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Picosecond carrier dynamics in indium antimonide (InSb) following excitation by below-bandgap broadband far infrared radiation were investigated at 200 K and 80 K. Using a novel THz-pump/THz-probe scheme with pump THz fields of 100 kV/cm…

Materials Science · Physics 2009-06-17 Matthias C. Hoffmann , Janos Hebling , Harold Y. Hwang , Ka-Lo Yeh , Keith A. Nelson

Pumping n-type GaAs and InSb with ultrafast THz pulses having intensities higher than 150 MW/cm2 shows strong free carrier absorption saturation at temperatures of 300 K and 200 K respectively. If the energy imparted to the carriers exceeds…

Materials Science · Physics 2009-06-17 Matthias C. Hoffmann , Janos Hebling , Harold Y. Hwang , Ka-Lo Yeh , Keith A. Nelson

Optical pump-terahertz probe spectroscopy has been used to investigate ultrafast photo-induced charge carrier transport in 3.4 $\mu$m wide graphene ribbons upon scaling the optical pump intensity. For low pump fluences, the deposited pump…

Materials Science · Physics 2026-03-02 Arvind Singh , Hynek Němec , Jan Kunc , Petr Kužel

Using synchronized near-infrared (NIR) and terahertz (THz) lasers, we have performed picosecond time-resolved THz spectroscopy of transient carriers in semiconductors. Specifically, we measured the temporal evolution of THz transmission and…

Condensed Matter · Physics 2009-11-07 M. A. Zudov , A. P. Mitchell , A. H. Chin , J. Kono

Using two-dimensional THz spectroscopy in combination with numerical models, we investigate the dynamics linked to carrier multiplication caused by high-field THz excitation of the low-gap semiconductor InSb. In addition to previously…

Other Condensed Matter · Physics 2022-12-21 Simone Biasco , Florence Burri , Sarah Houver , Elsa Abreu , Matteo Savoini , Steven L. Johnson

Time-resolved multi-terahertz (THz) spectroscopy is used to observe pump fluence-dependent dynamics in the optical conductivity of photoexcited tin selenide (SnSe) over an ultrabroadband spectral range of 0.5 - 11 THz at fluences from 0.1 -…

In an ultrafast optical-pump terahertz-probe measurement, the photoinduced material response can be modulated on a timescale shorter than the extent of the THz pulse. In this situation, the measured time-frequency response deviates from a…

Optics · Physics 2025-12-19 Benjamin J. Dringoli , David G. Cooke

We study the nature of photo-excited charge carriers in CsPbBr3 nanocrystal thin films by ultrafast optical pump - THz probe spectroscopy. We observe a deviation from a pure Drude dispersion of the THz dielectric response that is ascribed…

We present femtosecond transient transmission (or absorbance) measurements in silicon nanowires in the energy range 1.1-3.5 eV, from below the indirect band-gap to above the direct band-gap. Our pump-probe measurements allow us to give a…

We report on time-resolved broadband transient reflectivity (tr-bb-TR) measurements performed on a bulk single crystal of T$_d$-MoTe$_2$ as a function of the incident pump fluence (F). Tr-bb-TR data unveil photoinduced electronic changes…

Time-resolved multi-terahertz (THz) spectroscopy is used to observe an ultrafast, non-thermal electronic phase change in SnSe driven by interband photoexcitation with 1.55 eV pump photons. The transient THz photoconductivity spectrum is…

Materials Science · Physics 2024-02-12 Benjamin J. Dringoli , Mark Sutton , Zhongzhen Luo , Mercouri G. Kanatzidis , David G. Cooke

Ultrafast light-matter interaction has emerged as a powerful tool to control and probe the macroscopic properties of functional materials, especially two-dimensional transition metal dichalcogenides which can form different structural…

Mesoscale and Nanoscale Physics · Physics 2023-10-10 XinYu Zhou , H Wang , Q M Liu , S J Zhang , S X Xu , Q Wu , R S Li , L Yue , T C Hu , J Y Yuan , S S Han , T Dong , D Wu , N L Wang

Understanding the ultrafast dynamics and transport of photoexcited carriers in topological insulators is crucial for the optical manipulation of spins and may shed light on the nature of topological excitons. Here we investigate…

Mesoscale and Nanoscale Physics · Physics 2025-02-07 Rodrigo Becerra Silva , Jay Huang , Bob Minyu Wang , Ziyi Song , Henry Clark Travaglini , Dong Yu

Here we perform a series of time-resolved experiments where a 100 fs pump pulse is tuned between 528 nm and 555 nm, across the second indirect gap of intrinsic silicon at ~540 nm which involves electrons in a higher-lying conduction band…

Optics · Physics 2017-01-24 Fabio Novelli , Jeffrey A Davis

A model is developed for photoinduced absorption from localized states observed in femtosecond pump-probe experiments in high-Tc superconductors and other materials. The dynamics of localized carriers are described in terms of…

Superconductivity · Physics 2015-06-24 V. V. Kabanov , J. Demsar , D. Mihailovic

We present a microscopic explanation of the controversially discussed transient negative differential transmission observed in degenerate optical pump-probe measurements in graphene. Our approach is based on the density matrix formalism…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Faris Kadi , Torben Winzer , Ermin Malic , Andreas Knorr

A type-II InAs/AlAs$_{0.16}$Sb$_{0.84}$ multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a…

We report on time-resolved optical and terahertz ultrafast spectroscopy of charge-carrier dynamics in the room-temperature antiferromagnetic semiconductor $\alpha $-MnTe. By optically pumping the system with 1.55 eV photons at room…

THz Time-Resolved Photoconductivity is used to probe carrier dynamics in the dilute III-V nitride GaP0.49As0.47N0.036. In these measurements a femtosecond optical pump-pulse excites electron-hole pairs, and a delayed THz pulse measures the…

Materials Science · Physics 2018-11-14 J. N. Heyman , E. M. Weiss , J. R. Rollag , K. M. Yu , O. D. Dubon , Y. J. Kuang , C. W. Tu , W. Walukiewicz

We present measurements of the transient photoconductivity in pentacene single crystals using optical-pump THz-probe spectroscopy. We have measured the temperature and fluence dependence of the mobility of the photoexcited charge carriers…

Condensed Matter · Physics 2016-01-26 V. K. Thorsmolle , R. D. Averitt , X. Chi , D. J. Hilton , D. L. Smith , A. P. Ramirez , A. J. Taylor
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