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Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

High-order harmonic generation (HHG), characterized by its highly nonlinear nature, often exhibits a complex spatio-temporal profile that poses challenges for practical applications. In this study, we unveil a method for manipulating the…

Optics · Physics 2024-12-10 Qi Zeng , Yimin Deng , Xinyue Yang , Wei Cao , Peixiang Lu

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

High-harmonic generation (HHG) is a highly nonlinear optical process that typically requires an intense laser to trigger emissions at integer multiples of the driving field frequency. However, the strong fields required for conventional HHG…

Optics · Physics 2025-12-05 Lu Wang , Andrew M. Parks , Adam Thorpe , Graeme Bart , Giulio Vampa , Thomas Brabec

Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…

Optics · Physics 2024-10-16 Thomas K. Allison , Alice Kunin , Gerd Schönhense

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

High harmonic generation (HHG) enables coherent extreme-ultraviolet (XUV) radiation with ultra-short pulse duration in a table-top setup. This has already enabled a plethora of applications. Nearly all of these applications would benefit…

Optics · Physics 2021-06-07 R. Klas , A. Kirsche , M. Gebhardt , J. Buldt , H. Stark , S. Hädrich , J. Rothhardt , J. Limpert

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

Quantum Physics · Physics 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

We present a quantum optical generalization of the quantum-matter Lewenstein model of high-harmonic generation (HHG) in gases that contains two channels corresponding to the inter- and intraband HHG in solids. Both channels can be presented…

Atomic Physics · Physics 2025-08-21 Adam Thorpe , Neda Boroumand , Graeme Bart , Lu Wang , Giulio Vampa , Thomas Brabec

Real-space picture of electron recollision with the parent ion guides our understanding of the highly nonlinear response of atoms and molecules to intense low-frequency laser fields. It is also among several leading contestants for the…

Optics · Physics 2019-11-06 Mrudul M. S. , Adhip Pattanayak , Misha Ivanov , Gopal Dixit

High harmonic generation (HHG) is an extreme nonlinear frequency up-conversion process during which extremely short duration optical pulses at very short wavelengths are emitted. A major concern of HHG is the small conversion efficiency at…

The enhancement and control of non-linear phenomena at a nanometer scale has a wide range of applications in science and in industry. Among these phenomena, high-harmonic generation in solids is a recent focus of research to realize next…

High harmonic generation (HHG) is a nonlinear process that enables table-top generation of tunable, high-energy, coherent, ultrashort radiation pulses in the extreme ultraviolet (EUV) to soft X-ray range. These pulses find applications in…

We report on the development of a high-order harmonic generation (HHG)-based ultrafast high-repetition-rate (250 kHz) monochromatic extreme ultraviolet (21.6 eV) source with polarization tunability, specifically designed for multi-modal…

High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…

High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Joel D. Cox , Andrea Marini , F. Javier García de Abajo