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Related papers: Modeling high-order harmonic generation in quantum…

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An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

High-harmonic generation (HHG) is one of the fundamental processes at the heart of attosecond physics. Traditionally viewed as an effective single-particle effect, recent advances have focused on contributions beyond this single-particle…

We present a study of non-sequential double recombination (NSDR) high harmonic generation (HHG) in a molecular-like system. Using a Coulomb-corrected three-step model we are able to classically describe the observed NSDR HHG cutoffs…

Atomic Physics · Physics 2017-07-12 Kenneth K. Hansen , Lars Bojer Madsen

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

Optics · Physics 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

High harmonic generation (HHG) in solids reflects the underlying nonperturbative nonlinear dynamics of electrons in a strong light field and is a powerful tool for ultrafast spectroscopy of electronic structures. Photo-carrier doping allows…

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…

We present a method which computes many-electron energies and eigenfunctions by a full configuration interaction which uses a basis of atomistic tight-binding wave functions. This approach captures electron correlation as well as atomistic…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Erik Nielsen , Rajib Rahman , Richard P. Muller

We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous…

We make a systematic study of high-order harmonic generation (HHG) in a He$^+$-like model ion when the initial states are prepared as a coherent superposition of the ground state and an excited state. It is found that, according to the…

Atomic Physics · Physics 2009-11-11 Bingbing Wang , Taiwang Cheng , Xiaofeng Li , Panming Fu , Shigang Chen , Jie Liu

We propose a fully analytical method for describing high-order harmonic generation (HHG). This method is based on the strong-field approximation (SFA) and electron-trajectory theory, but utilizes the perturbation expansion on the Keldysh…

In this paper, we investigate the effects of full electronic correlation on the high harmonic generation in the helium atom subjected to laser pulses of extremely high intensity. To do this, we perform real-time propagations of the helium…

Chemical Physics · Physics 2022-05-18 Aleksander P. Woźniak , Michał Przybytek , Maciej Lewenstein , Robert Moszyński

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian

High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…

Particle transport and localization phenomena in condensed-matter systems can be modeled using a tight-binding lattice Hamiltonian. The ideal experimental emulation of such a model utilizes simultaneous, high-fidelity control and readout of…

We theoretically study high-harmonic generation (HHG) from transition metal elements Mn and Mn$^+$, using full-dimensional, all-electron, first-principles simulations. The HHG spectra calculated with the time-dependent complete-active-space…

Atomic Physics · Physics 2019-06-26 Imam S. Wahyutama , Takeshi Sato , Kenichi L. Ishikawa

Solid-state high-order harmonic generation (HHG) presents unique features different from gases.Whereas the gaseous harmonics driven by counter-rotating bicircular (CRB) pulse universally peak at a "magic" field ratio approximately…

Optics · Physics 2025-07-15 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Zhi Wang , Lin-Wang Wang , Jun-Wei Luo

We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide.…

Higher harmonic generation in plane graphene quantum dots initiated by intense coherent radiation is investigated, using dynamical Hartree-Fock mean-field theory. A microscopic theory describing the extreme nonlinear optical response of…

Mesoscale and Nanoscale Physics · Physics 2022-05-11 B. R. Avchyan , A. G. Ghazaryan , K. A. Sargsyan , Kh. V. Sedrakian

Using the Hubbard model we study how the process of high-order harmonic generation (HHG) is modified by beyond mean-field electron-electron correlation for both finite and bulk systems. A finite-size enhancement of the HHG signal is found…

Atomic Physics · Physics 2022-06-01 Thomas Hansen , Simon Vendelbo Bylling Jensen , Lars Bojer Madsen