English
Related papers

Related papers: Collective Vibronic Cascade in Cavity-Coupled Jahn…

200 papers

Enhancement of the sensitivities of optical magnetometers, atomic clocks and atom interferometers and other quantum metrology devices requires introducing new physical processes to improve on their present achievements. Many body collective…

Quantum Physics · Physics 2020-06-11 Reuben Shuker , Gennady A. Koganov

Resonant vibrational strong coupling (VSC) between molecular vibrations and quantized field modes of low-frequency optical cavities constitutes the conceptual cornerstone of vibro-polaritonic chemistry. In this work, we theoretically…

Chemical Physics · Physics 2025-12-02 Eric W. Fischer

Quantum dynamics of the photoisomerization of a single 3,3'-diethyl-2,2'-thiacynine iodide molecule embedded in an optical microcavity was theoretically studied. The molecule was coupled to a single cavity mode via the quantum Rabi…

Quantum Physics · Physics 2019-10-01 Juan B. Pérez-Sánchez , Joel Yuen-Zhou

We propose collective nuclear polaritons formed by hybridizing a 229Th nuclear ensemble with a vacuum-ultraviolet cavity mode generated via four-wave mixing, achieving a collective light-matter coupling that scales as $\sqrt{N}$. In the…

Quantum Physics · Physics 2026-03-17 Liufeng Yang , Jinling Wang , Huijun Li , Junhui Cao , Alexey Kavokin , Congjun Wu

The electromagnetic field in an optical cavity can dramatically modify and even control chemical reactivity via vibrational strong coupling (VSC). Since the typical vibration and cavity frequencies are considerably higher than thermal…

Quantum Physics · Physics 2021-09-29 Peiyun Yang , Jianshu Cao

Interaction between light and molecular vibrations leads to hybrid light-matter states called vibrational polaritons. Even though many intriguing phenomena have been predicted for single-molecule vibrational strong coupling (VSC), several…

A single cavity photon mode is expected to modify the Coulomb interaction of an electron system in the cavity. Here we investigate this phenomena in a parallel double quantum dot system. We explore properties of the closed system and the…

Mesoscale and Nanoscale Physics · Physics 2016-05-17 Vidar Gudmundsson , Anna Sitek , Nzar Rauf Abdullah , Chi-Shung Tang , Andrei Manolescu

A series of experiments demonstrate that strong light-matter coupling between vibrational excitations in isotropic solutions of molecules and resonant infrared optical microcavity modes leads to modified thermally-activated kinetics.…

Chemical Physics · Physics 2020-06-23 Jorge A. Campos-Gonzalez-Angulo , Joel Yuen-Zhou

Ultracold atoms uniformly filling an optical lattice can be treated like an artificial crystal. An implementation including the atomic occupation of a single excited atomic state can be represented by a two-component Bose-Hubbard model. Its…

Quantum Gases · Physics 2013-07-31 Hashem Zoubi , Helmut Ritsch

We study the dynamics of an one dimensional array of Jaynes-Cummings-Hubbard system of arbitrary number of coupled cavities, each containing a two level atom that interacts with a field mode. In particular, we consider propagation of a…

Quantum Physics · Physics 2011-03-04 R. Chakrabarti , G. Sreekumari

We assess the cavity molecular dynamics method for the calculation of vibrational polariton spectra, using liquid water as a specific example. We begin by disputing a recent suggestion that nuclear quantum effects may lead to a broadening…

The rapidly developing and converging fields of polaritonic chemistry and quantum optics necessitate a unified approach to predict strongly-correlated light-matter interactions with atomic-scale resolution. Combining concepts from both…

Quantum Physics · Physics 2018-09-19 Johannes Flick , Prineha Narang

As pioneering experiments have shown, strong vibrational coupling between molecular vibrations and light modes in an optical cavity can significantly alter molecular properties and even affect chemical reactivity. However, the current…

Chemical Physics · Physics 2024-07-26 Thomas Schnappinger , Markus Kowalewski

The demonstration of strong and ultrastrong coupling regimes of cavity QED with polyatomic molecules has opened new routes to control chemical dynamics at the nanoscale. We show that strong resonant coupling of a cavity field with an…

Quantum Physics · Physics 2016-06-09 Felipe Herrera , Frank C. Spano

When molecular transitions strongly couple to photon modes, they form hybrid light-matter modes called polaritons. Collective vibrational strong coupling is a promising avenue for control of chemistry, but this can be deterred by the large…

Jahn-Teller (JT) electron-phonon coupling effects in the colossal magnetoresistance perovskite compounds $La_{1-x}A_xMnO_3$ are investigated. Electron-electron correlations between two degenerate Mn $e_g$ orbitals are studied in the…

Condensed Matter · Physics 2009-10-28 Jun Zang , A. R. Bishop , H. Roder

We investigate the multi-photon resonance and multi-ion excitation in a single-mode cavity with identical vibrating ion-qubits, which enables the tripartite interaction among the internal states of ions, the cavity mode and the ions'…

Quantum Physics · Physics 2023-04-10 Wenjun Shao , Xun-Li Feng , Jian Li , Liang-Liang Wang

We experimentally study the interaction between a cold atom cloud and many longitudinal modes of a high quality Fabry-Perot cavity, by measuring signatures of collective light shifts in the cavity transmission spectrum of an optical…

Vibronic coupling parameters for C$_{60}^{+}$ were derived via DFT calculations with hybrid B3LYP and CAM-B3LYP functional, based on which the static Jahn-Teller effect were analyzed. The global minima of adiabatic potential energy surface…

Chemical Physics · Physics 2020-07-06 Zhishuo Huang , Dan Liu

This paper reviews recent experimental and theoretical developments of the dynamic Jahn-Teller effect-driven phenomena in heavy transition metal-based spin-orbit Mott insulators. In cubic $4d/5d$ transition metal compounds, the spin,…

Strongly Correlated Electrons · Physics 2024-11-13 Naoya Iwahara