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We extend the nested sampling algorithm to simulate materials under periodic boundary and constant pressure conditions, and show how it can be used to determine the complete equilibrium phase diagram, for a given potential energy function,…

Reactive chemistry of molecular hydrogen at surfaces, notably dissociative sticking and hydrogen evolution, plays a crucial role in energy storage and fuel cells. Theoretical studies can help to decipher underlying mechanisms and reaction…

Hydrogen atom transfer (HAT) reactions are essential in many biological processes, such as radical migration in damaged proteins, but their mechanistic pathways remain incompletely understood. Simulating HAT is challenging due to the need…

Machine Learning · Computer Science 2025-11-25 Marlen Neubert , Patrick Reiser , Frauke Gräter , Pascal Friederich

Nested sampling is a promising method for calculating phase diagrams of materials, however, the computational cost limits its applicability if ab-initio accuracy is required. In the present work, we report on the efficient use of a…

Materials Science · Physics 2023-08-23 N. Unglert , J. Carrete , L. B. Pártay , G. K. H. Madsen

This work presents a methodology to predict a near-optimal spacing function, which defines the element sizes, suitable to perform steady RANS turbulent viscous flow simulations. The strategy aims at utilising existing high fidelity…

Computational Engineering, Finance, and Science · Computer Science 2024-06-25 Sergi Sanchez-Gamero , Oubay Hassan , Ruben Sevilla

Re-training a deep learning model each time a single data point receives a new label is impractical due to the inherent complexity of the training process. Consequently, existing active learning (AL) algorithms tend to adopt a batch-based…

Machine Learning · Computer Science 2023-12-19 Yunpyo An , Suyeong Park , Kwang In Kim

When we can not assume a large amount of annotated data , active learning is a good strategy. It consists in learning a model on a small amount of annotated data (annotation budget) and in choosing the best set of points to annotate in…

Computer Vision and Pattern Recognition · Computer Science 2022-01-19 Umang Aggarwal , Adrian Popescu , Céline Hudelot

The atomistic modeling of amorphous materials requires structure sizes and sampling statistics that are challenging to achieve with first-principles methods. Here, we propose a methodology to speed up the sampling of amorphous and…

Disordered Systems and Neural Networks · Physics 2018-03-29 Nongnuch Artrith , Alexander Urban , Gerbrand Ceder

Reconfigurable intelligent surface (RIS) is a two-dimensional periodic structure integrated with a large number of reflective elements, which can manipulate electromagnetic waves in a digital way, offering great potentials for wireless…

Machine Learning · Computer Science 2025-01-22 Zhen Zhang , Jun Hui Qiu , Jun Wei Zhang , Hui Dong Li , Dong Tang , Qiang Cheng , Wei Lin

Active learning (AL) has emerged as a crucial methodology for minimizing labeling costs in deep learning by selecting the most valuable samples from a pool of unlabeled data for annotation. Traditional AL operates under a closed-set…

Machine Learning · Computer Science 2026-04-23 Zongyao Lyu , William J. Beksi

We show that the Gaussian Approximation Potential machine learning framework can describe complex magnetic potential energy surfaces, taking ferromagnetic iron as a paradigmatic challenging case. The training database includes total…

Materials Science · Physics 2018-02-07 Daniele Dragoni , Thomas D. Daff , Gabor Csanyi , Nicola Marzari

Materials composed of elements from the third and fifth columns of the periodic table display a very rich behavior, with the phase diagram usually containing a metallic liquid phase and a polar semiconducting solid. As a consequence, it is…

Materials Science · Physics 2022-01-13 Giulio imbalzano , Michele Ceriotti

We propose a novel approach for constructing training databases for Machine-Learned Interatomic Potential (MLIP) models, specifically designed to capture phase properties across a wide range of conditions. The framework is uniquely…

Materials Science · Physics 2025-12-03 Vincent G. Fletcher , Albert P. Bartók , Livia B. Pártay

The formally exact framework of equilibrium Density Functional Theory (DFT) is capable of simultaneously and consistently describing thermodynamic and structural properties of interacting many-body systems in arbitrary external potentials.…

The paucity of labeled data is a typical challenge in the automotive industry. Annotating time-series measurements requires solid domain knowledge and in-depth exploratory data analysis, which implies a high labeling effort. Conventional…

Machine Learning · Computer Science 2023-12-27 Yuqicheng Zhu , Mohamed-Ali Tnani , Timo Jahnz , Klaus Diepold

In this work, we present Enhanced Representation-Based Sampling (ERBS), a novel enhanced sampling method designed to generate structurally diverse training datasets for machine-learned interatomic potentials. ERBS automatically identifies…

Chemical Physics · Physics 2026-01-23 Moritz René Schäfer , Johannes Kästner

To leverage the power of big data from source tasks and overcome the scarcity of the target task samples, representation learning based on multi-task pretraining has become a standard approach in many applications. However, up until now,…

Machine Learning · Computer Science 2022-02-03 Yifang Chen , Simon S. Du , Kevin Jamieson

In this paper, we suggest a novel data-driven approach to active learning (AL). The key idea is to train a regressor that predicts the expected error reduction for a candidate sample in a particular learning state. By formulating the query…

Machine Learning · Computer Science 2017-07-17 Ksenia Konyushkova , Raphael Sznitman , Pascal Fua

Recent successes of Deep Neural Networks (DNNs) in a variety of research tasks, however, heavily rely on the large amounts of labeled samples. This may require considerable annotation cost in real-world applications. Fortunately, active…

Machine Learning · Computer Science 2020-09-08 Qiang Liu , Zhaocheng Liu , Xiaofang Zhu , Yeliang Xiu

Refractory multi-principal element alloys (RMPEAs) represent a novel class of alloys characterized by an extensive compositional design space and the potential for exceptional mechanical performance under extreme conditions. While accurate…

Materials Science · Physics 2026-04-21 A. K. Shargh , C. D. Stiles , J. A. El-Awady