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Ruddelsden-Popper halide perovskites are highly versatile quasi-two-dimensional energy materials with a wide range of tunable optoelectronic properties. Here we use the all-inorganic Cs$_{n+1}$Pb$_n$X$_{3n+1}$ Ruddelsden-Popper perovskites…

Spin-orbit coupling (SOC) in conjunction with broken inversion symmetry acts as a key ingredient for several intriguing quantum phenomena viz. persistent spin textures, topological surface states and Rashba-Dresselhaus (RD) effects. The…

Materials Science · Physics 2021-09-28 Preeti Bhumla , Deepika Gill , Sajjan Sheoran , Saswata Bhattacharya

The Rashba effect, i.e., the splitting of electronic spin-polarized bands in the momentum space of a crystal with broken inversion symmetry, has enabled the realization of spin-orbitronic devices, in which spins are manipulated by…

Polar metals are an intriguing class of materials in which electric polarisation and metallicity can coexist within a single phase. The unique properties of polar metals challenge expectations, making way for the exploration of exotic…

Strongly Correlated Electrons · Physics 2025-02-03 Evie Ladbrook , Urmimala Dey , Nicholas C. Bristowe , Robin S. Perry , Dominik Daisenberger , Mark R. Warren , Mark S. Senn

The strong spin-orbit interaction in the organic-inorganic perovskites tied to the incorporation of heavy elements (\textit{e.g.} Pb, I) makes these materials interesting for applications in spintronics. Due to a lack of inversion symmetry…

Interaction between electrons and phonons in solids is a key effect defining physical properties of materials such as electrical and thermal conductivity. In transitional metal dichalcogenides (TMDCs) the electron-phonon coupling results in…

Dimensionality engineering in A$_{n+1}$B$_n$X$_{3n+1}$ Ruddlesden-Popper (RP) perovskite phases has emerged as a promising strategy to enhance optoelectronic properties. These properties are highly material-dependent, requiring detailed…

Materials Science · Physics 2025-03-04 Surajit Adhikari , Aksaj Bharatwaj , Priya Johari

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

Materials Science · Physics 2024-05-07 Maximilian Black , Mehdi Asadi , Parsa Darman , Finja Schillmöller , Sara Darbari , Nahid Talebi

In recent years, metal halide perovskites have generated tremendous interest for optoelectronic applications and their underlying fundamental properties. Due to the large electron-phonon coupling characteristic of soft lattices,…

Associated with spin-orbit coupling (SOC) and inversion symmetry breaking, Rashba spin polarization opens a new avenue for spintronic applications that was previously limited to ordinary magnets. However, spin polarization effects in actual…

Computational Physics · Physics 2016-10-12 Qihang Liu , Xiuwen Zhang , J. A. Waugh , D. S. Dessau , Alex Zunger

Metal-halide perovskites (MHPs) emerged as a family of novel semiconductors with outstanding optoelectronic properties for applications in photovoltaics and light emission. Recently, they also attract interest as promising candidates for…

The Rashba effect is one of the most striking manifestations of spin-orbit coupling in solids, and provides a cornerstone for the burgeoning field of semiconductor spintronics. It is typically assumed to manifest as a momentum-dependent…

We investigate the two-dimensional (2D) highly spin-polarized electron accumulation layers commonly appearing near the surface of n-type polar semiconductors BiTeX (X = I, Br, and Cl) by angular-resolved photoemission spectroscopy. Due to…

Inorganic-organic lead halide perovskites, particularly methylammonium lead halide (MAPbI$_3$) perovskite, is perceived to be a promising material for optoelectronics and spintronics. However, lead toxicity and instability under air and…

Materials Science · Physics 2022-12-07 Megha Arya , Preeti Bhumla , Sajjan Sheoran , Suraj , S Bhattacharya

Quasi two-dimensional (2D) colloidal synthesis made quantum confinement readily accessible in perovskites, generating additional momentum in perovskite LED research and lasing. Ultrathin perovskite layers exhibit high exciton binding…

Materials Science · Physics 2024-09-04 André Niebur , Eugen Klein , Rostyslav Lesyuk , Christian Klinke , Jannika Lauth

We study the effects of the Rashba spin-orbit coupling on the polaron formation, using a suitable generalization of the Momentum Average approximation. Contrary to previous investigations of this problem, we find that the spin-orbit…

Strongly Correlated Electrons · Physics 2015-05-13 Lucian Covaci , Mona Berciu

Materials combining the optoelectronic functionalities of semiconductors with control of the spin degree of freedom are highly sought after for the advancement of quantum technology devices. Here, we report the paramagnetic…

Strong spin-orbit coupling in noncentrosymmetric materials and interfaces results in remarkable physical phenomena, such as nontrivial spin textures, which may exhibit Rashba, Dresselhaus, and other intricated configurations. This provides…

Mesoscale and Nanoscale Physics · Physics 2021-11-15 Thorsten Aull , Igor V. Maznichenko , Sergey Ostanin , Ersoy Şaşıoğlu , Ingrid Mertig

Two-dimensional (2D) hybrid organic-inorganic perovskites (HOIPs) are introducing new directions in the 2D materials landscape. The coexistence of ferroelectricity and spin-orbit interactions play a key role in their optoelectronic…

Materials Science · Physics 2021-04-08 Fei Wang , Heng Gao , Coen de Graaf , Josep M. Poblet , Branton J. Campbell , Alessandro Stroppa

Light-matter coupling in excitonic materials has been the subject of intense investigation due to emergence of new excitonic materials. Two-dimensional layered hybrid organic/inorganic perovskites (2D HOIPs) support strongly bound excitons…

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