Related papers: Hybrid Atomistic-Parametric Decoherence Model for …
Understanding the physical processes that determine the relaxation $T_{1}$ and dephasing $T_2$ times of molecular spin qubits is critical for envisioned applications in quantum metrology and information processing. Recent spin-echo $T_1$…
Quantum sensors and qubits are usually two-level systems (TLS), the quantum analogs of classical bits which assume binary values '0' or '1'. They are useful to the extent to which they can persist in quantum superpositions of '0' and '1' in…
The quantum nature of a microscopic system can only be revealed when it is sufficiently decoupled from surroundings. Interactions with the environment induce relaxation and decoherence that turn the quantum state into a classical mixture.…
We present a study of the prospects for coherence preservation in solid-state spin qubits using dynamical decoupling protocols. Recent experiments have provided the first demonstrations of multipulse dynamical decoupling sequences in this…
Molecular nanomagnets are quantum spin systems potentially serving as qudits for future quantum technologies thanks to their many accessible low-energy states. At low temperatures, the primary source of error in these systems is pure…
The realization of spin-based logical gates crucially depends on magnetically-coupled spin qubits. Thus, understanding decoherence when spin qubits are in close proximity will become a roadblock to overcome. Herein, we provide a general…
A major problem facing the realisation of scalable solid-state quantum computing is that of overcoming decoherence - the process whereby phase information encoded in a qubit is lost as the qubit interacts with its environment. Due to the…
We consider quantum decoherence in solid-state systems by studying the transverse dynamics of a single qubit interacting with a fermionic bath and driven by external pulses. Our interest is in investigating the extent to which the lost…
Spin qubits in semiconductor quantum dots are one of the promizing devices to realize a quantum processor. A better knowledge of the noise sources affecting the coherence of such a qubit is therefore of prime importance. In this work, we…
We consider the decoherence of a single localized electron spin due to its coupling to the lattice nuclear spin bath in a semiconductor quantum computer architecture. In the presence of an external magnetic field and at low temperatures,…
We investigate the decoherence of a qubit coupled to either a quantum two-level system (TLS) again coupled to an environment, or a classical fluctuator modeled by random telegraph noise. In order to do this we construct a model for the…
Understanding and controlling spin relaxation in molecular qubits is essential for developing chemically tunable quantum information platforms. We present a fully first-principles framework for computing the spin relaxation tensor in a…
In semiconductors, the T2* coherence time of a single confined spin is limited either by the fluctuating magnetic environment (via the hyperfine interaction), or by charge fluctuations (via the spin-orbit interaction). We demonstrate that…
Predicting the quantum dynamics of promising solid-state and molecular quantum technology candidates remains a formidable challenge. Yet, accessing these dynamics is key to understanding and controlling decoherence mechanisms -- a…
We explore how to encode more than a qubit in vanadyl porphyrin molecules hosting a electronic spin 1/2 coupled to a nuclear spin 7/2. The spin Hamiltonian and its parameters, as well as the spin dynamics, have been determined via a…
The evolution of a quantum system interacting with an environment can be described as a unitary process acting on both the system and the environment. In this framework, the system's evolution can be predicted by tracing out the…
The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…
A high degree of quantum coherence is a crucial requirement for the implementation of quantum logic devices. Solid state nanodevices seem particularly promising from the point of view of integrability and flexibility in the design. However…
Optically active solid-state spin defects are promising candidates for quantum applications, however a unified theoretical framework to predict their spin dynamics at high temperatures is not yet available. Here, using Kubo linear--response…
A successful and promising device for the physical implementation of electron spin-valley based qubits is the Transition Metal Dichalcogenide monolayer (TMD-ML) semiconductor quantum dot. The electron spin in TMD-ML semiconductor quantum…