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Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

Atomic Physics · Physics 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

We realize a continuous guided beam of cold deuterated ammonia with a flux of 3e11 ND3 molecules/s and a continuous free-space beam of cold potassium with a flux of 1e16 K atoms/s. A novel feature of the buffer gas source used to produce…

Atomic Physics · Physics 2015-05-13 David Patterson , Julia Rasmussen , John M. Doyle

We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. The beam is formed by…

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

Atomic Physics · Physics 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

A cryogenic neon solid doped with barium monofluoride (BaF) is created on a cryogenic substrate using a stream of Ne gas and a high-intensity beam of BaF molecules produced in a cryogenic helium-buffer-gas laser-ablation source. The…

Cryogenically cooled buffer gas beam sources of the molecule thorium monoxide (ThO) are optimized and characterized. Both helium and neon buffer gas sources are shown to produce ThO beams with high flux, low divergence, low forward…

A novel two-stage helium buffer gas cooled beam source is introduced. The properties of the molecular beams produced from this source are investigated theoretically using the CaF as a test molecule. The gas-phase molecules are first…

Atomic Physics · Physics 2020-04-14 Vijay Singh

We present a combined experimental and theoretical study of beam formation from a cryogenic buffer gas cell. Atoms and molecules are loaded into the cell by laser ablation of a target, and are cooled and swept out of the cell by a flow of…

Atomic Physics · Physics 2017-09-13 N. E. Bulleid , S. M. Skoff , R. J. Hendricks , B. E. Sauer , E. A. Hinds , M. R. Tarbutt

We study the properties of a cryogenic buffer gas source that uses a low temperature two-stage buffer gas cell to produce very slow beams of ytterbium monofluoride molecules. The molecules are produced by laser ablation inside the cell and…

Atomic Physics · Physics 2024-11-19 A. D. White , S. Popa , J. Mellado-Munoz , N. J. Fitch , B. E. Sauer , J. Lim , M. R. Tarbutt

We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation…

Atomic Physics · Physics 2017-03-22 Wenhao Bu , Tao Chen , Guitao Lv , Bo Yan

We demonstrate a cryogenic buffer gas-cooled molecular beam source capable of producing bright, continuous beams of cold and slow free radicals via laser ablation over durations of up to 60~seconds. The source design uses a closed liquid…

Atomic Physics · Physics 2020-10-28 J. C. Shaw , D. J. McCarron

As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample.…

Atomic Physics · Physics 2024-10-29 Zixuan Zeng , Shuhua Deng , Shoukang Yang , Bo Yan

We demonstrate buffer-gas cooling, high-resolution spectroscopy and cycling fluorescence of cold barium monofluoride (BaF) molecules. Our source produces an intense and internally cold molecular beam containing the different BaF…

Atomic Physics · Physics 2020-01-13 Ralf Albrecht , Michael Scharwaechter , Tobias Sixt , Lucas Hofer , Tim Langen

We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…

Chemical Physics · Physics 2018-12-04 X. Wu , T. Gantner , M. Zeppenfeld , S. Chervenkov , G. Rempe

Experiments with cold molecules usually begin with a molecular source. We describe the construction and characteristics of a cryogenic buffer gas source of CaF molecules. The source emits pulses with a typical duration of 240 $\mu$s, a mean…

Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…

Atomic Physics · Physics 2012-10-02 Nicholas R. Hutzler , Hsin-I Lu , John M. Doyle

We use narrow-band laser excitation of Yb to substantially enhance the brightness of a cold beam of YbOH, a polyatomic molecule with high sensitivity to physics beyond the Standard Model (BSM). By exciting atomic Yb to the metastable…

We describe the combination of buffer-gas cooling with electrostatic velocity filtering to produce a high-flux continuous guided beam of internally cold and slow polar molecules. In a previous paper (L.D. van Buuren et al.,…

A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…

The design and performance of a cryogenic buffer gas beam (CBGB) source with a load-lock system is presented. The ACME III electron electric dipole moment (eEDM) search experiment uses this source to produce a beam of cold, slow thorium…

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