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Aqueous zinc-air batteries (ZABs) are a low-cost, safe, and sustainable technology for stationary energy storage. ZABs with pH-buffered near-neutral electrolytes have the potential for longer lifetime compared to traditional alkaline ZABs…

Rechargeable Zn batteries offer safe, inexpensive energy storage, but when deeply discharged to compete with lithium-ion batteries, they are plagued by parasitic reactions at the Zn anodes. We apply super-concentrated alkaline electrolytes…

Materials Science · Physics 2024-05-14 Yilin Ma , Jiajia Huang , Shengyong Gao , iangyu Li , Zhibin Yi , Diwen Xiao , Cheuk Kai Kevin Chan , Ding Pan , Qing Chen

This paper presents a combined theoretical and experimental investigation of aqueous near-neutral electrolytes based on chloride salts for rechargeable zinc-air batteries (ZABs). The resilience of near-neutral chloride electrolytes in air…

Polymer electrolytes present a promising solution to the challenges posed by aqueous electrolytes in energy storage systems, offering the flexibility needed for wearable electronics. Despite the increasing interest in polymer…

Materials Science · Physics 2025-05-06 Roya Rajabi , Shichen Sun , Booker Wu , Jamil Khan , Kevin Huang

Zinc-based batteries offer good volumetric energy densities and are compatible with environmentally friendly aqueous electrolytes. Zinc-ion batteries (ZIBs) rely on a lithium-ion-like Zn$^{2+}$-shuttle, which enables higher roundtrip…

Chemical Physics · Physics 2023-12-11 Niklas J. Herrmann , Holger Euchner , Axel Groß , Birger Horstmann

Electrochemical water electrolysis, which produces clean energy carriers to mitigate carbon emissions, lacks suitable, low-cost electrodes for efficient oxygen evolution reaction (OER) in alkaline water splitting. To address this challenge,…

Aqueous zinc (Zn) batteries (AZBs) face significant challenges due to the limited compatibility of Zn anodes with conventional separators, leading to dendrite growth, hydrogen evolution reaction (HER), and poor cycling stability. While…

Corrosion and the formation of by-products resulting from parasitic side reactions, as well as random dendrite growth, pose significant challenges for aqueous zinc-ion batteries (AZIBs). In this study, phytate ammonium is introduced into…

Applied Physics · Physics 2024-09-04 Fangyuan Xiao , Xiaoke Wang , Kaitong Sun , Qian Zhao , Cuiping Han , Hai-Feng Li

Efficient energy storage systems are crucial to address the intermittency of renewable energy sources. As multivalent batteries, Zn-ion batteries (ZIBs), while inherently low voltage, offer a promising low cost alternative to Li-ion…

Materials Science · Physics 2025-04-17 Roberta Pascazio , Qian Chen , Haoming Howard Li , Aaron D. Kaplan , Kristin A. Persson

Aqueous zinc (Zn)-ion batteries (AZIB) are promising candidates for the next-generation energy store systems due to their high capacity and low cost. Despite their nominal performance, Zn anodes tend to rapidly develop dendrite and…

Materials Science · Physics 2022-09-20 Musanna Galib , Okan K. Orhan , Mauricio Ponga

The parasitic reactions associated with reduced oxygen species and the difficulty in achieving the high theoretical capacity have been major issues plaguing development of practical non-aqueous Li-O2 batteries. We hereby address the above…

"Anode-free" lithium-metal batteries promise significantly higher energy density than conventional graphite-based lithium-ion batteries; however, lithium dendrite growth can lead to internal short circuits with associated safety risks.…

Zinc-based electrochromic devices offer a sustainable route for dynamic optical management but are plagued by poor cycling stability due to irreversible zinc plating/stripping and side reactions. Herein, we report a robust, high-contrast,…

Materials Science · Physics 2026-02-05 Fei Peng , Zhichao Liang , Zhoutao Yang , Yijia Chen , Wenjie Mai , Chuanxi Zhao

Zinc-ion batteries are promising alternatives to lithium-ion batteries, offering advantages in safety, cost, and environmental impact. However, their performance is often limited by the functioning of the zinc anode. This study employs…

Materials Science · Physics 2025-03-31 Xinxin Hu , Shivam Dangwal , Xucheng Wang , Fan Zhang , Haijuan Kong , Jun Li , Kaveh Edalati

Spinel-type LiNi0.5Mn1.5O4 (LNMO) is one of the most promising 5 V-class cathode materials for Li-ion batteries that can achieve high energy density and low production costs. However, in liquid electrolyte cells, the high voltage causes…

We report the synthesis, physical properties and electrochemical performance of Zn substituted Na$_{0.44}$Mn$_{1-x}$Zn$_x$O$_2$ ($x=$ 0 -- 0.02) nanostructures as cathode in Na-ion batteries for energy storage applications. These samples…

Materials Science · Physics 2018-10-18 Mahesh Chandra , Rishabh Shukla , Rakesh Saroha , A. K. Panwar , Amit Gupta , S. Basu , R. S. Dhaka

We report a neutral salt water based battery which uses p-type and n-type solution processed polymer films as the cathode and the anode of the cell. The specific capacity of the electrodes (approximately 30 mAh cm-3) is achieved via…

We present a refined Mn-Zn-H$_2$O Pourbaix diagram with the emphasis on parameters relevant for the Zn/MnO$_2$ rechargeable cells. It maps out boundaries of electrochemical stability for MnO$_2$, ZnMn$_2$O$_4$, ZnMn$_3$O$_7$, and MnOOH. The…

Zn metal battery has been considered a promising alternative energy storage technology in renewable energy storage and grid storage. It is well-known that the surface orientation of a Zn metal anode is vital to the reversibility of a Zn…

Materials Science · Physics 2022-06-13 Ziyi Hu , Linming Zhou , Dechao Meng , Liyan Zhao , Yihua Li , Yuhui Huang , Yongjun Wu , Shikuan Yang , Linsen Li , Zijian Hong

Magnesium sulfate (${ \rm MgSO_4 }$) is used as an additive to reduce capacity fading in rechargeable zinc-ion batteries. This study investigates the ion pairing and solvation structure of ${ \rm Zn^{2+}-SO_4^{2-} }$ and ${ \rm…

Chemical Physics · Physics 2024-10-22 Mayank Dixit , Timir Hajari , Bhalachandra Laxmanrao Tembe
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