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It is developed a microscopic description of superconductivity in ferromagnetic materials with triplet pairing triggered by the exchange of magnetic fluctuations. Instead widely used paramagnon model we work with phenomenological spectrum…

Superconductivity · Physics 2015-05-20 V. P. Mineev

Molecular spin systems based on photoexcited triplet pairs formed via singlet fission (SF) are attractive as carriers of quantum information because of their potentially pure and controllable spin polarization, but developing systems that…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Gajadhar Joshi , Ryan D. Dill , Karl J. Thorley , John E. Anthony , Obadiah G. Reid , Justin C. Johnson

We present a theory of polarized photoluminescence of triplet excitons in semiconductor nanocrystal ensembles with the random fine structure contributed by the electron-hole exchange and carrier-nuclear hyperfine interactions. The…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 D. S. Smirnov , E. L. Ivchenko

We investigate the physical mechanisms for spin-dependent recombination of a strongly bound pair of triplet excitons generated by singlet fission and forming a spin quintet (total spin of two) bi-exciton. For triplet excitons the…

Mesoscale and Nanoscale Physics · Physics 2024-02-16 Yan Sun , L. R. Weiss , V. Derkach , J. E. Anthony , M. Monteverde , A. D. Chepelianskii

We perform charge-induced absorption and electroluminescence spectroscopy in a polyfluorene organic magnetoresistive device. Our experiments allow us to measure the singlet exciton, triplet exciton and polaron densities in a live device…

Soft Condensed Matter · Physics 2009-11-13 T. D. Nguyen , J. Rybicki , Y. Sheng , M. Wohlgenannt

The effect of a magnetic field on the electroluminescence of organic light emitting devices originates from the hyperfine interaction between the electron/hole polarons and the hydrogen nuclei of the host molecules. In this paper, we…

Decoherence effects for entangled triplet pairs in organic molecular crystals are analyzed for the case when excitons can hop between inequivalent lattice sites. The fluorescence quantum beats caused by quantum interference upon…

Quantum Physics · Physics 2025-12-09 Gerald Curran , Luke J. Weaver , Zachary Rex , Ivan Biaggio

The magnetoelectroluminescence of conjugated organic polymer films is widely accepted to arise from a polaron pair mechanism, but their magnetoconductance is less well understood. Here we derive a new relationship between the experimentally…

Chemical Physics · Physics 2016-06-13 Joseph E. Lawrence , Alan M. Lewis , David E. Manolopoulos , P. J. Hore

The geminate annihilation of two triplet excitons created by singlet exciton fission is affected by the dimensionality of transport as determined by typically anisotropic triplet exciton mobilities in organic molecular crystals. We analyze…

Materials Science · Physics 2024-05-16 Eric A. Wolf , Ivan Biaggio

Organic solar cells (OSCs) have recently shown a rapid improvement in their performance, bringing power conversion efficiencies (PCEs) closer to the point where commercial applications of the technology become viable. However, the low…

Resonance fluorescence from atomic systems consists of a single spectral peak that evolves into a Mollow triplet for a strong excitation field. Photons from different peaks of the triplet show distinct photon correlation that make the…

Quantum Physics · Physics 2022-12-29 Boon Long Ng , Chang Hoong Chow , Christian Kurtsiefer

The dependence of the spin reorientation transition in ultra-thin ferromagnetic films on external magnetic fields is studied. For different orientations of the applied field with respect to the film, phase diagrams are calculated within a…

Statistical Mechanics · Physics 2017-02-08 A. Hucht , K. D. Usadel

In a recent Letter Lee et al. studied the spin 1/2 photoluminescence-detected magnetic resonance (PLDMR) of a soluble derivative of poly-phenylene vinylene [MEH-PPV] and argued that it originates from the interaction of triplet excitons…

Other Condensed Matter · Physics 2009-11-11 C. G. Yang , E. Eherenfreund , Z. V. Vardeny

A general symmetry analysis of the optical conductivity or scattering tensor is used to rewrite the conductivity tensor as a sum of fundamental spectra multiplied by simple functions depending on the local magnetization direction. Using…

Strongly Correlated Electrons · Physics 2010-09-17 M. W. Haverkort , N. Hollmann , I. P. Krug , A. Tanaka

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum…

Materials Science · Physics 2015-05-14 B. F. Ding , Y. Yao , X. Y. Sun , Z. Y. Sun , X. D. Gao , Z. T. Xie , Z. J. Wang , X. M. Ding , Y. Z. Wu , X. F. Jin , C. Q. Wu , X. Y. Hou

We conduct polarization-dependent ultrafast spectroscopy to study the dynamics of singlet fission in tetracene single crystals. The spectrotemporal species for singlet and triplet excitons in transient absorption spectra are found to be…

Materials Science · Physics 2015-06-23 Bo Zhang , Chunfeng Zhang , Yanqing Xu , Rui Wang , Bin He , Yunlong Liu , Shimeng Zhang , Xiaoyong Wang , Min Xiao

To understand the photophysics of molecular aggregates, exciton model of J- and H-aggregate has been extensively utilized. However, it lacks consideration of crystal symmetry. Although discrete molecules may lack symmetry, their aggregates…

Mesoscale and Nanoscale Physics · Physics 2023-10-10 Qingyun Wan , Chi-Ming Che

We report first-principles GW-Bethe Salpeter Equation and Quantum Monte Carlo calculations of the optical and electronic properties of molecular and crystalline rubrene (C$_{42}$H$_{28}$). Many-body effects dominate the optical spectrum and…

Materials Science · Physics 2008-04-30 Na Sai , Murilo L. Tiago , James R. Chelikowsky , Fernando A. Reboredo

Misoriented bilayer graphene with commensurate angles shows unique magneto-optical properties. The optical absorption spectra of such a system strongly depend on the angle of rotation. For a general commensurate twist angle the absorption…

Mesoscale and Nanoscale Physics · Physics 2011-03-01 Vadim M. Apalkov , Tapash Chakraborty

The generalized tight-binding model with exact diagonalization method is developed to calculate the optical properties of monolayer graphene in the presence of composite magnetic fields. The ratio of the uniform magnetic field and the…

Mesoscale and Nanoscale Physics · Physics 2014-04-10 Y. C. Ou , Y. H. Chiu , P. H. Yang , M. F. Lin
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