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The past 15 years have seen an astonishing increase in Nuclear Magnetic Resonance (NMR) sensitivity and accessible pressure range in high-pressure NMR experiments, owing to a series of new developments of NMR spectroscopy applied to the…

Spin defects in semiconductors are widely investigated for various applications in quantum sensing. Conventional host materials such as diamond and hexagonal boron nitride (hBN) provide bulk or low-dimensional platforms for optically…

Color centers in hexagonal boron nitride (hBN) have recently emerged as promising candidates for a new wave of quantum applications. Thanks to hBN's high stability and 2-dimensional (2D) layered structure, color centers in hBN can serve as…

Quantum Physics · Physics 2023-05-02 Sumukh Vaidya , Xingyu Gao , Saakshi Dikshit , Igor Aharonovich , Tongcang Li

Nuclear spins in solids offer a promising avenue for developing scalable quantum hardware. Leveraging nearby single-color centers, these spins can be efficiently addressed at the single-site level through spin resonance. However,…

Quantum Physics · Physics 2024-02-14 Majid Zahedian , Vadim Vorobyov , Jörg Wrachtrup

Nitrogen-vacancy centers in diamond are a promising platform for nanoscale nuclear magnetic resonance sensing. Despite significant progress towards using NV centers to detect and localize nuclear spins down to the single spin level,…

We show that high-resolution NMR can reach picomole sensitivity for micromolar concentrations of analyte by combining parahydrogen induced hyperpolarisation (PHIP)with a high-sensitivity transmission line micro-detector. The para-enriched…

Chemical Physics · Physics 2019-05-20 James Eills , William Hale , Manvendra Sharma , Matheus Rossetto , Malcolm H. Levitt , Marcel Utz

Performing nanoscale scanning electron paramagnetic resonance (EPR) requires three essential ingredients. First, a static magnetic field together to field gradients to Zeeman split the electronic energy levels with spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2024-01-16 Carlos A. González-Gutiérrez , David García-Pons , David Zueco , María José Martínez-Pérez

Spins bound to point defects are increasingly viewed as an important resource for solid-state implementations of quantum information technologies. In particular, there is a growing interest in the identification of new classes of defect…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 William F. Koehl , Berk Diler , Samuel J. Whiteley , Alexandre Bourassa , N. T. Son , Erik Janzén , David D. Awschalom

We report detection of nuclear magnetic resonance (NMR) using an anisotropic magnetoresistive (AMR) sensor. A ``remote-detection'' arrangement was used, in which protons in flowing water were pre-polarized in the field of a superconducting…

Chemical Physics · Physics 2015-05-13 F. Verpillat , M. P. Ledbetter , D. Budker , S. Xu , D. Michalak , C. Hilty , S. Antonijevic , A. Pines , L. -S. Bouchard

Microfluidic NMR spectroscopy can probe chemical and bio-chemical processes non-invasively in a tightly controlled environment. We present a dual-channel modular probe assembly for high efficiency microfluidic NMR spectroscopy and imaging.…

Instrumentation and Detectors · Physics 2019-05-22 Manvendra Sharma , Marcel Utz

Magnetic resonance imaging (MRI) is a non-invasive and label-free technique widely used in medical diagnosis and life science research, and its success has benefited greatly from continuing efforts on enhancing contrast and resolution. Here…

Magnetic resonance imaging (MRI) revolutionized diagnostic medicine and biomedical research by allowing a noninvasive access to spin ensembles. To enhance MRI resolution to the nanometer scale, new approaches including scanning probe…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 Philip Willke , Kai Yang , Yujeong Bae , Andreas J. Heinrich , Christopher P. Lutz

We report a method for nanometer-scale pulsed nuclear magnetic resonance imaging and spectroscopy. Periodic radiofrequency pulses are used to create temporal correlations in the statistical polarization of a solid organic sample. The spin…

Mesoscale and Nanoscale Physics · Physics 2013-10-01 John M. Nichol , Tyler R. Naibert , Eric R. Hemesath , Lincoln J. Lauhon , Raffi Budakian

The field of nanoscale magnetic resonance imaging (NanoMRI) was started 30 years ago. It was motivated by the desire to image single molecules and molecular assemblies, such as proteins and virus particles, with near-atomic spatial…

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

We present theoretical proposals for two-dimensional nuclear magnetic resonance spectroscopy protocols based on Nitrogen-vacancy (NV) centers in diamond that are strongly coupled to the target nuclei. Continuous microwave and…

Quantum Physics · Physics 2024-10-31 Matthias Kost , Jianming Cai , Martin B. Plenio

Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the…

Quantum Physics · Physics 2022-03-01 Min Jiang , Teng Wu , John W. Blanchard , Guanru Feng , Xinhua Peng , Dmitry Budker

Nitrogen-vacancy (NV) centers in diamond have emerged as valuable tools for sensing and polarizing spins. Motivated by potential applications in chemistry, biology, and medicine, we show that NV-based sensors are capable of detecting single…

Quantum Physics · Physics 2016-03-10 M. Bruderer , P. Fernández-Acebal , R. Aurich , M. B. Plenio

Optically accessible spin-active nanomaterials are promising as quantum nanosensors for probing biological samples. However, achieving bioimaging-level brightness and high-quality spin properties for these materials is challenging and…

Molecular Nanomagnets have attracted the attention of the scientific community since the rich physics behind their magnetic behaviour make them ideal test-beds for fundamental concepts in quantum mechanics. Sophisticated experiments and…

Mesoscale and Nanoscale Physics · Physics 2021-01-19 Elena Garlatti , Alessandro Chiesa , Tatiana Guidi , Giuseppe Amoretti , Paolo Santini , Stefano Carretta