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We report on the isolation of single SiV$^-$ centers in nanodiamonds. We observe the fine-structure of single SiV$^-$ center with improved inhomogeneous ensemble linewidth below the excited state splitting, stable optical transitions, good…

We present a rigorous theoretical model for the optical interaction between a nitrogen-vacancy (NV) centre in diamond and a plasmonic metal nanoparticle (MNP), accompanied by a computationally efficient procedure to solve the evolution. The…

Mesoscale and Nanoscale Physics · Physics 2022-02-11 Harini Hapuarachchi , Francesco Campaioli , Jared H. Cole

High biocompatibility, variable size ranging from ~ 5 nm, stable luminescence from its color centers and simple carbon chemistry for biomolecule grafting make nanodiamond (ND) particles an attractive alternative to molecular dyes for…

Conventional nuclear magnetic resonance (NMR) spectroscopy relies on acquiring signal from a macroscopic ensemble of molecules to gain information about molecular structure and dynamics. Transferring this technique to nanoscale sample sizes…

Mesoscale and Nanoscale Physics · Physics 2019-02-06 Jeffrey Holzgrafe , Qiushi Gu , Jan Beitner , Dhiren Kara , Helena S. Knowles , Mete Atatüre

Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the…

Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a…

Quantum Physics · Physics 2013-09-11 J. H. Shim , B. Nowak , I. Niemeyer , J. Zhang , F. D. Brandao , D. Suter

The nitrogen-vacancy (NV) defect center in diamond has demonstrated great capability for nanoscale magnetic sensing and imaging for both static and periodically modulated target fields. However, it remains a challenge to detect and image…

Mesoscale and Nanoscale Physics · Physics 2014-09-19 Lan Luan , Michael S. Grinolds , Sungkun Hong , Patrick Maletinsky , Ronald L. Walsworth , Amir Yacoby

We probe the relaxation dynamics of the full three-level spin system of near-surface nitrogen-vacancy (NV) centers in diamond to define a $T_{1}$ relaxation time that helps resolve the $T_{2} \leq 2T_{1}$ coherence limit of the NV's subset…

Mesoscale and Nanoscale Physics · Physics 2017-05-17 Bryan A. Myers , Amila Ariyaratne , Ania C. Bleszynski Jayich

The protocols for the control and readout of Nitrogen Vacancy (NV) centres electron spins in diamond offer an advanced platform for quantum computation, metrology and sensing. These protocols are based on the optical readout of photons…

Mesoscale and Nanoscale Physics · Physics 2019-06-26 E. Bourgeois , A. Jarmola , M. Gulka , J. Hruby , D. Budker , M. Nesladek

In drug discovery research there is a clear and urgent need for non-invasive detection of cell membrane ion channel operation with wide-field capability. Existing techniques are generally invasive, require specialized nano structures, or…

We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

We demonstrate an all-optical method for magnetic sensing of individual molecules in ambient conditions at room temperature. Our approach is based on shallow nitrogen-vacancy (NV) centers near the surface of a diamond crystal, which we use…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. O. Sushkov , N. Chisholm , I. Lovchinsky , M. Kubo , P. K. Lo , S. D. Bennett , D. Hunger , A. Akimov , R. L. Walsworth , H. Park , M. D. Lukin

The electrical conductivity of a material can feature subtle, nontrivial, and spatially-varying signatures with critical insight into the material's underlying physics. Here we demonstrate a conductivity imaging technique based on the…

Mesoscale and Nanoscale Physics · Physics 2018-06-26 Amila Ariyaratne , Dolev Bluvstein , Bryan A. Myers , Ania C. Bleszynski Jayich

Thanks to their versatility, nitrogen-vacancy (NV) centers in nanodiamonds have been widely adopted as nanoscale sensors. However, their sensitivities are limited by their short coherence times relative to NVs in bulk diamond. A more…

Mesoscale and Nanoscale Physics · Physics 2020-03-09 Aedan Gardill , Matthew C. Cambria , Shimon Kolkowitz

The negatively-charged nitrogen-vacancy (NV) center in diamond has been shown recently as an excellent sensor for external spins. Nevertheless, their optimum engineering in the near-surface region still requires quantitative knowledge in…

Mesoscale and Nanoscale Physics · Physics 2016-03-08 F. Favaro de Oliveira , S. A. Momenzadeh , D. Antonov , J. Scharpf , C. Osterkamp , B. Naydenov , F. Jelezko , A. Denisenko , J. Wrachtrup

New schemes that exploit the unique properties of Nitrogen-Vacancy (NV) centers in diamond are presently being explored as a platform for high-resolution magnetic sensing. Here we focus on the ability of a NV center to monitor an adjacent…

Mesoscale and Nanoscale Physics · Physics 2011-10-12 Abdelghani Laraoui , Jonathan S. Hodges , Colm Ryan , Carlos A. Meriles

Chemical sensors with high sensitivity that can be used in extreme conditions and can be miniaturized are of high interest in science and industry. The Nitrogen-vacancy (NV) center in diamond is an ideal candidate as a nanosensor due to the…

Quantum Physics · Physics 2021-02-16 Hossein T. Dinani , Enrique Muñoz , Jeronimo R. Maze

Nitrogen-Vacancy (NV) centers in diamond have been used in recent years for a wide range of applications, from nano-scale NMR to quantum computation. These applications depend strongly on the efficient readout of the NV center's spin state,…

Quantum Physics · Physics 2019-10-02 Idan Meirzada , Sigal A. Wolf , Alex Naiman , Uriel Levy , Nir Bar-Gill

Single-molecule technology stands as a powerful tool, enabling the characterization of intricate structural and dynamic information that would otherwise remain concealed within the averaged behaviors of numerous molecules. This technology…

Quantum Physics · Physics 2025-01-08 Jiangfeng Du , Fazhan Shi , Xi Kong , Fedor Jekezko , Jörg Wrachtrup

Hands-on experimental experience with quantum systems in the undergraduate physics curriculum provides students with a deeper understanding of quantum physics and equips them for the fast-growing quantum science industry. Here we present an…

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