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Using first-principles total-energy methods, we investigate Jahn-Teller distortions in III-V dilute magnetic semiconductors, GaAs:Mn and GaN:Mn in the cubic zinc blende structure. The results for an isolated Mn impurity on a Ga site show…

Materials Science · Physics 2009-11-10 Xuan Luo , Richard M. Martin

The silicon-vacancy (SiV) and nitrogen-vacancy (NV) centers in diamond are commonly regarded as prototypical defects for solid-state quantum information processing. Here we show that when silicon and nitrogen are simultaneously introduced…

Negatively-charged nitrogen-vacancy (NV$^-$) color centers in diamond have generated much interest for use in quantum technology. Despite the progress made in developing their applications, many questions about the basic properties of…

We report on a mathematical model of the photoelectric response of NV colour centres in diamond, that can be employed for sensing and quantum science information applications. Although the model applies to NV centre in diamond, it can be…

Quantum Physics · Physics 2026-01-15 Josef Soucek , Michael Petrov , Michal Gulka , Emilie Bourgeois , Milos Nesladek

Vibrational and magnetic properties of single-crystal uranium-thorium dioxide (UxTh1-xO2) with a full range of 0<x<1 is investigated. Thorium dioxide is a diamagnet whose thermal properties are governed by lattice vibration. The addition of…

Vibronic coupling parameters for C$_{60}^{+}$ were derived via DFT calculations with hybrid B3LYP and CAM-B3LYP functional, based on which the static Jahn-Teller effect were analyzed. The global minima of adiabatic potential energy surface…

Chemical Physics · Physics 2020-07-06 Zhishuo Huang , Dan Liu

At 750K, LaMnO_3 has a cooperative Jahn-Teller (JT) distortion, with Mn atoms in distorted oxygen octahedra. This lifts the degeneracy of the singly-occupied $e_g$ orbitals of the Mn$^{3+}$ ions, which then become orbitally ordered. We use…

Strongly Correlated Electrons · Physics 2015-06-25 Vasili Perebeinos , Philip B. Allen

A mechanism of non-magnetic Kondo effect is proposed on the basis of a multiorbital Anderson model coupled with dynamical Jahn-Teller (JT) phonons. An electron system coupled dynamically with JT phonons has a vibronic ground state with…

Strongly Correlated Electrons · Physics 2009-11-11 Takashi Hotta

The nitrogen-vacancy (NV) center is a well utilized system for quantum technology, in particular quantum sensing and microscopy. Fully employing the NV center's capabilities for metrology requires a strong understanding of the behavior of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 M. S. J. Barson , P. M. Reddy , S. Yang , N. B. Manson , J. Wrachtrup , M. W. Doherty

In LiNiO$_2$ Ni$^{3+}$ ion has $d^7$ configuration in cubic crystal field with one electron on double degenerate $e_g$ orbitals, and such ion is considered to be Jahn-Teller (JT) active. However despite the fact, that this compound is an…

Strongly Correlated Electrons · Physics 2019-01-09 Dm. M. Korotin , D. Novoselov , V. I. Anisimov

We created dense ensembles of negatively charged nitrogen-vacancy (NV-) centers in diamond by neutron and electron irradiation for applications in hybrid quantum systems and magnetometry. We characterize fluorescence intensity, optical and…

Electrically-active defects have a significant impact on the performance of electronic devices based on wide band-gap materials such as diamond. This issue is ubiquitous in diamond science and technology, since the presence of charge traps…

We analyze the electronic structure of a mixed-valence ladder system. We find that structural anisotropy and complex electron correlations lead to on-rung charge localization and insulating character. Charge fluctuations within the rung of…

Strongly Correlated Electrons · Physics 2009-11-11 L. Hozoi , S. Nishimoto , A. Yamasaki

This study utilises linear-scaling density functional theory (DFT) and develops a new machine-learning potential for carbon and nitrogen (GAP-CN), based on the carbon potential (GAP20), to investigate the interaction between carbon…

Computational Physics · Physics 2025-01-22 Guangzhao Chen , Joseph C. A. Prentice , Jason M. Smith

Negatively charged nitrogen-vacancy (NV) center in diamond is the representative solid state defect qubit for quantum information science, offering long coherence time at room temperature. To achieve high sensitivity and spatial resolution,…

Materials Science · Physics 2025-08-12 Pei Li , Guanjian Hu , Xiao Yu , Bing Huang , Song Li

The interplay between ion beam modification techniques in the MeV range and the controlled generation of negatively charged nitrogen-vacancy (NV-) centers in nitrogen-doped synthetic diamond crystals is explored. An experimental approach…

We present a micrometer-resolution millimeter-field-of-view stress imaging method for diamonds containing a thin surface layer of nitrogen vacancy (NV) centers. In this method, we reconstruct stress tensor elements over a two-dimensional…

We develop a systematic study of Jahn-Teller (JT) models with continuous symmetries by explor- ing their algebraic properties. The compact symmetric spaces corresponding to JT models carrying a Lie group symmetry are identified, and their…

Chemical Physics · Physics 2018-08-15 Raphael F. Ribeiro , Joel Yuen-Zhou

The quadratic Jahn-Teller effect of C$_{60}^{n-}$ ($n=$ 1-5) is investigated from the first principles. Employing the density functional theory calculations with hybrid functional, the quadratic vibronic coupling constants of C$_{60}^-$…

Strongly Correlated Electrons · Physics 2018-07-03 Dan Liu , Yasuyuki Niwa , Naoya Iwahara , Tohru Sato , Liviu F. Chibotaru

Below its Jahn--Teller transition temperature, $T_\mathrm{JT}$, NaNiO$_2$ has a monoclinic layered structure consisting of alternating layers of edge-sharing NaO$_6$ and Jahn-Teller-distorted NiO$_6$ octahedra. Above $T_\mathrm{JT}$ where…

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