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Inelastic transport through a single magnetic molecule weakly coupled to metallic leads is studied theoretically. We consider dynamical processes that are relevant for writing, storing, and reading spin information in molecular memory…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Carsten Timm , Florian Elste

Dynamic nuclear polarization (DNP) is a promising strategy for generating a significantly increased non-thermal spin polarization in nuclear magnetic resonance (NMR) applications thereby circumventing the need for strong magnetic fields.…

Quantum Physics · Physics 2015-07-15 Alexander Karabanov , Daniel Wisniewski , Igor Lesanovsky , Walter Köckenberger

We describe how a local non-equilibrium nuclear polarisation can be generated and detected by electrical means in a semiconductor quantum point contact device. We show that measurements of the nuclear spin relaxation rate will provide clear…

Mesoscale and Nanoscale Physics · Physics 2008-06-26 N. R. Cooper , V. Tripathi

Searches for physics beyond the Standard Model using spin sensors are susceptible to spurious frequency shifts and noise due to magnetic fields. Therefore a comagnetometer -- an auxiliary sensor that allows mundane magnetic field effects to…

Atomic Physics · Physics 2025-09-15 Bassam Nima , Mingyu Fan , Aleksandar Radak , Andrew M. Jayich , Amar C. Vutha

Ultralight axion-like particles (ALPs) are well-motivated dark matter candidates introduced by theories beyond the standard model. However, the constraints on the existence of ALPs through existing laboratory experiments are hindered by…

High Energy Physics - Phenomenology · Physics 2022-03-01 Min Jiang , Haowen Su , Antoine Garcon , Xinhua Peng , Dmitry Budker

Nuclear spins of dopant atoms in semiconductors are promising candidates as quantum bits, due to the long lifetime of their quantum states. Conventionally, coherent control of nuclear spins is done using ac magnetic fields. Using the…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 Péter Boross , Gábor Széchenyi , András Pályi

The synthesis of molecular magnets has undergone rapid progress in recent years. Each of the identical molecular units can contain as few as two and up to several dozens of paramagnetic ions (spins). Although these materials appear as…

Strongly Correlated Electrons · Physics 2009-11-11 J. Schnack

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

Electron spin resonance (ESR) is a useful tool to investigate properties of materials in magnetic fields where high spin polarization of target electron spins is required in order to obtain high sensitivity. However, the smaller magnetic…

Quantum Physics · Physics 2022-02-09 Shingo Kukita , Hideaki Ookane , Yuichiro Matsuzaki , Yasushi Kondo

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…

We attract attention to the fact that the ultimate (shot-noise-limited) polarimetric sensitivity can be enhanced by orders of magnitude leaving the photon flux incident onto the photodetector on the same low level. This opportunity is of…

Mesoscale and Nanoscale Physics · Physics 2014-03-14 P. Glasenapp , A. Greilich , I. I. Ryzhov , V. S. Zapasskii , D. R. Yakovlev , G. G. Kozlov , M. Bayer

Dipolar coupled homonuclear spins present challenging, yet useful systems for quantum information processing. In such systems, eigenbasis of the system Hamiltonian is the appropriate computational basis and coherent control can be achieved…

Quantum Physics · Physics 2009-11-13 T. S. Mahesh , Dieter Suter

Enrichment of nuclear spin isomers of molecules by infrared radiation resonant to molecular rovibrational transition is considered. Special attention is given to the enrichment by light-induced crossing of far separated ortho and para…

Chemical Physics · Physics 2007-05-23 Pavel Chapovsky

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

Due to their long coherence times, nuclear spins have gained considerable attention as physical qubits. Two-qubit gates between nuclear spins of distinct resonance frequencies can be mediated by electron spins, usually employing a sequence…

Quantum Physics · Physics 2021-01-26 Benedikt Tratzmiller , Jan F. Haase , Zhenyu Wang , Martin B. Plenio

Nuclear spin optical rotation (NSOR) is a recently developed technique for detection of nuclear magnetic resonance via rotation of light polarization, instead of the usual long-range magnetic fields. NSOR signals depend on hyperfine…

Chemical Physics · Physics 2012-02-21 Junhui Shi , Suvi Ikäläinen , Juha Vaara , Michael V. Romalis

We present a protocol for designing appropriately extended $\pi$ pulses that achieves tunable, thus selective, electron-nuclear spin interactions with low-driving radiation power. Our method is general since it can be applied to different…

Quantum Physics · Physics 2019-06-11 I. Arrazola , E. Solano , J. Casanova

We propose a new method for dynamic nuclear polarisation in a quasi one-dimensional quantum wire utilising the spin-orbit interaction, the hyperfine interaction, and a finite source-drain potential difference. In contrast with current…

Mesoscale and Nanoscale Physics · Physics 2008-03-05 V. Tripathi , A. C. H. Cheung , N. R. Cooper

The possibility of coherent radiation by molecular magnets is investigated. It is shown that to realize the coherent radiation, it is necessary to couple the considered sample to a resonant electric circuit. A theory for describing this…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 V. I. Yukalov , E. P. Yukalova

We propose the use of non-equally spaced decoupling pulses for high-resolution selective addressing of nuclear spins by a quantum sensor. The analytical model of the basic operating principle is supplemented by detailed numerical studies…

Quantum Physics · Physics 2015-10-13 J. Casanova , Z. -Y. Wang , J. F. Haase , M. B. Plenio