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Related papers: Unifying Decoherence and Phase Evolution in Mixed …

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In this article, we report the recent progress on decoherence dynamics of electrons in quantum dot quantum computing systems using the exact master equation we derived recently based on the Feynman-Vernon influence functional approach. The…

Mesoscale and Nanoscale Physics · Physics 2010-05-07 Matisse W. Y. Tu , Ming-Tsung Lee , Wei-Min Zhang

We discuss the various manifestations of quantum decoherence in the forms of dephasing, entanglement with the environment, and revelation of "which-path" information. As a specific example, we consider an electron interference experiment.…

Quantum Physics · Physics 2015-05-13 Jen-Tsung Hsiang , L. H. Ford

We present a new formulation of the correlated electron-ion dynamics (CEID) scheme, which systematically improves Ehrenfest dynamics by including quantum fluctuations around the mean-field atomic trajectories. We show that the method can…

Materials Science · Physics 2007-12-13 L. Stella , M. Meister , A. J. Fisher , A. P. Horsfield

Although the quantum classical Liouville equation (QCLE) arises by cutting off the exact equation of motion for a coupled nuclear-electronic system at order 1 (1 = $\hbar^0$ ), we show that the QCLE does include Berry's phase effects and…

Chemical Physics · Physics 2020-01-29 Joseph Subotnik , Gaohan Miao , Nicole Bellonzi , Hung-Hsuan Teh , Wenjie Dou

We derive an analytical expression of a Wigner function that approximately describes the time evolution of the one-dimensional motion of a particle in a nonharmonic potential. Our method involves two exact frame transformations, accounting…

The exact factorization approach, originally developed for electron-nuclear dynamics, is extended to light-matter interactions within the dipole approximation. This allows for a Schrodinger equation for the photonic wavefunction, in which…

Quantum Physics · Physics 2018-08-29 Norah M. Hoffmann , Heiko Appel , Angel Rubio , Neepa T. Maitra

An ab initio quantum-classical mixed scheme for the time evolution of electrode-device-electrode systems is introduced to study nuclear dynamics in quantum transport. Two model systems are discussed to illustrate the method. Our results…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Claudio Verdozzi , Gianluca Stefanucci , Carl-Olof Almbladh

Due to the electron correlation, a fast removal of an electron from a molecule may create a coherent superposition of cationic states and in this way initiate pure electronic dynamics in which the hole-charge left by ionization migrates…

Chemical Physics · Physics 2023-04-03 J. Vester , V. Despré , A. I. Kuleff

We introduce a theory that exposes the fundamental and previously overlooked connection between the correlation among electrons and the degree of quantum coherence of electronic states in matter. For arbitrary states, the effects only…

Quantum Physics · Physics 2016-04-21 Arnab Kar , Liping Chen , Ignacio Franco

We study the dynamics of initial nucleation processes of photoinduced structural change of molecular crystals. In order to describe the nonadiabatic transition in each molecule, we employ a model of localized electrons coupled with a fully…

Materials Science · Physics 2009-11-13 Kunio Ishida , Keiichiro Nasu

An accurate description of nonadiabatic dynamics of molecular species on metallic surfaces poses a serious computational challenge associated with a multitude of closely-spaced electronic states. We propose a mixed quantum-classical scheme…

Chemical Physics · Physics 2017-01-10 Ilya G. Ryabinkin , Artur F. Izmaylov

We study the interplay between ordered and chaotic dynamics at the critical point of a generic first-order quantum phase transition in the interacting boson model of nuclei. Classical and quantum analyses reveal a distinct behavior of the…

Nuclear Theory · Physics 2011-10-05 M. Macek , A. Leviatan

Conventional theoretical and computational approaches to fully coupled quantum molecular dynamics, i.e. when both the electrons and nuclei are treated as quantum-mechanical particles, are impractical for all but the smallest chemical…

Chemical Physics · Physics 2025-10-10 Julian Stetzler , Sophya Garashchuk , Vitaly A. Rassolov

A direct classical analog of quantum decoherence is introduced. Similarities and differences between decoherence dynamics examined quantum mechanically and classically are exposed via a second-order perturbative treatment and via a strong…

Quantum Physics · Physics 2009-11-07 Jiangbin Gong , Paul Brumer

A surface-hopping algorithm recently derived from the exact factorization approach, SHXF, [Ha, Lee, Min, J. Phys. Chem. Lett. 9, 1097 (2018)] introduces an additional term in the electronic equation of surface-hopping, which couples…

Chemical Physics · Physics 2022-02-08 Patricia Vindel-Zandbergen , Spiridoula Matsika , Neepa T. Maitra

We analytically solve the {\it Non-Markovian} single electron spin dynamics due to hyperfine interaction with surrounding nuclei in a quantum dot. We use the equation-of-motion method assisted with a large field expansion, and find that…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Changxue Deng , Xuedong Hu

Hyperfine interaction of electron spins with nuclear spins, in coupled double quantum dots is studied. Results of successive electron spin measurements exhibit bunching due to correlations induced via the nuclear spins. Further nuclear…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Ozgur Cakir , Toshihide Takagahara

Quantum entanglement is known as a unique quantum feature that cannot be obtained by classical physics. Over the last several decades, however, such an understanding on quantum entanglement might have confined us in a limited world of weird…

Quantum Physics · Physics 2023-08-01 B. S. Ham

Deformation quantization is a powerful tool to quantize some classical systems especially in noncommutative space. In this work we first show that for a class of special Hamiltonian one can easily find relevant time evolution functions and…

Mathematical Physics · Physics 2009-04-03 Bing-Sheng Lin , Si-Cong Jing , Tai-Hua Heng

We describe quantum and classical Hamiltonian dynamics in a common Hilbert space framework, that allows the treatment of mixed quantum-classical systems. The analysis of some examples illustrates the possibility of entanglement between…

Quantum Physics · Physics 2011-11-28 H. R. Jauslin , D. Sugny