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The monolithic tandem integration of third-generation solar energy materials on silicon holds great promise for photoelectrochemistry and photovoltaics. However, this can be challenging when it involves high-temperature reactive processes,…

Black phosphorus is a layered semiconductor that is intensely researched in view of applications in optoelectronics. In this Letter, we investigate a multi-layer black phosphorus photo-detector that is capable of acquiring high-contrast…

Materials Science · Physics 2016-01-12 Michael Engel , Mathias Steiner , Phaedon Avouris

We present a theoretical study on the impact of an active optical layer on the emission properties of an ultrathin luminescent film. While the study can be generalized to any material, we focus here on a simple layered medium composed of a…

Materials Science · Physics 2015-06-16 R. Aad , S. Blaize , A. Bruyant , C. Couteau , G. Lérondel

Transfer of energy and information through molecule aggregates requires as one important building block anisotropic, cable-like structures. Knowledge on the spatial correlation of luminescence and morphology represents a prerequisite in the…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 M. Bahrami , S. Kraft , J. Becker , H. Hartmann , B. Vogler , K. Wardelmann , H. Behle , J. A. A. W. Elemans , I. Barke , S. Speller

Recently, we have suggested dielectric metamaterial composed as an array of submicron dielectric spheres located on top of an amorphous thin-film solar cell. We have theoretically shown that this metamaterial can decrease the reflection and…

The templated growth of the basic porphyrin unit, free-base porphine (2H-P), is characterized by means of X-ray photoelectron spectroscopy (XPS) and near-edge X-ray absorption fine-structure (NEXAFS) spectroscopy measurements and density…

The large - scale commercialization of promising lithium - sulfur (Li - S) batteries remains limited by the polysulfide shuttle effect, which causes rapid capacity fading and poor cycle life. In this study, we present a scalable strategy to…

The recent renaissance of black phosphorus (BP) as a two-dimensional 2D layered material has generated tremendous interest in its tunable electronic band gap and highly anisotropic transport properties that offer new opportunities for…

Mesoscale and Nanoscale Physics · Physics 2016-03-08 Shan Dong , Anmin Zhang , Kai Liu , Jianting Ji , Y. G. Ye , X. G. Luo , X. H. Chen , Xiaoli Ma , Yinghao Jie , Changfeng Chen , Xiaoqun Wang , Qingming Zhang

Thin layers of black phosphorus have recently raised interest for their two-dimensional (2D) semiconducting properties, such as tunable direct bandgap and high carrier mobilities. This lamellar crystal of P atoms stacked together by weak…

Mesoscale and Nanoscale Physics · Physics 2014-08-22 A. Favron , E. Gaufrès , F. Fossard , P. L. Lévesque , A-L. Phaneuf-L'Heureux , N. Y-W. Tang , A. Loiseau , R. Leonelli , S. Francoeur , R. Martel

Using interlayer interaction to control functional heterostructures with atomic-scale designs has become one of the most effective interface-engineering strategies nowadays. Here, we demonstrate the effect of a crystalline LaFeO3 buffer…

The organic spinterface describes the spin-polarized properties that develop, due to charge transfer, at the interface between a ferromagnetic metal (FM) and the molecules of an organic semiconductor. Yet, if the latter is also magnetic…

The strength of light-matter interaction is of central importance in photonics and optoelectronics. For many widely studied two-dimensional semiconductors, such as MoS2, the optical absorption due to exciton resonances increases with…

Mesoscale and Nanoscale Physics · Physics 2020-04-16 Guowei Zhang , Shenyang Huang , Fanjie Wang , Qiaoxia Xing , Chaoyu Song , Chong Wang , Yuchen Lei , Mingyuan Huang , Hugen Yan

Sulfide chalcopyrite, Cu(In,Ga)S2, having wide bandgap (larger than 1.5 eV), favorable optoelectronic properties, and high stability, is a promising top-cell absorber for tandem applications. Adapting device structures optimized for 1.0 -…

The control of exciton transport in organic materials is of fundamental importance for the development of efficient light-harvesting systems. This transport is easily deteriorated by traps in the disordered energy landscape. Here, we…

Materials Science · Physics 2015-12-09 Joel Yuen-Zhou , Semion S. Saikin , Norman Y. Yao , Alán Aspuru-Guzik

Recent ab initio calculations and experiments reported insulating-semimetallic phase transitions in multilayer phosphorene under a perpendicular dc field, pressure or doping, as a possible route to realize topological phases. In this work,…

Mesoscale and Nanoscale Physics · Physics 2017-01-20 C. Dutreix , E. A. Stepanov , M. I. Katsnelson

Negative compressibility generated by many-body effects in 2D electronic systems can enhance gate capacitance. We observe capacitance enhancement in a newly emerged 2D layered material, atomically thin black phosphorus (BP). The…

Mesoscale and Nanoscale Physics · Physics 2016-04-05 Yingying Wu , Xiaolong Chen , Zefei Wu , Shuigang Xu , Tianyi Han , Jiangxiazi Lin , Yuan Cai , Yuheng He , Chun Cheng , Ning Wang

Black phosphorus thin films might offer attractive alternatives to narrow gap compound semiconductors for optoelectronics across mid- to near-infrared frequencies. In this work, we calculate the optical conductivity tensor of multilayer…

Materials Science · Physics 2014-09-18 Tony Low , A. S. Rodin , A. Carvalho , Yongjin Jiang , Han Wang , Fengnian Xia , A. H. Castro Neto

We investigate the possibility of band structure engineering in the recently predicted 2D layered form of blue phosphorus via an electric field (E$_z$) applied perpendicular to the layer(s). Using density functional theory, we study the…

Mesoscale and Nanoscale Physics · Physics 2015-03-26 Barun Ghosh , Suhas Nahas , Somnath Bhowmick , Amit Agarwal

Black phosphorus exhibits a layered structure similar to graphene, allowing mechanical exfoliation of ultrathin single crystals. Here we demonstrate few-layer black phosphorus field effect devices on Si/SiO$_2$ and measure charge carrier…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Steven P. Koenig , Rostislav A. Doganov , Hennrik Schmidt , A. H. Castro Neto , Barbaros Oezyilmaz

As a new two-dimensional layered material, black phosphorus (BP) is a promising material for nanoelectronics and nano-optoelectronics. We use Raman spectroscopy and first-principles theory to report our findings related to low-frequency…

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