Related papers: Dark-State-Mediated Efficient Energy Trapping in a…
Photophoretic forces - which are of thermal origin - have defined an alternative route of optical trapping of absorbing microparticles in air. Here, we show that a single multi-mode fiber facilitates significantly more robust optical traps…
Light harvesting as the first step in photosynthesis is of prime importance for life on earth. For a theoretical description of photochemical processes during light harvesting, spectral densities are key quantities. They serve as input…
Pi-conjugated segments - chromophores - constitute the electronically active units of polymer materials used in organic electronics. To elucidate the effect of bending of these linear moieties on elementary electronic properties such as…
Relativistic coupled-cluster calculations of the ionization potential, dissociation energy, and excited electronic states under 35,000 cm$^{-1}$ are presented for the actinium monofluoride (AcF) molecule. The ionization potential is…
Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…
A two-state model Hamiltonian is proposed to model the coupling of twisting displacements to charge-transfer behavior in the ground and excited states of a general monomethine dye molecule. This coupling may be relevant to the molecular…
Understanding light-induced hidden orders is relevant for nonequilibrium materials control and future ultrafast technologies. Hidden superconducting order, in particular, has been a focus of recent experimental and theoretical efforts. In…
Confining electromagnetic energy is crucial to enhance light-matter interactions, with important implications for science and technology. Here, we discuss the opportunities offered by trapping and confining light in open structures, based…
Harnessing the interaction between light and matter at the quantum level has been a central theme in atomic physics and quantum optics, with applications from quantum computation to quantum metrology. Combining complex interactions with…
Efficient devices for light harvesting and photon sensing are fundamental building blocks of basic energy science and many essential technologies. Recent efforts have turned to biomimicry to design the next generation of light-capturing…
We report the radiation trapping effect inside a hollow-core photonic crystal fiber (PCF). An optical dipole trap was used to load and confine the atoms in the PCF without contacting the wall of the fiber. The transmission of a probe light…
A novel effective Hamiltonian in the subspace of singly occupied states is obtained by applying the Gutzwiller projection approach to a generalized Hubbard model with the interactions between two nearest- neighbor sites. This model provides…
We study the formation and destabilization of dark states in a single trapped 88Sr+ ion caused by the cooling and repumping laser fields required for Doppler cooling and fluorescence detection of the ion. By numerically solving the…
By combining complementary optical techniques, photoluminescence and time-resolved excited state absorption, we achieve a comprehensive picture of the relaxation processes in the organic/inorganic hybrid system SP6/ZnO. We identify two…
We show that it is possible to ``store'' quantum states of single-photon fields by mapping them onto {\it collective} meta-stable states of an optically dense, coherently driven medium inside an optical resonator. An adiabatic technique is…
A bacterial photosynthetic light harvesting complex PLHC absorbs a photon and transfers this energy almost perfectly at room temperature RT to a Reaction Center RC, where charge separation occurs. While there are a number of possible light…
Using a combined theoretical and experimental approach, we investigate the non-adiabatic dynamics of the prototypical ethylene (C2H4) molecule upon {\pi} \to {\pi}* excitation. In this first part of a two part series, we focus on the…
The coherent interaction of light with matter imprints the phase information of the light field on the wavefunction of the photon-dressed electronic state. Driving electric field, together with a stable phase that is associated with the…
Quanta emitted by an open quantum system carry information about intrinsic parameters, enabling their estimation via continuous monitoring. In practice, however, only a fraction of the emitted quanta is detected, reducing the achievable…
The conversion of optical and electrical energy in novel materials is key to modern optoelectronic and light-harvesting applications. Here, we investigate the equilibration dynamics of photoexcited…