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We demonstrate the first cavity-enhanced optical frequency comb spectroscopy in the mid-infrared wavelength region and report the sensitive real-time trace detection of hydrogen peroxide in the presence of a large amount of water. The…

The optical microresonator-based frequency comb (microcomb) provides a versatile platform for nonlinear physics studies and has wide applications ranging from metrology to spectroscopy. Deterministic quantum regime is an unexplored aspect…

Modern experiments in quantum metrology, sensing, and quantum computing require precise control of the state of atoms and molecules, achieved through the use of highly stable lasers and microwave generators with low phase noise. One of the…

Over the last two decades, frequency combs have brought breakthroughs in length metrology with traceability to length standards. In particular, frequency-comb-based spectral interferometry is regarded as a promising technology for…

Optics · Physics 2025-01-20 Yoon-Soo Jang , Heulbi Ahn , Sunghoon Eom , Jungjae Park , Jonghan Jin

We combine a tunable continuous-wave optical parametric oscillator and a femtosecond Ti:Sapphire laser frequency comb to provide a phase-coherent bridge between the visible and mid-infrared spectral ranges. As a first demonstration of this…

Optics · Physics 2009-11-11 Evgeny Kovalchuk , Thilo Schuldt , Achim Peters

We demonstrate a new technique for the experimental measurement of the spectral coherence of microresonator optical frequency combs. Specifically, we use a spectral interference method, typically used in the context of supercontinuum…

We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

Quantum Physics · Physics 2015-06-04 Fritz Keilmann , Sergiu Amarie

Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing…

The generation of spectrally pure high-frequency microwave signals is a critical functionality in fundamental and applied sciences, including metrology and communications. The development of optical frequency combs has enabled the powerful…

This paper studies sensor calibration in spectral estimation where the true frequencies are located on a continuous domain. We consider a uniform array of sensors that collects measurements whose spectrum is composed of a finite number of…

Information Theory · Computer Science 2019-01-15 Yonina C. Eldar , Wenjing Liao , Sui Tang

Over the past decades hollow-cathode lamps have been calibration standards for spectroscopic measurements. Advancing to cm/s radial velocity precisions with the next generation of instruments requires more suitable calibration sources with…

Instrumentation and Methods for Astrophysics · Physics 2015-09-30 Florian F. Bauer , Mathias Zechmeister , Ansgar Reiners

We phase-coherently measure the frequency of continuous-wave (CW) laser light by use of optical-phase modulation and f-2f nonlinear interferometry. Periodic electro-optic modulation (EOM) transforms the CW laser into a continuous train of…

Molecular spectroscopy in the mid-infrared portion of the electromagnetic spectrum (3--25 um) has been a cornerstone interdisciplinary analytical technique widely adapted across the biological, chemical, and physical sciences. Applications…

Instrumentation and Detectors · Physics 2018-09-18 Abijith S. Kowligy , Henry Timmers , Alex Lind , Ugaitz Elu , Flavio C. Cruz , Peter G. Schunemann , Jens Biegert , Scott A. Diddams

Multiheterodyne techniques using frequency combs -- light sources whose lines are perfectly evenly-spaced -- have revolutionized optical science. By beating an unknown signal with the many lines of a comb, its spectrum is recovered.…

Optics · Physics 2020-04-23 David Burghoff

High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low…

We present a dual-comb spectrometer based on two passively mode-locked waveguide lasers integrated in a single Er-doped ZBLAN chip. This original design yields two free-running frequency combs having a high level of mutual stability. We…

Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…

Optics · Physics 2018-08-10 Zaijun Chen , Ming Yan , Theodor W. Hänsch , Nathalie Picqué

We report on the fabrication of high-Q, fused-quartz microresonators and the parametric generation of a frequency comb with 36 GHz line spacing using them. We have characterized the intrinsic stability of the comb in both the time and…

Optics · Physics 2011-11-18 Scott B. Papp , Scott A. Diddams

We have investigated parametric seeding of a microresonator frequency comb (microcomb) by way of a pump laser with two electro-optic-modulation sidebands. We show that the pump-sideband spacing is precisely replicated throughout the…

Optics · Physics 2013-05-15 Scott B. Papp , Pascal Del'Haye , Scott A. Diddams

Broadband dual-comb spectroscopy (DCS) based on portable mode-locked fiber frequency combs is a powerful tool for in situ, calibration free, multi-species spectroscopy. While the acquisition of a single spectrum with mode-locked DCS…

Optics · Physics 2021-02-03 Nazanin Hoghooghi , Ryan K. Cole , Gregory B. Rieker
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