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We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

We present a multichannel photoelectron interferometry technique based on trichromatic pulse shaping for unambiguous determination of quantum phases in multiphoton ionization (MPI) of potassium atoms. The colors of the laser field are…

Atomic Physics · Physics 2022-05-25 K. Eickhoff , D. Köhnke , L. Feld , T. Bayer , M. Wollenhaupt

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…

Based upon standard angular momentum theory, we develop a framework to investigate polarization squeezing and multipartite entanglement of a quantum light field. Both mean polarization and variances of the Stokes parameters are obtained…

Quantum Physics · Physics 2016-04-27 G. R. Jin , S. Luo , Y. C. Liu , H. Jing , W. M. Liu

We consider the process of atomic ionization driven by a laser pulse with varying ellipticity. We study distribution of the momenta of the photoelectrons, ionized by a strong laser field, emitted in the direction perpendicular to the…

Atomic Physics · Physics 2015-06-22 I. A. Ivanov

We investigate the strong-field ionization of atomic hydrogen in a few-cycle elliptically polarized infrared pulse by solving the time-dependent Schr\"odinger equation. The dependence of the photoelectron momentum distribution on the pulse…

Atomic Physics · Physics 2022-11-30 Nicolas Douguet , Klaus Bartschat

Angle-resolved multiphoton ionization of fenchone and camphor by short intense laser pulses is computed by the time-dependent Single Center (TDSC) method. Thereby, the photoelectron circular dichroism (PECD) in the three-photon resonance…

Atomic and Molecular Clusters · Physics 2018-06-11 Anne D. Müller , Anton N. Artemyev , Philipp V. Demekhin

We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…

Atomic Physics · Physics 2018-04-03 Ruihua Xu , Zhaoyan Zhou , Xu Wang

Population of levels of the hyperfine and fine split ground state of an atom is affected by radiative transitions induced by anisotropic radiation flux. Such aligned atoms precess in the external magnetic field and this affects properties…

Astrophysics · Physics 2007-05-23 Huirong Yan , A. Lazarian

Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…

Atomic Physics · Physics 2021-02-03 Joss Wiese , Jolijn Onvlee , Sebastian Trippel , Jochen Küpper

Photoelectron circular dichroism (PECD) in different regimes of multiphoton ionization of fenchone is studied theoretically using the time-dependent single center method. In particular, we investigate the chiral response to the one-color…

Atomic and Molecular Clusters · Physics 2020-01-24 Anne D. Müller , Eric Kutscher , Anton N. Artemyev , Philipp V. Demekhin

We show experimentally and theoretically that vortex-shaped structures in the photoelectron momentum distribution can be observed for atoms interacting with a single intense elliptically polarized laser pulse. Our analysis reveals that…

Inelastic interaction of free-electrons with optical near fields has recently attracted attention for manipulating and shaping free-electron wavepackets. Understanding the nature and the dependence of the inelastic cross section on the…

Optics · Physics 2023-02-15 Fatemeh chahshouri , Nahid Talebi

The dynamics of the electron impact multiphoton ionization of a hydrogen atom in the presence of an intense laser field has been studied theoretically, with a view to comparing (qualitatively) the results with the recent kinematically…

Atomic Physics · Physics 2008-02-11 S. Ghosh Deb , S. Roy , C. Sinha

We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and…

Atomic Physics · Physics 2017-09-05 Vinay Pramod Majety , Armin Scrinzi

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant…

Atomic Physics · Physics 2018-10-03 J. Fedyk , A. B. Voitkiv , C. Müller

Generation of ultrarelativistic polarized positrons during interaction of an ultrarelativistic electron beam with a counterpropagating two-color petawatt laser pulse is investigated theoretically. Our Monte Carlo simulation based on a…

Interfacing electrons and light enables ultrafast electron microscopy, quantum control of electrons, as well as new optical elements for high sensitivity imaging. Here we demonstrate for the first time programmable transverse electron beam…

We demonstrate that the angular distribution of photoelectrons from a strongly polarizable target exposed to a laser field can deviate noticeably from the prediction of conventional theory. Even within the dipole-photon approximation the…

Atomic and Molecular Clusters · Physics 2009-11-13 A. V. Korol , A. V. Solov'yov
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