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We investigated the rare-earth triangular-lattice antiferromagnet NdMgAl$_{11}$O$_{19}$ using single-crystal magnetization (1.8~K $\leq T \leq$ 300~K, $\mu_0 H \leq 7$~T) and specific-heat measurements down to 45~mK. The dc susceptibility…

The ytterbium-based delafossite NaYbSe$_2$ is discussed as a prototype for a spin-orbit entangled, effective spin-1/2 triangular spin lattice with emerging antiferromagnetic correlations and a quantum-spin-liquid (QSL) ground state. We…

Strongly Correlated Electrons · Physics 2025-01-08 S. Luther , K. M. Ranjith , Th. Doert , J. Wosnitza , H. Kühne , M. Baenitz

The majority of magnetic materials possess some degree of magnetic anisotropy, either at the level of a single ion, or in the exchange interactions between different magnetic ions. Where these exchange interactions are also frustrated, the…

Strongly Correlated Electrons · Physics 2011-05-18 Luis Seabra , Nic Shannon

Our studies evidence an anisotropic magnetic order below $T_N = 32$~K. Susceptibility data in small fields of about 1~T reveal an antiferromagnetic (AFM) order for $H \perp c$, whereas for $H \parallel c$ the data are reminiscent of a…

We set forth the structural and magnetic properties of the frustrated spin-$5/2$ triangle lattice antiferromagnet Na$_3$Fe(PO$_4$)$_2$ examined via x-ray diffraction, magnetization, heat capacity, and neutron diffraction measurements on the…

Materials Science · Physics 2022-01-26 Sebin J. Sebastian , A. Jain , S. M. Yusuf , M. Uhlarz , R. Nath

Triangular-lattice systems host a variety of ground states, ranging from quantum spin liquids to magnetically ordered phases, the latter of which can exhibit a sequence of magnetic phase transitions under applied magnetic fields. Here, we…

Spin-1/2 antiferromagnetic triangular lattice models are paradigms of geometrical frustration, revealing very different ground states and quantum effects depending on the nature of anisotropies in the model. Due to strong spin orbit…

Recently, several putative quantum spin liquid (QSL) states were discovered in ${\tilde S} = 1/2$ rare-earth based triangular-lattice antiferromagnets (TLAF) with the delafossite structure. A way to clarify the origin of the QSL state in…

Magnetism of the $S$ = 1 Heisenberg antiferromagnets on the spatially anisotropic square lattice has been scarcely explored. Here we report a study of the magnetism, specific heat, and thermal conductivity on Ni[SC(NH$_2$)$_2$]$_6$Br$_2$…

Materials Science · Physics 2019-03-15 X. Zhao , Z. Y. Zhao , L. M. Chen , X. Rao , H. L. Che , L. G. Chu , H. D. Zhou , L. S. Ling , J. F. Wang , X. F. Sun

We report the physical properties of $R$Cd$_{3}$As$_{3}$ ($R$ = La and Ce) compounds, crystallized into a hexagonal ScAl$_{3}$C$_{3}$-type structure ($P$6$_{3}$/mmc) such that the $R$ sublattice forms a spin-orbit coupled triangular…

Strongly Correlated Electrons · Physics 2022-06-15 S. R. Dunsiger , J. Lee , J. E. Sonier , E. D. Mun

We report the revised crystal structure, static and dynamic magnetic properties of quasi-two dimensional honeycomb-lattice silver delafossite Ag3Co2SbO6. The magnetic susceptibility and specific heat data are consistent with the onset of…

Electrical resistivity ($\rho$), magnetoresistance (MR), magnetization, thermopower and Hall effect measurements on the single crystal Gd$_{2}$PdSi$_3$, crystallizing in an AlB$_2$-derived hexagonal structure are reported. The well-defined…

Strongly Correlated Electrons · Physics 2009-10-31 S. R. Saha , H. Sugawara , T. D. Matsuda , H. Sato , R. Mallik , E. V. Sampathkumaran

We investigate the magnetic interactions in triangular rare-earth delafossites materials NaYbO$_2$ and NaYbS$_2$ via first-principles calculations. The calculated Curie-Weiss temperatures are in good agreement with experiments. We perform…

Materials Science · Physics 2021-04-21 Da-Ye Zheng , Zhen-Xiong Shen , Meng Zhang , Lixin He

We have performed high-field magnetization and ESR measurements on Ba$_3$CoSb$_2$O$_9$ single crystals, as a representative two-dimensional spin-1/2 Heisenberg antiferromagnet on a uniform triangular lattice, and have determined all the…

Strongly Correlated Electrons · Physics 2015-06-15 Takuya Susuki , Nobuyuki Kurita , Takuya Tanaka , Hiroyuki Nojiri , Akira Matsuo , Koichi Kindo , Hidekazu Tanaka

We present an experimental study of macroscopic and microscopic magnetic anisotropy of a spin tetramer system \cso using torque magnetometry and ESR spectroscopy. Large rotation of macroscopic magnetic axes with temperature observed from…

Strongly Correlated Electrons · Physics 2016-08-08 Mirta Herak , Dijana Žilić , Dubravka Matković Čalogović , Helmuth Berger

The determination of Lande's g-factor and the damping constant is central to extracting crucial information about the spin-spin and spin-orbit interactions in magnetically ordered systems. In insulating compounds based on 3d elements, the…

Materials Science · Physics 2025-02-04 Alapan Bera , Nirmalya Jana , Amit Agarwal , Soumik Mukhopadhyay

While the Heisenberg model for magnetic Mott insulators on planar lattice structures is comparatively well understood in the case of transition metal ions, the intrinsic spin-orbit entanglement of 4f magnetic ions on such lattices shows…

Strongly Correlated Electrons · Physics 2021-06-29 B. Schmidt , J. Sichelschmidt , K. M. Ranjith , Th. Doert , M. Baenitz

The results of dc and ac magnetization, electrical resistance and heat capacity studies in an admixed rare earth alloy Nd0.75Gd0.25Rh3B2, which is close to the zero magnetization limit, are reported. Novel observations include the two…

Strongly Correlated Electrons · Physics 2019-08-15 Prasanna D. Kulkarni , U. V. Vaidya , V. C. Rakhecha , A. Thamizhavel , S. K. Dhar , A. K. Nigam , S. Ramakrishnan , A. K. Grover

We successfully synthesize single crystals of the verdazyl radical $\alpha$-2,3,5-Cl$_3$-V. $Ab$ $initio$ molecular orbital calculations indicate that the two dominant antiferromagnetic interactions, $J_{\rm{1}}$ and $J_{\rm{2}}$ ($\alpha…

Strongly Correlated Electrons · Physics 2017-06-26 Hironori Yamaguchi , Yusuke Tamekuni , Yoshiki Iwasaki , Rei Otsuka , Yuko Hosokoshi , Takanori Kida , Masayuki Hagiwara

We examine the anisotropic properties of the exchange stiffness constant, $\mathcal{A}$, for rare-earth permanent magnet, Nd$_2$Fe$_{14}$B, by connecting analyses with two different scales of length, i.e., Monte Carlo (MC) method with an…

Materials Science · Physics 2018-08-22 Yuta Toga , Masamichi Nishino , Seiji Miyashita , Takashi Miyake , Akimasa Sakuma
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