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The original observation of the Einstein-de Haas effect was a landmark experiment in the early history of modern physics that illustrates the relationship between magnetism and angular momentum. Today the effect is still discussed in…

The orbital angular momenta (OAM) of electrons play an increasingly important role in ultrafast electron and magnetization dynamics. In this theoretical study, we investigate the electron dynamics induced by femtosecond laser pulses in a…

Materials Science · Physics 2023-10-13 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

Experimentally observed ultrafast all-optical magnetization reversal in ferrimagnetic metals and heterostructures based on antiferromagnetically coupled ferromagnetic $d-$ and $f-$metallic layers relies on intricate energy and angular…

Strongly Correlated Electrons · Physics 2016-03-02 Alexandra Kalashnikova , Veniamin Kozub

Light-matter interaction at the nanoscale in magnetic alloys and heterostructures is a topic of intense research in view of potential applications in high-density magnetic recording. While the element-specific dynamics of electron spins is…

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

Femtosecond laser induced ultrafast magnetization dynamics have been studied in multisublattice CoxDy1-x alloys. By performing element and time-resolved X-ray spectroscopy, we distinguish the ultrafast quenching of Co3d and Dy4f magnetic…

Materials Science · Physics 2017-10-16 T. Ferte , N. Bergeard , L. Le Guyader , M. Hehn , G. Malinowski , E. Terrier , E. Otero , K. Holldack , N. Pontius , C. Boeglin

Femtosecond laser-pulse excitation provides an energy efficient and fast way to control magnetization at the nanoscale, providing great potential for ultrafast next-generation data manipulation and nonvolatile storage devices. Ferromagnetic…

Understanding how fast short-range interactions build up long-range order is one of the most intriguing topics in condensed matter physics. FeRh is a test specimen for studying this problem in magnetism, where the microscopic spin-spin…

We report on optically induced, ultrafast magnetization dynamics in the Heusler alloy $\mathrm{Co_{2}FeAl}$, probed by time-resolved magneto-optical Kerr effect. Experimental results are compared to results from electronic structure theory…

Controlling magnetic order on ultrafast timescales, driven by spintronic and recording applications, is one of the main directions of current research in magnetism. Despite major advances in understanding the temporal evolution of magnetic…

Femtosecond laser pulses can induce ultrafast demagnetization as well as generate bursts of hot electron spin currents. In trilayer spin valves consisting of two metallic ferromagnetic layers separated by a nonmagnetic one, hot electron…

Materials Science · Physics 2020-05-27 Ulrike Ritzmann , Pavel Baláž , Pablo Maldonado , Karel Carva , Peter M. Oppeneer

We develop a theory of the magnetization dynamics triggered by ultrafast optical excitation of ferromagnetic semiconductors. We describe the effects of the strong carrier spin relaxation on the nonlinear optical response by using the…

Strongly Correlated Electrons · Physics 2008-08-04 J. Chovan , E. G. Kavousanaki , I. E. Perakis

Ultrafast heating of FeRh by a femtosecond laser pulse launches a magneto-structural phase transition from an antiferromagnetic to a ferromagnetic state. Aiming to reveal the ultrafast kinetics of this transition, we studied magnetization…

We investigate the ultrafast magnetization dynamics of an interlayer-exchange-coupled Co/Mn/Co trilayer system after excitation with an ultrafast optical pump. We probe element- and time-resolved ferromagnetic order by X-ray magnetic…

Laser-induced ultrafast demagnetization is an important phenomenon that probes arguably ultimate limits of the angular momentum dynamics in solid. Unfortunately, many aspects of the dynamics remain unclear except that the demagnetization…

Materials Science · Physics 2023-07-03 Kyuhwe Kang , Hiroki Omura , Oukjae Lee , Kyung-Jin Lee , Hyun-Woo Lee , Tomoyasu Taniyama , Gyung-Min Choi

Engineering and controlling heat and spin transport on the femtosecond time-scale in spintronic devices opens up new ways to manipulate magnetization with unprecedented speed. Yet the underlying reversal mechanisms remain poorly understood…

Mesoscale and Nanoscale Physics · Physics 2026-02-04 Harjinder Singh , Alberto Anadón , Junta Igarashi , Quentin Remy , Stéphane Mangin , Michel Hehn , Jon Gorchon , Gregory Malinowski

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

We study ultrafast magnetization quenching of ferromagnetic iron following excitation by an optical vs a terahertz pump pulse. While the optical pump (photon energy of 3.1 eV) induces a strongly nonthermal electron distribution, terahertz…

Here we carry out a first-principles time-dependent calculation to investigate how fast electrons actually move under laser excitation and how large the electron transport affects demagnetization on the shortest time scale. To take into…

Materials Science · Physics 2018-11-14 G. P. Zhang , Y. H. Bai , T. Jenkins , T. F. George

Ultrafast demagnetization of magnetic layers pumped by a femtosecond laser pulse is accompanied by a nonthermal spin-polarized current of hot electrons. These spin currents are studied here theoretically in a spin valve with noncollinear…

Mesoscale and Nanoscale Physics · Physics 2018-02-26 Pavel Baláž , Martin Žonda , Karel Carva , Pablo Maldonado , Peter M. Oppeneer