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The bulk photovoltaic effect (BPVE) generates a direct current photocurrent under uniform irradiation and is a nonlinear optical effect traditionally studied in non-centrosymmetric materials. The two main origins of BPVE are the shift and…

Mesoscale and Nanoscale Physics · Physics 2025-03-03 Ying-Ming Xie , Naoto Nagaosa

The bulk photovoltaic effect (BPVE) -- generation of electric currents by light in noncentrosymmetric materials in the absence of electric fields and gradients -- has been intensively investigated in the end of the last century. The…

Mesoscale and Nanoscale Physics · Physics 2019-11-28 Boris Sturman

We calculate the bulk photovoltaic response of the ferroelectrics BaTiO$_3$ and PbTiO$_3$ from first principles by applying "shift current" theory to the electronic structure from density functional theory. The first principles results for…

Materials Science · Physics 2015-06-04 Steve M. Young , Andrew M. Rappe

Designing materials with controlled photovoltaic response may lead to improved solar cells or photosensors. In this regard, ferroelectric superlattices have emerged as a rich platform to engineer functional properties. In addition,…

Materials Science · Physics 2025-02-20 Francesco Delodovici , Charles Paillard

The bulk photovoltaic effect (BPVE) is a second-order optical process in noncentrosymmetric materials that converts the light into DC currents. BPVE is classified into shift current and injection current according to the generation…

Materials Science · Physics 2023-02-21 Hanqi Pi , Shuai Zhang , Hongming Weng

The bulk photovoltaic effect (BPVE) converts light into a coherent dc current at zero bias, through what is commonly known as the shift current. This current has previously been attributed to the displacement of the electronic wave function…

Mesoscale and Nanoscale Physics · Physics 2022-03-24 Daniel Kaplan , Tobias Holder , Binghai Yan

DC photoelectrical currents can be generated purely as a non-linear effect in uniform media lacking inversion symmetry without the need for a material junction or bias voltages to drive it, in what is termed photogalvanic effect. These…

Mesoscale and Nanoscale Physics · Physics 2016-08-17 F. Hipolito , Thomas G. Pedersen , Vitor M. Pereira

The bulk photovoltaic effect in noncentrosymmetric materials is an intriguing physical phenomenon that holds potential for high-efficiency energy harvesting. Here, we study the shift current bulk photovoltaic effect in the transition metal…

Materials Science · Physics 2021-01-28 Aaron M. Schankler , Lingyuan Gao , Andrew M. Rappe

Bulk photovoltaic (BPV) effect, a second order nonlinear process that generates static current under light irradiation, requires centrosymmetric broken systems as its application platform. In order to realize measurable BPV photocurrent in…

Materials Science · Physics 2023-01-05 Xingchi Mu , Qianqian Xue , Yan Sun , Jian Zhou

Pyroelectric and photovoltaic effects are vital in cutting-edge thermal imaging, infrared sensors, thermal and solar energy harvesting. Recent advances revealed the great potential of the bulk photovoltaic effect in two-dimensional (2D)…

Applied Physics · Physics 2024-01-01 Michael Uzhansky , Abhishek Rakshit , Yoav Kalcheim , Elad Koren

The bulk photovoltaic effect (BPVE) refers to the direct current generation in a noncentrosymmetric material under illumination and can be applied to solar energy technology. BPVE includes injection and shift currents, led by the change of…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Bo-Xin Lin , Hsiu-Chuan Hsu

Hybrid halide perovskites exhibit nearly 20% power conversion efficiency, but the origin of their high efficiency is still unknown. Here, we compute the shift current, a dominant mechanism of bulk photovoltaic (PV) effect for ferroelectric…

Materials Science · Physics 2014-10-14 Fan Zheng , Hiroyuki Takenaka , Fenggong Wang , Nathan Z. Koocher , Andrew M. Rappe

We employ first-principles calculations to investigate the ferroelectric properties and the bulk photovoltaic effect (BPVE) of antimony sulfur iodide (SbSI). The BPVE enables direct sunlight-to-electricity conversion in homogeneous…

Materials Science · Physics 2025-06-13 Giuseppe Cuono , Subhadeep Bandyopadhyay , Andrea Droghetti , Silvia Picozzi

The bulk photovoltaic effect (BPVE), arising from broken inversion symmetry in ferroelectrics, offers a distinct pathway toward high-efficiency next-generation photovoltaics. We propose and investigate A/A$^\prime$-ordered double…

Materials Science · Physics 2025-11-11 Sathiyamoorthy Buvaneswaran , Trilochan Sahoo , Saurabh Ghosh

Giant photovoltaic effect due to bulk photovoltaic effect observed in multiferroic BiFeO3 thin films has triggered a renewed interest on photoferroelectric materials for photovoltaic applications. Tremendous advance has been done to improve…

Materials Science · Physics 2022-10-03 I. Fina , C. Paillard , B. Dkhil

Ferroelectrics are polar materials whose polarization can be switched by applying electric fields; they offer unique opportunities to develop performant photostrictive materials, i.e., materials that can deform under visible light…

Noncentrosymmetric bulk crystals generate photocurrent without any bias voltage. One of the dominant mechanisms, shift current, comes from a quantum interference of electron wave functions being distinct from classical current caused by…

Materials Science · Physics 2018-12-17 M. Nakamura , H. Hatada , Y. Kaneko , N. Ogawa , Y. Tokura , M. Kawasaki

The bulk photovoltaic effect exhibited by the non-centrosymmetric system gains research interest due to the observed large open-circuit voltage. The ferroelectric systems exhibiting anomalous photovoltaic effect are mostly crystallized with…

Materials Science · Physics 2021-04-08 Subhajit Pal , S. Muthukrishnan , Banasree Sadhukhan , Sarath N. , D. Murali , Pattukkannu Murugavel

The bulk photovoltaic effect that is intimately associated with crystalline symmetry has been extensively studied in various nonmagnetic materials, especially ferroelectrics with a switchable electric polarization. In order to further…

Materials Science · Physics 2022-12-28 Chunmei Zhang , Ping Guo , Jian Zhou

In future solar cell technologies, the thermodynamic Shockley-Queisser limit for solar-to-current conversion in traditional p-n junctions could potentially be overcome with a bulk photovoltaic effect by creating an inversion broken symmetry…