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At cryogenic temperatures, the photoluminescence spectrum of monolayer WSe2features a num-ber of lines related to the recombination of so-called localized excitons. The intensity of these lines strongly decreases with increasing…

Exciton resonances in monolayer transition-metal dichalcogenides (TMDs) provide exceptionally strong light-matter interaction at room temperature. Their spectral line shape is critical in the design of a myriad of optoelectronic devices,…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Jorik van de Groep , Qitong Li , Jung-Hwan Song , Pieter G. Kik , Mark L. Brongersma

The low crystal symmetry of rhenium disulphide (ReS2) leads to the emergence of dichroic optical and optoelectronic response, absent in other layered transition metal dichalcogenides, which could be exploited for device applications…

In recent years, much research has been undertaken to investigate the suitability of two-dimensional materials to act as single-photon sources with high optical and quantum optical quality. Amongst them, transition-metal dichalcogenides,…

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

Mesoscale and Nanoscale Physics · Physics 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

Engineering and probing excitonic properties at the nanoscale remains a central challenge in quantum photonics and optoelectronics. While exciton confinement via electrical control and strain engineering has been demonstrated in 2D…

Mesoscale and Nanoscale Physics · Physics 2025-09-03 Yueh-Chun Wu , Bogdan Dryzhakov , Huan Zhao , Ivan Vlassiouk , Kyle Kelley , Takashi Taniguchi , Kenji Watanabe , Jun Yan , Benjamin Lawrie

Transition metal dichalcogenide monolayers are promising candidates for exploring new electronic and optical phenomena and for realizing atomically thin optoelectronic devices. They host tightly bound electron-hole pairs (excitons) that can…

Monolayers of transition-metal dichalcogenides such as WSe2 have become increasingly attractive due to their potential in electrical and optical applications. Because the properties of these 2D systems are known to be affected by their…

Two-dimensional transition metal di-chalcogenide semiconductors provide unique possibilities to investigate strongly confined excitonic physics and a plasmonic platform integrable to such materials constitutes a hybrid system that can be of…

Mesoscale and Nanoscale Physics · Physics 2022-05-26 Bidisha Roy , Maex Blauth , Siddharth Dhomkar , Michael Kaniber , Vinod M. Menon , Jonathan. J. Finley

Engineering non-linear hybrid light-matter states in tailored optical lattices is a central research strategy for the simulation of complex Hamiltonians. Excitons in atomically thin crystals are an ideal active medium for such purposes,…

In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek

The broadening and polarization of excitonic luminescence in monolayer TMDs largely suffer from inhomogeneity and temperature - an unresolved problem to date. In this work, through few-layer-graphene encapsulation of monolayer WS$_2$, we…

Mesoscale and Nanoscale Physics · Physics 2023-09-04 Garima Gupta , Kausik Majumdar

Several monolayer transition metal dichalcogenides (TMDs) are direct band gap semiconductors and potentially efficient emitters in light emitting devices. Photons are emitted when strongly bound excitons decay radiatively, and accurate…

Excitons in atomically-thin semiconductors necessarily lie close to a surface, and therefore their properties are expected to be strongly influenced by the surrounding dielectric environment. However, systematic studies exploring this role…

Mesoscale and Nanoscale Physics · Physics 2016-12-06 Andreas V. Stier , Nathan P. Wilson , Genevieve Clark , Xiaodong Xu , Scott A. Crooker

Strong spatial confinement and highly reduced dielectric screening provide monolayer transition metal dichalcogenides (TMDCs) with strong many-body effects, thereby possessing optically forbidden excitonic states (i.e., dark excitons) at…

Strong light-matter interactions in layered transition metal dichalcogenides (TMDs) open up vivid possibilities for novel exciton-based devices. The optical properties of TMDs are dominated mostly by the tightly bound excitons and more…

Two-dimensional transition metal dichalcogenides (2D TMDCs) are promising candidates for ultra-thin active nanophotonic elements due to the strong tunable excitonic resonances that dominate their optical response. Here we demonstrate…

Optics · Physics 2023-04-26 Melissa Li , Claudio U. Hail , Souvik Biswas , Harry A. Atwater

Monolayer transition metal dichalcogenides (TMDs) support robust excitons in the visible to near-infrared spectral range. Their reduced dielectric screening results in large binding energies, and combined with a direct bandgap in monolayer…

We report Raman spectra measurements on a MoS2 monolayer supported on SiO2 as a function of temperature. Unlike in previous studies, the positions of the two main Raman modes, E2g1 and A1g exhibited nonlinear temperature dependence.…

Mesoscale and Nanoscale Physics · Physics 2014-06-13 Andrzej Taube , Jarosław Judek , Cezariusz Jastrzębski , Anna Duzynska , Krzysztof Świtkowski , Mariusz Zdrojek

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 Dinh Van Tuan , Hanan Dery