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In this dissertation I analyze Hamiltonian control of $d$-dimensional quantum systems as realized in alkali atomic spins. Alkali atoms provide an ideal platform for studies of quantum control due to the extreme precision with which the…

Quantum Physics · Physics 2009-06-29 Seth Merkel

Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, e.g. in chemistry, medicine, materials science and mining. Nuclear spins also featured in early…

The dynamics of a quantum system driven by an external field is well described by a unitary transformation generated by a time dependent Hamiltonian. The inverse problem of finding the field that generates a specific unitary transformation…

Quantum Physics · Physics 2009-11-10 Jose P. Palao , R. Kosloff

We introduce a novel quantum control method for superconducting transmon qubits that substantially outperforms conventional techniques in precision and robustness against coherent errors. Our approach leverages composite pulses (CP) to…

Quantum Physics · Physics 2025-06-10 Hristo G. Tonchev , Boyan T. Torosov , Nikolay V. Vitanov

We apply theoretically open-loop quantum optimal control techniques to provide methods for the verification of various quantum coherent transport mechanisms in natural and artificial light-harvesting complexes under realistic experimental…

Quantum Physics · Physics 2012-05-01 Filippo Caruso , Simone Montangero , Tommaso Calarco , Susana F. Huelga , Martin B. Plenio

The goal of the present article is to review the major developments that have led to the current understanding of molecule-field interactions and experimental methods for manipulating molecules with electromagnetic fields. Molecule-field…

Atomic Physics · Physics 2013-09-18 Mikhail Lemeshko , Roman V. Krems , John M. Doyle , Sabre Kais

Simple, precise, and robust control is demanded for operating a large quantum information processor. However, existing routes to high-fidelity quantum control rely heavily on arbitrary waveform generators that are difficult to scale up.…

Quantum Physics · Physics 2022-09-21 Qi-Ming Chen , Herschel Rabitz , Re-Bing Wu

The spin states of electrons and holes confined in InAs quantum dot molecules have recently come to fore as a promising system for the storage or manipulation of quantum information. We describe here a feasible scheme for complete quantum…

Mesoscale and Nanoscale Physics · Physics 2015-01-09 Guy Z. Cohen

We perform a combined analytical and numerical investigation to explore how an analytically designed pulse can precisely control the rotational motions of a single-molecular polariton formed by the strong coupling of two low-lying…

Quantum Physics · Physics 2023-08-04 Li-Bao Fan , Chuan-Cun Shu

We develop a methodology for performing approximate optimal control simulations for quantum systems with multiple interacting degrees of freedom. The quantum dynamics are modeled using the first-order Magnus approximation in the interaction…

Quantum Physics · Physics 2020-08-05 Andrew Ma , Alicia B. Magann , Tak-San Ho , Herschel Rabitz

We propose a new monotonically convergent algorithm which can enforce spectral constraints on the control field (and extends to arbitrary filters). The procedure differs from standard algorithms in that at each iteration the control field…

Quantum Physics · Physics 2015-05-13 M. Lapert , R. Tehini , G. Turinici , D. Sugny

One fundamental requirement for quantum computation is to perform universal manipulations of quantum bits at rates much faster than the qubit's rate of decoherence. Recently, fast gate operations have been demonstrated in logical spin…

Mesoscale and Nanoscale Physics · Physics 2010-09-28 Sandra Foletti , Hendrik Bluhm , Diana Mahalu , Vladimir Umansky , Amir Yacoby

We give a framework for molecular multiphoton excitation process induced by an optimally designed electric field. The molecule is initially prepared in a coherent superposition state of two of its eigenfunctions. The relative phase of the…

Chemical Physics · Physics 2009-11-10 Bijoy K Dey

We present theory and calculations for coherent high-fidelity quantum control of many-particle states in semiconductor quantum wells. We show that coupling a two-electron double quantum dot to a terahertz optical source enables targeted…

Mesoscale and Nanoscale Physics · Physics 2013-02-04 E. Rasanen , T. Blasi , M. F. Borunda , E. J. Heller

The control of quantum system dynamics is generally performed by seeking a suitable applied field. The physical objective as a functional of the field forms the quantum control landscape, whose topology, under certain conditions, has been…

Quantum Physics · Physics 2014-11-11 Arun Nanduri , Ofer M. Shir , Ashley Donovan , Tak-San Ho , Herschel Rabitz

We investigate experimentally and numerically the field-free orientation of the symmetric top molecule of methyl-iodide at high temperature using a terahertz radiation generated by a plasma induced by a two-color laser beam. The degree of…

Quantum Physics · Physics 2016-11-03 P. Babilotte , K. Hamraoui , F. Billard , E. Hertz , B. Lavorel , O. Faucher , D. Sugny

We experimentally study the optical- and terahertz- induced rotational dynamics of asymmetric molecules in the gas phase. Terahertz and optical fields are identified as two distinct control handles over asymmetric molecules, as they couple…

Chemical Physics · Physics 2016-09-07 Ran Damari , Shimshon Kallush , Sharly Fleischer

Coherent control experiments in molecules are often done with shaped laser fields. The electric field is described classically and control over the time evolution of the system is achieved by shaping the laser pulses in the time or…

Chemical Physics · Physics 2019-11-27 András Csehi , Gábor J. Halász , Ágnes Vibók , Markus Kowalewski

Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 F. Fras , Q. Mermillod , G. Nogues , C. Hoarau , C. Schneider , M. Kamp , S. Höfling , W. Langbein , J. Kasprzak

Quantum computation is based on implementing selected unitary transformations which represent algorithms. A generalized optimal control theory is used to find the driving field that generates a prespecified unitary transformation. The…

Quantum Physics · Physics 2009-11-07 Jose P. Palao , Ronnie Kosloff