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Optical pump-probe spectroscopy is a powerful tool to directly probe the carrier dynamics in materials down to sub-femtosecond resolution. To perform such measurement, while keeping the pump induced perturbation to the sample as small as…

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…

Spectroscopy sampling along delay time is typically performed with uniform delay spacing, which has to be low enough to satisfy the Nyquist-Shannon sampling theorem. The sampling theorem puts the lower bound for the sampling rate to ensure…

Chemical Physics · Physics 2025-03-04 Junyan Sun , Deran Zhang , Ziqian Cheng , Dazhi Xu , Hui Dong

We demonstrate a new technique for saturated-absorption spectroscopy using co-propagating beams that does not have the problem of crossover resonances. The pump beam is locked to a transition and its absorption signal is monitored while the…

Atomic Physics · Physics 2009-11-10 Ayan Banerjee , Vasant Natarajan

The ability to resolve and quantify features at submicrometer scales from a single-shot image is crucial for real-time uncovering intricate structures in unlabeled biological samples and analyzing them at the subcellular level. We introduce…

Optics · Physics 2025-01-22 Jaromír Běhal , Miroslav Ježek

We propose the new method of essential decrease of transit-time broadening of Doppler-free absorption resonances on transitions between long-lived quantum levels of atoms (or molecules) of a rarefied gas medium. This method is based on…

Atomic Physics · Physics 2018-02-06 Azad Ch. Izmailov

Mid-infrared photothermal (MIP) microscopy has been a promising label-free chemical imaging technique for functional characterization of specimens owing to its enhanced spatial resolution and high specificity. Recently developed wide-field…

A major limitation of transient optical spectroscopy is that relatively high laser fluences are required to enable broadband, multichannel detection with acceptable signal-to-noise levels. Under typical experimental conditions, many…

Optics · Physics 2023-05-03 Siedah J. Hall , Peter J. Budden , Anne Zats , Matthew Y. Sfeir

Precise measurements in optical and atomic systems often rely on differential interferometry. This method allows to handle large and correlated phase noise contributions -- such as environmental vibrations, thermal fluctuations, or…

Quantum Physics · Physics 2025-03-25 Luca Pezzè , Andrea Santoni , Chiara Mazzinghi , Marco Fattori , Augusto Smerzi

Interferometric imaging is a well established method to image phase objects by mixing the image wavefront with a reference one on a CCD camera. It has also been applied to fast transient phenomena, mostly through the analysis of single…

Time-resolved measurements of quantum dynamics are based on the availability of controlled events (e.g. pump and probe pulses) that are shorter in duration than the typical evolution time scale of the dynamical processes to be observed.…

Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however,…

Optics · Physics 2019-05-01 Ondřej Denk , Kaibo Zheng , Donatas Zigmantas , Karel Žídek

The precise optical, label-free, measurement of mass at the nanoscale has been significantly advanced by techniques based on interferometric scattering, such as mass photometry (MP). These methods exploit the interference between a…

Optics · Physics 2025-01-14 Jan Becker

Quantitative phase microscopy (QPM) enables label-free measurement of local optical path length variations, providing critical insight into the structure and dynamics of transparent biological specimens. Here, a highly sensitive lateral…

Interferometric scattering microscopy has been a very promising technology for highly sensitive label-free imaging of a broad spectrum of biological nanoparticles from proteins to viruses in a high-throughput manner. Although it can reveal…

Optics · Physics 2021-08-11 Celalettin Yurdakul , Haonan Zong , Yeran Bai , Ji-Xin Cheng , M. Selim Unlu

Presented is a novel way to combine snapshot compressive imaging and lateral shearing interferometry in order to capture the spatio-spectral phase of an ultrashort laser pulse in a single shot. A deep unrolling algorithm is utilised for the…

We demonstrate that a reduction in the noise-to-signal ratio may be obtained for hadrons at non-zero momenta whilst maintaining a good overlap with the ground state through a generalisation of Gaussian/Wuppertal smearing. The use of an…

High Energy Physics - Lattice · Physics 2012-11-07 Michele Della Morte , Benjamin Jäger , Thomas D. Rae , Hartmut Wittig

Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…

Optics · Physics 2021-04-07 Jun Jiang , David Grass , Yue Zhou , Warren S. Warren , Martin C. Fischer

We demonstrate a femtosecond pump-probe spectrometer which utilizes a white light supercontinuum as input, and relies on mutual synchronization of acousto-optical chopper, pump-probe delay stage and the CCD camera to record shot-to-shot…

Chemical Physics · Physics 2022-12-27 Vivek N. Bhat , Asha S. Thomas , Vivek Tiwari

We have shown earlier that hyperfine spectroscopy in a vapor cell using co-propagating pump-probe beams has many advantages over the usual technique of saturated-absorption spectroscopy using counter-propagating beams. The main advantages…

Atomic Physics · Physics 2010-09-01 Alok K. Singh , Sapam Ranjita Chanu , Dipankar Kaundilya , Vasant Natarajan
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