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The ultrafast formation of strongly bound excitons in two-dimensional semiconductors provide a rich platform for studying fundamental physics as well as developing novel optoelectronic technologies. While extensive research has explored the…

The monolayers of semiconducting transition metal dichalcogenides host strongly bound excitonic complexes and are an excellent platform for exploring many-body physics. Here we demonstrate a controlled kinetic manipulation of the…

Mesoscale and Nanoscale Physics · Physics 2022-04-05 Suman Chatterjee , Sarthak Das , Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

We develop a non-local dielectric response theory to describe the temperature dependence of exciton lifetime in metal-semiconductor heterostructures. Coupling between excitons and surface plasmons results in a strongly nonmonotonous…

Mesoscale and Nanoscale Physics · Physics 2015-05-07 M. V. Durnev , A. V. Kavokin , B. Gil

Moir\'e potentials in two-dimensional materials have been proven to be of fundamental importance to fully understand the electronic structure of van der Waals heterostructures, from superconductivity to correlated excitonic states. However,…

The advancement of quantum photonic technologies relies on the ability to precisely control the degrees of freedom of optically active states. Here, we realize real-time, room-temperature tunable strong plasmon-exciton coupling in 2D…

The optically dark states play an important role in the electronic and optical properties of monolayers (MLs) of semiconducting transition metal dichalcogenides. The effect of temperature on the in-plane-field activation of the neutral and…

TMDCs have attracted a lot of attention in recent years due to their unique indirect to direct band gap transition from bulk to monolayer thickness. Strong confinement in the out-of-plane direction enhances the Coulomb potential between the…

Since the seminal observation of room-temperature laser emission from ZnO thin films and nanowires, numerous attempts have been carried out for detailed understanding of the lasing mechanism in ZnO. In spite of the extensive efforts…

Materials Science · Physics 2017-10-04 Ryosuke Matsuzaki , Haruka Soma , Kanae Fukuoka , Takashi Uchino

Atomically thin semi-conductors are characterized by strongly bound excitons which govern the optical properties of the materials below and near the band edge. Efficient conversion of photons into electrical current requires, as a first…

Mesoscale and Nanoscale Physics · Physics 2016-02-15 Sten Haastrup , Simone Latini , Kirill Bolotin , Kristian Sommer Thygesen

Two-dimensional (2D) monolayer phosphorene, a 2D system with quasi-one-dimensional (quasi-1D) excitons, provides a unique 2D platform for investigating the dynamics of excitons in reduced dimensions and fundamental many-body interactions.…

Materials Science · Physics 2016-02-03 Renjing Xu , Jiong Yang , Ye Win Myint , Jiajie Pei , Han Yan , Fan Wang , Yuerui Lu

Two-dimensional materials give access to the ultimate physical limits of Photonics with appealing properties for ultracompact optical components such as waveguides and modulators. Specifically, in monolayer semiconductors, a strong…

Understanding the effects of atomic defects on the optical functionality of two-dimensional (2D) layered materials is critical to develop novel optical and optoelectronic applications of these ultimate materials. Herein, we correlate sulfur…

The dynamics of exciton formation in transition metal dichalcogenides is difficult to measure experimentally, since many momentum-indirect exciton states are not accessible to optical interband spectroscopy. Here, we combine a tuneable…

We study the excitonic recombination dynamics in an ensemble of (9,4) semiconducting single-wall carbon nanotubes by high sensitivity time-resolved photo-luminescence experiments. Measurements from cryogenic to room temperature allow us to…

Other Condensed Matter · Physics 2015-06-25 S. Berger , C. Voisin , G. Cassabois , C. Delalande , Philippe Roussignol , X. Marie

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

The fine structure of the exciton spectrum, containing optically allowed (bright) and forbidden (dark) exciton states, determines the radiation efficiency in nanostructures. We study time-resolved micro-photoluminescence in MoS$_2$…

In monolayer semiconductor transition metal dichalcogenides, the exciton-phonon interaction is expected to strongly affect the photocarrier dynamics. Here, we report on an unusual oscillatory enhancement of the neutral exciton…

We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing,…

Mesoscale and Nanoscale Physics · Physics 2016-06-14 Ahsan Nazir , Dara P. S. McCutcheon

Excitons, quasi particles composed of an electron and a hole, play an important role in optical responses in low-dimensional nanostructures. In this work, we have investigated exciton diffusion in a monolayer MoSe2 encapsulated between…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 T. Hotta , S. Higuchi , A. Ueda , K. Shinokita , Y. Miyauchi , K. Matsuda , K. Ueno , T. Taniguchi , K. Watanabe , R. Kitaura

We have studied the nature of excitons in the transition metal dichalcogenide alloy Mo0.6W0.4 S2, compared to pure MoS2 and WS2 grown by atomic layer deposition (ALD). For this, optical absorption/transmission spectroscopy and…

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