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Full coherent soft X-ray attosecond pulses are now available through high-order harmonic generation (HHG); however, its insufficient output energy hinders various applications, such as attosecond-scale soft X-ray nonlinear experiments, the…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

Atomic and Molecular Clusters · Physics 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

We report on the new optical gating technique used for the direct photoconductive detection of short pulses of terahertz radiation with the resolution up to 250 femtoseconds. The femtosecond optical laser pulse time delayed with respect to…

Materials Science · Physics 2016-06-29 A. Muraviev , A. Gutin , G. Rupper , S. Rudin , X. Shen , Y. Yamaguchi , G. Aizin , M. Shur

We present a method of performing high-speed rotational anisotropy nonlinear optical harmonic generation experiments at rotational frequencies of several hertz by projecting the harmonic light reflected at different angles from a sample…

Materials Science · Physics 2015-10-15 J. W. Harter , L. Niu , A. J. Woss , D. Hsieh

Extreme ultraviolet (XUV) transient absorption (TA) and transient reflectivity (TR) spectroscopies enable element-specific insights into attosecond-timescale processes in solids. XUV transient grating spectroscopy (TGS) is an emerging tool…

Small Angle-X-ray Scattering Tensor Tomography (SAS-TT) is a relatively new, but powerful technique for studying the multiscale architecture of hierarchical structures, which is of particular interest for life science applications.…

Core excitons in solids have garnered increasing interest, yet their behavior and decay mechanisms are not fully understood. Here, we use attosecond extreme ultraviolet (XUV) transient absorption spectroscopy, performed with a broadband…

Materials Science · Physics 2023-11-07 Rafael Quintero-Bermudez Stephen R. Leone

Time- and angle-resolved photoelectron spectroscopy (trARPES) employing a 500 kHz extreme-ultravioled (XUV) light source operating at 21.7 eV probe photon energy is reported. Based on a high-power ytterbium laser, optical parametric chirped…

Instrumentation and Detectors · Physics 2019-02-14 M. Puppin , Y. Deng , C. W. Nicholson , J. Feldl , N. B. M. Schroeter , H. Vita , P. S. Kirchmann , C. Monney , L. Rettig , M. Wolf , R. Ernstorfer

Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time…

Electrons in atoms and molecules move on attosecond time scales. Deciphering their quantum dynamics in space and time calls for high-resolution microscopy at this speed. While scanning tunnelling microscopy (STM) driven with terahertz…

Femtosecond transient soft X-ray Absorption Spectroscopy (XAS) is a very promising technique that can be employed at X-ray Free Electron Lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here we…

Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time. What began as a technological breakthrough - generating…

Optics · Physics 2026-04-17 Rocio Borrego Varillas , Pierre Agostini , Fernando Ardana-Lamas , Cord L. Arnold , David Ayuso , Maurizio Reduzzi , Jakub Benda , Jens Biegert , Charles Bourassin-Bouchet , Thomas Brabec , Christian Brahms , Andrew C. Brown , David Busto , Jérémie Caillat , Francesca Calegari , Carlo Callegari , Stefanos Carlström , Zenghu Chang , Ming-Chang Chen , Anna G. Ciriolo , Paul Corkum , Gabriele Crippa , Rafael de Q. Garcia , Louis DiMauro , Nirit Dudovich , Per Eng-Johnsson , Davide Faccialà , Philip Flores , Titouan Gadeyne , Gianluca Aldo Geloni , Chase Geirger , Shima Gholam-Mirzaei , Jimena D. Gorfinkiel , Eleftherios Goulielmakis , Mohammed Hassan , Carlos Hernández-García , Phay Ho , Dandan Hui , Lynda R. Hutcheson , Misha Ivanov , Subhendu Kahaly , Henry Kapteyn , Nicholas Karpowicz , Franz X. Kärtner , Matthias Kling , Omer Kneller , Dong Hyuk Ko , Peter M. Kraus , Maximilian Kubullek , Stephen R. Leone , Franck Lépine , Anne L'Huillier , Chen-Ting Liao , Thomas Linker , Alexander Gabriel Lohr , Matteo Lucchini , Lars Bojer Madsen , Roland E. Mainz , Balázs Major , Jon P. Marangos , David Marco , Hugo Marroux , Sean Marshallsay , Rebeca Martínez Vázquez , Rodrigo Martín-Hernández , Zdeněk Mašín , Michael Meyer , Felipe Morales Moreno , Margaret Murnane , Daniel M. Neumark , Mauro Nisoli , Marcus Ossiander , Sreelakshmi Palakka , Serguei Patchkovskii , Zekun Pi , Luis Plaja , Julita Poborska , Miguel A. Porras , Kevin C. Prince , David N. Purschke , Nicolette G. Puskar , Giulio Maria Rossi , Jérémy R. Rouxel , Thierry Ruchon , Patrick Rupprecht , Pascal Salières , Giuseppe Sansone , Fabian Scheiba , Martin Schultze , Bernd Schütte , Svitozar Serkez , Miguel A. Silva-Toledo , Olga Smirnova , Salvatore Stagira , Andrea Trabattoni , John C. Travers , Igor Tyulnev , Morgane Vacher , Giulio Vampa , Hugo W. van der Hart , Katalin Varjú , Anne-Lise Viotti , Vartika Vishnoi , Marc Vrakking , Vincent Wanie , Stefan Witte , Fei Xu , Vladislav S. Yakovlev , Linda Young , Diling Zhu , Caterina Vozzi

High-resolution Fourier-transform spectroscopy using table-top sources in the extreme ultraviolet (XUV) spectral range is still in its infancy. In this contribution a significant advance is presented based on a Michelson-type all-reflective…

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie

The almost unexplored frequency window from submillimeter to mid-infrared (mid-IR) may bring new clues about the particle acceleration and transport processes and the atmospheric thermal response during solar flares. Because of its…

Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…

Atomic Physics · Physics 2013-05-14 Stefan Pabst

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

Atomic Physics · Physics 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost
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