gradients on the distribution of colloidal particles, i.e., colloidal banding, induced via diffusiophoresis. The solute gradients are generated by spatially…

Soft Condensed Matter · Physics 2023-01-11 Ritu R. Raj , C. Wyatt Shields , Ankur Gupta

When the concentration of electrolyte solution varies along the channel the forces arise that drag the fluid toward the higher or lower concentration region inducing a flow termed diffusio-osmotic. This article investigates a flow that…

Soft Condensed Matter · Physics 2025-12-30 Evgeny S. Asmolov , Elena F. Silkina , Olga I. Vinogradova

The controlled transport of colloids in dead-end structures is a key capability that can enable a wide range of applications, such as bio-chemical analysis, drug delivery and underground oil recovery. This letter presents a new trapping…

Slow long-lived fluctuations of mechanical properties of drying drops of instant coffee water solutions have been found by means of the Drying Drop Technology developed earlier. Parameters of the fluctuations depended on the extent of…

Soft Condensed Matter · Physics 2016-10-26 Tatiana A. Yakhno , Vladimir G. Yakhno

Colloidal particles that are confined to an interface effectively form a two-dimensional fluid. We examine the dynamics of such colloids when they are subject to a constant external force, which drives them in a particular direction over…

Soft Condensed Matter · Physics 2011-06-24 Andrew J. Archer , Alexandr Malijevsky

We study the diffusiophoretic self-propulsion of a colloidal catalytic particle due to a surface chemical reaction in a vicinity of a solid wall. Diffusiophoresis is a chemico-mechanical transduction mechanism in which a concentration…

Soft Condensed Matter · Physics 2016-06-22 Ali Mozaffari , Nima Sharifi-Mood , Joel Koplik , Charles Maldarelli

Breaking spatial symmetry is an essential requirement for phoretic active particles to swim at low Reynolds number. This fundamental prerequisite for swimming at the micro-scale is fulfilled either by chemical patterning of the surface of…

Soft Condensed Matter · Physics 2022-04-20 Abdallah Daddi-Moussa-Ider , Andrej Vilfan , Ramin Golestanian

Microorganisms are able to overcome the thermal randomness of their surroundings by harvesting energy to navigate in viscous fluid environments. In a similar manner, synthetic colloidal microswimmers are capable of mimicking complex…

Unrestricted particle transport through microfluidic channels is of paramount importance to a wide range of applications, including lab-on-a-chip devices. In this article, we study using video microscopy the electro-osmotic aggregation of…

Soft Condensed Matter · Physics 2021-04-02 Zhu Zhang , Joost de Graaf , Sanli Faez

The macroscopic phenomenon of filtration is the separation between suspended and liquid phases and it takes place in natural environments (e.g. groundwater, soil, hyporheic zone) and industrial systems (e.g. filtration plants,…

The connection between fundamental interactions acting in molecules in a fluid and macroscopically measured properties, such as the viscosity between colloidal particles coated with polymers, is studied here. The role that hydrodynamic and…

Soft Condensed Matter · Physics 2015-09-02 A. Gama Goicochea , M. A. Balderas Altamirano , R. Lopez-Esparza , M. A. Waldo , E. Perez

In colloidal systems, Brownian motion emerges from the massive separation of time and length scales associated to characteristic dynamics of the solute and solvent constituents. This separation of scales produces several temporal regimes in…

Phase separation driven by nonequilibrium fluctuations is a hallmark of both living and synthetic active matter. Unlike equilibrium systems, where ordered states arise from the minimization of free energy, active systems are fueled by a…

Inertial effects should be considered for micro- and nano-swimmers moving in a low-density medium confined by irregular structures that create entropic barriers, where viscous effects are no longer paramount. Here, we present a separation…

Soft Condensed Matter · Physics 2024-05-03 Narender Khatri

Most available theoretical predictions for the self-diffusiophoretic motion of colloidal particles are based on the hydrodynamic thin boundary layer approximation in combination with a solvent body force due to a self-generated local solute…

Soft Condensed Matter · Physics 2019-06-19 Thomas Speck