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Large exciton diffusion lengths generally improve the performance of organic semiconductor devices, since they enable energy to be transported farther during the exciton lifetime. However, the physics of exciton motion in disordered organic…

Chemical Physics · Physics 2023-03-17 Daniel Balzer , Ivan Kassal

The coherent manipulation of excitons in bulk semiconductors via the lattice degrees of freedom is key to the development of acousto-optic and acousto-excitonic devices. Wide-bandgap transition metal oxides exhibit strongly bound excitons…

Tightly bound excitons in monolayer semiconductors represent a versatile platform to study two-dimensional propagation of neutral quasiparticles. Their intrinsic properties, however, can be severely obscured by spatial energy fluctuations…

Exciton many-body interaction bear great implication for application in advanced photonic devices and quantum science and technology such as quantum computing, but the fundamental understanding about exciton many-body interaction is very…

Materials Science · Physics 2020-09-17 Yiling Yu , Guoqing Li , Linyou Cao

Semiconductors in all dimensionalities ranging from 0D quantum dots and molecules to 3D bulk crystals support bound electron-hole pair quasiparticles termed as excitons. Over the past two decades, the emergence of a variety of…

Materials Science · Physics 2021-08-03 Surendra B. Anantharaman , Kiyoung Jo , Deep Jariwala

A theoretical study of the exciton binding energy in the two-dimensional hexagonal boron nitride monolayer is presented within the tight-binding approximation (TBA). A self-consistent equation for the interband electron-hole propagators is…

Materials Science · Physics 2018-03-28 Zoran Rukelj , Vito Despoja

The dynamics of exciton and electron-hole plasma populations is studied via time-resolved photoluminescence after nonresonant excitation. By comparing the peak emission at the exciton resonance with the emission of the continuum, it is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Hoyer , C. Ell , M. Kira , S. W. Koch , S. Chatterjee , S. Mosor , G. Khitrova , H. M. Gibbs , H. Stolz

Excitons drive the optoelectronic properties of organic semiconductors which underpin devices including solar cells and light-emitting diodes. Here we show that excitons can exhibit topologically non-trivial states protected by inversion…

Mesoscale and Nanoscale Physics · Physics 2025-05-21 Wojciech J. Jankowski , Joshua J. P. Thompson , Bartomeu Monserrat , Robert-Jan Slager

The localization length of a low energy tightly bound electron-hole pair (excitons) is calculated by exact diagonalization for small interacting disordered systems. The exciton localization length (which corresponds to the thermal…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Richard Berkovits

Calculations combining first-principles electron-phonon ($e$-ph) interactions with the Boltzmann equation enable studies of ultrafast carrier and phonon dynamics. However, in materials with weak Coulomb screening, electrons and holes form…

Materials Science · Physics 2022-10-13 Hsiao-Yi Chen , Marco Bernardi

We analyze the many-particle correlations that affect the optical properties of two-dimensional semiconductors. These correlations manifest themselves through the specific optical resonances such as excitons, trions, etc. Starting from the…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 A. Kudlis , I. Iorsh

Time-dependent density-functional theory (TDDFT) is a computationally efficient first-principles approach for calculating optical spectra in insulators and semiconductors, including excitonic effects. We show how exciton wave functions can…

Materials Science · Physics 2020-12-29 Jared R. Williams , Nicolas Tancogne-Dejean , Carsten A. Ullrich

Excitons play major roles in optical processes in modern semiconductors, such as single-wall carbon nanotubes (SWCNTs), transition metal dichalcogenides, and 2D perovskite quantum wells. They possess extremely large binding energies…

We analyze time-resolved spontaneous emission from excitons confined in self-assembled $\mathrm{InAs}$ quantum dots placed at various distances to a semiconductor-air interface. The modification of the local density of optical states due to…

Other Condensed Matter · Physics 2010-11-05 Søren Stobbe , Jeppe Johansen , Philip Trøst Kristensen , Jørn M. Hvam , Peter Lodahl

Time-resolved, angle-resolved photoemission spectroscopy (TR-ARPES) is a one-particle spectroscopic technique that can probe excitons (two-particle excitations) in momentum space. We present an ab initio, time-domain GW approach to TR-ARPES…

Materials Science · Physics 2023-02-06 Y. -H. Chan , Diana Y. Qiu , Felipe H. da Jornada , Steven G. Louie

Exciton-polaritons -- hybrid states of photons and excitons -- offer unique avenues for controlling electronic, optical, and chemical properties of materials. However, their modeling is mostly limited to formalisms that wash out atomistic…

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie

We investigate the dynamical formation of excitons from photoexcited electron-hole plasma and its subsequent decay dynamics in monolayer MoS2 grown by chemical vapor deposition using ultrafast pump and terahertz probe spectroscopy.…

Materials Science · Physics 2014-10-14 Xuefeng Liu , Qingqing Ji , Zhihan Gao , Shaofeng Ge , Jun Qiu , Zhongfan Liu , Yanfeng Zhang , Dong Sun

An overview on photon echo spectroscopy under resonant excitation of the exciton complexes in semiconductor nanostructures is presented. The use of four-wave-mixing technique with the pulsed excitation and heterodyne detection allowed us to…

Mesoscale and Nanoscale Physics · Physics 2018-08-29 S. V. Poltavtsev , I. A. Yugova , I. A. Akimov D. R. Yakovlev , M. Bayer

The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…

Materials Science · Physics 2020-10-09 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir