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We develop a phenomenological theory to predict the characteristic features of the momentum-dependent scattering amplitude in resonant inelastic x-ray scattering (RIXS) at the energy scale of the superconducting gap in iron-based…

Superconductivity · Physics 2016-05-10 Pasquale Marra , Jeroen van den Brink , Steffen Sykora

We present a resonant inelastic x-ray scattering (RIXS) study of spin and charge excitations in overdoped La1.77Sr0.23CuO4 along two high-symmetry directions. The line shape of these excitations is analyzed and they are shown to be highly…

Superconductivity · Physics 2016-02-05 C. Monney , T. Schmitt , C. E. Matt , J. Mesot , V. N. Strocov , O. J. Lipscombe , S. M. Hayden , J. Chang

We use Ru $L_3$-edge (2838.5 eV) resonant inelastic x-ray scattering (RIXS) to quantify the electronic structure of Ca$_2$RuO$_4$, a layered $4d$-electron compound that exhibits a correlation-driven metal-insulator transition and…

Strongly Correlated Electrons · Physics 2019-07-24 H. Gretarsson , H. Suzuki , Hoon Kim , K. Ueda , M. Krautloher , B. J. Kim , H. Yavaş , G. Khaliullin , B. Keimer

Transition Edge Sensor (TES) spectrometers for hard X-ray beamline science will enable improved X-ray emission and absorption spectroscopy in the information-rich 2 to 20 keV energy range. We are building a TES-based instrument for the…

Instrumentation and Detectors · Physics 2020-08-26 Tejas Guruswamy , Lisa M. Gades , Antonino Miceli , Umeshkumar M. Patel , John T. Weizeorick , Orlando Quaranta

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge density wave order,…

Strongly Correlated Electrons · Physics 2017-07-03 T. P. Devereaux , A. M. Shvaika , K. Wu , K. Wohlfeld , C. J. Jia , Y. Wang , B. Moritz , L. Chaix , W. -S. Lee , Z. -X. Shen , G. Ghiringhelli , L. Braicovich

Ruddlesden-Popper and reduced Ruddlesden-Popper nickelates are intriguing candidates for mimicking the properties of high-temperature superconducting cuprates. The degree of similarity between these nickelates and cuprates has been the…

A detailed tight-binding analysis of the electron band structure of the CuO_2 plane of layered cuprates is performed within a sigma-band Hamiltonian including four orbitals - Cu3d_x^2-y^2, Cu4s, O2p_x, and O2p_y. Both the experimental and…

Superconductivity · Physics 2009-10-31 T. Mishonov , E. Penev

We propose two possible new compounds, Ba$_2$CuO$_2$Fe$_2$As$_2$ and K$_2$CuO$_2$Fe$_2$Se$_2$, which hybridize the building blocks of two high temperature superconductors, cuprates and iron-based superconductors. These compounds consist of…

Superconductivity · Physics 2016-06-14 Xia Dai , Congcong Le , Xianxin Wu , Jiangping Hu

We report resonant inelastic x-ray measurements of insulating La$_2$CuO$_4$ and Sr$_2$CuO$_2$Cl$_2$ taken with the incident energy tuned near the Cu K absorption edge. We show that the spectra are well described in a shakeup picture in 3rd…

Strongly Correlated Electrons · Physics 2009-10-31 P. Abbamonte , C. A. Burns , E. D. Isaacs , P. M. Platzman , L. L. Miller , S. W. Cheong , M. V. Klein

We present theoretical study of relative stability as well as of the magnetic and electronic properties of AgF2 and CuF2, in two related structural forms: orthorhombic (ambient pressure form of AgF2) and monoclinic (ambient pressure form of…

Materials Science · Physics 2024-03-28 Daniel Jezierski , Wojciech Grochala

This paper presents a simple formalism for calculating X-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) that has as input orbital-resolved density of states from a single-particle or many-body \textit{ab initio}…

Strongly Correlated Electrons · Physics 2023-04-18 M. R. Norman , A. S. Botana , J. Karp , A. Hampel , H. LaBollita , A. J. Millis , G. Fabbris , Y. Shen , M. P. M. Dean

How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering…

Strongly Correlated Electrons · Physics 2015-02-27 C. J. Jia , E. A. Nowadnick , K. Wohlfeld , Y. F. Kung , C. -C. Chen , S. Johnston , T. Tohyama , B. Moritz , T. P. Devereaux

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…

We present a relativistic time-dependent density functional theory (TDDFT) approach for the simulation of resonant inelastic X-ray scattering (RIXS) spectra, based on both a full four-component (4c) Dirac-Coulomb Hamiltonian and a modern…

Chemical Physics · Physics 2026-04-17 Lukas Konecny , Muhammed A. Dada , Daniel R. Nascimento , Michal Repisky

Group IB metal halides (CuX and AgX, X=Cl, Br and I) are widely used in optoelectronic devices and photochemical catalysis due to their appropriate optical and electronic properties. First-principles calculations have confronted…

Materials Science · Physics 2019-11-27 Min-Ye Zhang , Hong Jiang

High resolution angle-resolved photoemission spectroscopy (ARPES) measurements are carried out on CaKFe$_4$As$_4$, KCa$_2$Fe$_4$As$_4$F$_2$ and (Ba$_{0.6}$K$_{0.4}$)Fe$_2$As$_2$ superconductors. Clear evidence of band folding between the…

Our investigation explores the intricate domain of thermoelectric phenomena within silver (Ag)-infused chalcopyrites, focusing on compositions such as AgXTe$_2$ (where X=Ga, In) and the complex quaternary system Ag$_2$ZnSn/GeY$_2$ (with…

Materials Science · Physics 2025-06-09 Dimple Rani , Subarata Jana , Manish Kumar Niranjan , Prasanjit Samal

Resonant X-ray scattering (RXS) is a spectroscopy where both the power of site selective diffraction and the power of local absorption spectroscopy regarding atomic species are combined. By virtue of the dependence on the core level state…

Materials Science · Physics 2007-11-12 Yves Joly , Elena S. Nazarenko , José-Emilio Lorenzo , Sergio Di Matteo , Calogero R. Natoli

We report a resonant inelastic x-ray scattering (RIXS) study of charge excitations in the electron-doped high-Tc superconductor Nd1.85Ce0.15CuO4. The intraband and interband excitations across the Fermi energy are separated for the first…

Strongly Correlated Electrons · Physics 2007-05-23 K. Ishii , K. Tsutsui , Y. Endoh , T. Tohyama , S. Maekawa , M. Hoesch , K. Kuzushita , M. Tsubota , T. Inami , J. Mizuki , Y. Murakami , K. Yamada

The importance of electronic correlation effects in the layered perovskite Sr$_2$RuO$_4$ is evidenced. To this end we use state-of-the-art LDA+DMFT (Local Density Approximation + Dynamical Mean-Field Theory) in the basis of Wannier…

Strongly Correlated Electrons · Physics 2007-05-23 Z. V. Pchelkina , I. A. Nekrasov , Th. Pruschke , A. Sekiyama , S. Suga , V. I. Anisimov , D. Vollhardt