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Classical physics is often a good approximation for quantum systems composed of many interacting particles, although wavepacket dispersion and scattering processes continuously induce delocalization and entanglement. According to…

Using a combination of high-level ab initio electronic structure methods with efficient on-the-fly semiclassical evaluation of nuclear dynamics, we performed a massive scan of small polyatomic molecules searching for a long lasting…

Chemical Physics · Physics 2024-09-26 Alan Scheidegger , Jiří Vaníček , Nikolay V. Golubev

We present an exact single-electron picture that describes the correlated electron dynamics in strong laser fields. Our approach is based on the factorization of the electronic wavefunction as a product of a marginal and a conditional…

Chemical Physics · Physics 2017-04-26 Axel Schild , E. K. U. Gross

The thorough treatment of electron-lattice interactions from first principles is one of the main goals in condensed matter physics. While the commonly applied adiabatic Born-Oppenheimer approximation is sufficient for describing many…

We present a universal expression for the electronic friction as felt by a set of classical nuclear degrees of freedom (DoF's) coupled to a manifold of quantum electronic DoF's; no assumptions are made regarding the nature of the electronic…

Materials Science · Physics 2017-08-02 Wenjie Dou , Gaohan Miao , Joseph E. Subotnik

We have discovered a class of dynamically stable coherent states for motion on the half-line. The regularization of the half-line boundary and the consequent quantum motion are expounded within the framework of covariant affine…

Quantum Physics · Physics 2024-02-01 Hervé Bergeron , Jean-Pierre Gazeau , Przemysław Małkiewicz , Patrick Peter

A generalized formalism of the so-called non-adiabatic quantum molecular dynamics is presented, which applies for atomic many-body systems in external laser fields. The theory treats the nuclear dynamics and electronic transitions…

Atomic Physics · Physics 2007-05-23 Thomas Kunert , Ruediger Schmidt

The conditions under which an open quantum mechanical system may be described by mixed quantum-classical dynamics are investigated. Decoherence is studied using influence functional methods in a model composite quantum system comprising two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Kazutomu Shiokawa , Raymond Kapral

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

Using a simple geometrical construction based upon the linear action of the Heisenberg--Weyl group we deduce a new nonlinear Schr\"{o}dinger equation that provides an exact dynamic and energetic model of any classical system whatsoever, be…

Quantum Physics · Physics 2014-05-27 K. R. W. Jones

Quantum cosmology implies corrections to the classical equations of motion which may lead to significant departures from the classical trajectory, especially at high curvature near the big-bang singularity. Corrections could in principle be…

General Relativity and Quantum Cosmology · Physics 2014-09-09 Martin Bojowald , David Simpson

Entanglement is at the core of quantum physics, playing a central role in quantum phenomena involving composite systems. According to the timeless picture of quantum dynamics, entanglement may also be essential for understanding the very…

Quantum Physics · Physics 2020-12-22 A. Valdés-Hernández , C. G. Maglione , A. P. Majtey , A. R. Plastino

We develop a new master equation as a unified description of the effects of both quantum noise (system-bath interaction) and classical noise on a system's dynamics, using a two-dimensional series expansion method. When quantum and classical…

Quantum Physics · Physics 2020-04-30 Li Yu

The standard wave function approach for the treatment of neutrino oscillations fails in situations where quantum ensembles at a finite temperature with or without an interacting background plasma are encountered. As a first step to treat…

High Energy Physics - Phenomenology · Physics 2015-05-27 Sebastian Hollenberg , Heinrich Päs

Predicting the quantum dynamics of promising solid-state and molecular quantum technology candidates remains a formidable challenge. Yet, accessing these dynamics is key to understanding and controlling decoherence mechanisms -- a…

Chemical Physics · Physics 2026-04-10 Tianchu Li , Pranay Venkatesh , Nanako Shitara , Andrés Montoya-Castillo

An ab initio, three-dimensional quantum mechanical calculation has been performed for the time-evolution of continuum electrons in the fields of moving charges. Here the essential singularity associated with the diverging phase factor in…

Atomic Physics · Physics 2009-11-13 Teck-Ghee Lee , S. Yu. Ovchinnikov , J. Sternberg , V. Chupryna , D. R. Schultz , J. H. Macek

We derive a "classical-quantum" approximation scheme for a broad class of bipartite quantum systems from fully quantum dynamics. In this approximation, one subsystem evolves via classical equations of motion with quantum corrections, and…

Quantum Physics · Physics 2023-06-05 Viqar Husain , Irfan Javed , Sanjeev S. Seahra , Nomaan X

Coherent or exact equations of motion for a post-Newtonian Lagrangian formalism are the Euler-Lagrange equations without any terms truncated. They naturally conserve energy {and} angular momentum. Doubling the phase-space variables of…

General Relativity and Quantum Cosmology · Physics 2021-12-14 Guifan Pan , Xin Wu , Enwei Liang

We study the evolution of the dynamics across a generic first order quantum phase transition in an interacting boson model of nuclei. The dynamics inside the phase coexistence region exhibits a very simple pattern. A classical analysis…

Nuclear Theory · Physics 2015-03-13 A. Leviatan , M. Macek

The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…

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