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In this work, we investigate the microscopic mechanisms of anharmonic lattice dynamics and thermal transport in lead-free halide double perovskite Cs2AgBiBr6 from first principles. We combine self-consistent phonon calculations with bubble…

Materials Science · Physics 2024-02-09 Jiongzhi Zheng , Changpeng Lin , Chongjia Lin , Geoffroy Hautier , Ruiqiang Guo , Baoling Huang

The Boltzmann transport equation is one of the most relevant framework to study the heat transport at the nanoscale, beyond the diffusive regime and up to the micrometer-scale. In the general case of three-dimensional devices, the particle…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 B. Davier , J. Larroque , P. Dollfus , L. Chaput , S. Volz , D. Lacroix , J. Saint-Martin

The heat transfer properties of the organic molecular crystal ${\alpha}$-RDX were studied using three phonon-based thermal conductivity models. It was found that the widely used Peierls-Boltzmann model for thermal transport in crystalline…

Materials Science · Physics 2020-07-20 Gaurav Kumar , Francis G. VanGessel , Daniel C. Elton , Peter W. Chung

In this study, we use the transient thermal grating optical technique \textemdash a non-contact, laser-based thermal metrology technique with intrinsically high accuracy \textemdash to investigate room-temperature phonon-mediated thermal…

We investigate the nanoscale mechanisms determining lattice thermal conductivity (LTC) of pristine and W-doped MX$_2$-M$^\prime$X$^\prime_2$ transition metal dichalcogenide heterobilayers from first principles, using the exact solution of…

Materials Science · Physics 2026-04-29 Elliot Perviz , Antonio Cammarata

We perform an ab initio computational investigation of the electronic and thermoelectric transport properties of one of the best performance half-Heusler (HH) alloys, NbFeSb. We use Boltzmann Transport equation while taking into account the…

Materials Science · Physics 2025-10-28 Bhawna Sahni , Yao Zhao , Zhen Li , Rajeev Dutt , Patrizio Graziosi , Neophytos Neophytou

Phonon boundary scattering is typically treated using the Fuchs-Sondheimer theory, which assumes that phonons are thermalized to the local temperature at the boundary. However, whether such a thermalization process actually occurs and its…

Materials Science · Physics 2020-06-26 Navaneetha K. Ravichandran , Austin J. Minnich

The relaxation of a spatially sinusoidal temperature perturbation in a dielectric crystal at a temperature comparable to or higher than the Debye temperature is investigated theoretically. We assume that most phonons contributing to the…

Materials Science · Physics 2011-12-12 A. A. Maznev , Jeremy A. Johnson , Keith A. Nelson

The ab initio model for heat propagation is the phonon transport equation, a Boltzmann-like kinetic equation. When two materials are put side by side, the heat that propagates from one material to the other experiences thermal boundary…

Numerical Analysis · Mathematics 2025-10-13 Irene M Gamba , Qin Li , Anjali Nair

While thermal anisotropicity is a desirable materials property for many applications, including transverse thermoelectrics and thermal management in electronic devices, it remains elusive in practical natural compounds. In this work, we…

Materials Science · Physics 2017-04-05 Giuseppe Romano , Alexie M. Kolpak

For low density gases the validity of the Boltzmann transport equation is well established. The central object is the one-particle distribution function, $f$, which in the Boltzmann-Grad limit satisfies the Boltzmann equation. Grad and,…

Mathematical Physics · Physics 2009-11-11 Herbert Spohn

Heat transfer in layered metal-dielectric structures is considered theoretically based on an analytical solution of the Boltzmann transfer equation for the phonon distribution function. Taking into account the size effect, the problem of…

Materials Science · Physics 2023-11-27 A. I. Bezuglyj , I. V. Mironenko , V. A. Shklovskij

Electronic transport in narrow gap semiconductors is characterized by spontaneous vertical transitions between carriers in the valence and conduction bands, a phenomenon also known as Zener tunneling. However, this effect is not captured by…

Materials Science · Physics 2021-04-21 Andrea Cepellotti , Boris Kozinsky

Heat transport in bulk materials is well described using the Debye theory of 3D vibrational modes (phonons) and the acoustic match model. However, in cryogenic nanodevices, phonon wavelengths exceed device dimensions, leading to confinement…

Mesoscale and Nanoscale Physics · Physics 2024-10-14 M. Sidorova , A. D. Semenov , A. Zaccone , I. Charaev , M. Gonzalez , A. Schilling , S. Gyger , S. Steinhauer

Phonon transport of recently-fabricated $\mathrm{Na_2He}$ at high pressure is investigated from a combination of first-principles calculations and the linearized phonon Boltzmann equation within the single-mode relaxation time approximation…

Materials Science · Physics 2017-05-24 San-Dong Guo , Ai-Xia Zhang

We present a formula for thermal transport in the bulk of Bose systems based on the quantum Boltzmann equation (QBE). First, starting from the quantum kinetic equation and using the Born approximation for impurity scattering, we derive the…

Mesoscale and Nanoscale Physics · Physics 2021-08-09 Kouki Nakata , Yuichi Ohnuma

Surface scattering is the key limiting factor to thermal transport in dielectric crystals as the length scales are reduced or when temperature is lowered. To explain this phenomenon, it is commonly assumed that the mean free paths of heat…

Materials Science · Physics 2017-08-17 Andrea Cepellotti , Nicola Marzari

A discovery of the unusual thermal properties of graphene stimulated experimental, theoretical and computational research directed at understanding phonon transport and thermal conduction in two-dimensional material systems. We provide a…

Materials Science · Physics 2017-02-16 Denis L. Nika , Alexander A. Balandin

The thermal transport properties of biphenylene network (BPN), a novel sp2 -hybridized two-dimensional allotrope of carbon atoms recently realized in experiments [Fan et al., Science, 372 852-856 (2021)], are studied using the density…

Materials Science · Physics 2021-06-08 Harish P. Veeravenkata , Ankit Jain

The electrons and phonons in metal films after ultra-short pulse laser heating are in highly non-equilibrium states not only between the electron sub-system and the phonon sub-system but also within the electron sub-system. An…

Materials Science · Physics 2014-08-05 Jun Zhou , Nianbei Li , Ronggui Yang
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