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In this work, we introduce a correction to the unitary coupled cluster method with single and double excitations (UCCSD) that incorporates the effects of missing triple excitations through a treatment that is correct through fifth-order in…

Chemical Physics · Physics 2025-09-08 Zachary W. Windom , Daniel Claudino

We present an efficient implementation of four-component linear response coupled cluster singles and doubles (4c-LRCCSD) theory that enables accurate and computationally efficient calculation of polarizabilities for systems containing heavy…

Chemical Physics · Physics 2025-09-17 Sudipta Chakraborty , Amrita Manna , T. Daniel Crawford , Achintya Kumar Dutta

Relativistic magnetic reconnection is a non-ideal plasma process that is a source of non-thermal particle acceleration in many high-energy astrophysical systems. Particle-in-cell (PIC) methods are commonly used for simulating reconnection…

High Energy Astrophysical Phenomena · Physics 2023-07-19 Hannah Klion , Revathi Jambunathan , Michael E. Rowan , Eloise Yang , Donald Willcox , Jean-Luc Vay , Remi Lehe , Andrew Myers , Axel Huebl , Weiqun Zhang

Systolic arrays and shared-L1-memory manycore clusters are commonly used architectural paradigms that offer different trade-offs to accelerate parallel workloads. While the first excel with regular dataflow at the cost of rigid…

Hardware Architecture · Computer Science 2024-04-25 Sergio Mazzola , Samuel Riedel , Luca Benini

We report internally contracted relativistic multireference configuration interaction (ic-MRCI), complete active space second-order perturbation (CASPT2), and strongly contracted n-electron valence state perturbation theory (NEVPT2) on the…

Chemical Physics · Physics 2015-12-31 Toru Shiozaki , Wataru Mizukami

In this work, we develop a mathematical framework for a Selected Configuration Interaction (SCI) algorithm within a bi-orthogonal basis for transcorrelated (TC) calculations. The bi-orthogonal basis used here serves as the equivalent of the…

Chemical Physics · Physics 2023-06-22 Abdallah Ammar , Anthony Scemama , Emmanuel Giner

Near-term quantum devices require wavefunction ans\"atze that are expressive while also of shallow circuit depth in order to both accurately and efficiently simulate molecular electronic structure. While unitary coupled cluster (e.g.,…

We propose a new multi-scale molecular dynamics simulation method which can achieve high accuracy and high sampling efficiency simultaneously without aforehand knowledge of the coarse grained (CG) potential and test it for a biomolecular…

Biological Physics · Physics 2009-08-05 Wenfei Li , Shoji Takada

While restricted single-reference coupled cluster theory truncated to singles and doubles (CCSD) provides very accurate results for weakly correlated systems, it usually fails in the presence of static or strong correlation. This failure is…

Chemical Physics · Physics 2016-02-25 Ireneusz W. Bulik , Thomas M. Henderson , Gustavo E. Scuseria

The scale and complexity of quantum system to which real-space quantum Monte Carlo (QMC) can be applied in part depends on the representation and memory usage of the trial wavefunction. B-splines, the computationally most efficient basis…

Materials Science · Physics 2018-09-05 Ye Luo , Kenneth P. Esler , Paul R. C. Kent , Luke Shulenburger

Global correlations are widely seen in human anatomical structures due to similarity across tissues and bones. These correlations are reflected in magnetic resonance imaging (MRI) scans as a result of close-range proton density and T1/T2…

Image and Video Processing · Electrical Eng. & Systems 2022-12-22 Mevan Ekanayake , Kamlesh Pawar , Mehrtash Harandi , Gary Egan , Zhaolin Chen

Quantum chemistry calculations of large, strongly correlated systems are typically limited by the computation cost that scales exponentially with the size of the system. Quantum algorithms, designed specifically for quantum computers, can…

RISC-V CPUs leverage the RVV (RISC-V Vector) extension to accelerate data-parallel workloads. In addition to arithmetic operations, RVV includes powerful permutation instructions that enable flexible element rearrangement within vector…

Hardware Architecture · Computer Science 2025-06-02 Vasileios Titopoulos , George Alexakis , Chrysostomos Nicopoulos , Giorgos Dimitrakopoulos

The variational quantum eigensolver (VQE) algorithm, designed to calculate the energy of molecular ground states on near-term quantum computers, requires specification of symmetries that describe the system, e.g. spin state and number of…

Quantum Physics · Physics 2020-06-18 Gabriel Greene-Diniz , David Muñoz Ramo

Recent works have demonstrated that large quantum circuits can be cut and decomposed into smaller clusters of quantum circuits with fewer qubits that can be executed independently on a small quantum computer. Classical post-processing then…

Quantum Physics · Physics 2022-11-15 Gideon Uchehara , Tor M. Aamodt , Olivia Di Matteo

Redshift measurement of active galactic nuclei (AGNs) remains a time-consuming and challenging task, as it requires follow up spectroscopic observations and detailed analysis. Hence, there exists an urgent requirement for alternative…

We merge two successful ab initio nuclear-structure methods, the no-core shell model (NCSM) and the multi-reference in-medium similarity renormalization group (IM-SRG) to define a new many-body approach for the comprehensive description of…

Nuclear Theory · Physics 2017-04-20 Eskendr Gebrerufael , Klaus Vobig , Heiko Hergert , Robert Roth

Reservoir computing (RC) is an effective method for predicting chaotic systems by using a high-dimensional dynamic reservoir with fixed internal weights, while keeping the learning phase linear, which simplifies training and reduces…

Resistive In-Memory Computing (RIMC) offers ultra-efficient computation for edge AI but faces accuracy degradation due to RRAM conductance drift over time. Traditional retraining methods are limited by RRAM's high energy consumption, write…

Hardware Architecture · Computer Science 2025-04-08 Weirong Dong , Kai Zhou , Zhen Kong , Quan Cheng , Junkai Huang , Zhengke Yang , Masanori Hashimoto , Longyang Lin

We present a new C++ code for collisional N-body simulations of star clusters. The code uses the Hermite fourth-order scheme with block time steps, for advancing the particles in time, while the forces and neighboring particles are computed…

Instrumentation and Methods for Astrophysics · Physics 2010-11-08 Simos Konstantinidis , Kostas D. Kokkotas