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Generative models of 3D molecular structure play a rapidly growing role in the design and simulation of molecules. Diffusion models currently dominate the space of 3D molecule generation, while autoregressive models have trailed behind. In…

Machine Learning · Computer Science 2025-09-10 Austin H. Cheng , Chong Sun , Alán Aspuru-Guzik

With the recent advances in machine learning for quantum chemistry, it is now possible to predict the chemical properties of compounds and to generate novel molecules. Existing generative models mostly use a string- or graph-based…

Biomolecules · Quantitative Biology 2020-10-14 Vitali Nesterov , Mario Wieser , Volker Roth

Transformer-based autoregressive models offer an efficient alternative to diffusion- and flow-matching-based approaches for generating 3D molecules. One challenge remains: standard transformer architectures require a sequential ordering of…

Machine Learning · Computer Science 2026-05-07 Daniel Rose , Roxane Axel Jacob , Johannes Kirchmair , Thierry Langer

3D structure modeling is essential across scales, enabling applications from fluid simulation and 3D reconstruction to protein folding and molecular docking. Yet, despite shared 3D spatial patterns, current approaches remain fragmented,…

Machine Learning · Computer Science 2025-10-10 Shuqi Lu , Haowei Lin , Lin Yao , Zhifeng Gao , Xiaohong Ji , Yitao Liang , Weinan E , Linfeng Zhang , Guolin Ke

This paper presents Diffusion via Autoregressive models (D-AR), a new paradigm recasting the image diffusion process as a vanilla autoregressive procedure in the standard next-token-prediction fashion. We start by designing the tokenizer…

Computer Vision and Pattern Recognition · Computer Science 2025-05-30 Ziteng Gao , Mike Zheng Shou

Auto-Regressive (AR) models have achieved impressive results in 2D image generation by modeling joint distributions in the grid space. While this approach has been extended to the 3D domain for powerful shape generation, it still has two…

Computer Vision and Pattern Recognition · Computer Science 2023-03-28 Simian Luo , Xuelin Qian , Yanwei Fu , Yinda Zhang , Ying Tai , Zhenyu Zhang , Chengjie Wang , Xiangyang Xue

Autoregressive (AR) models have reformulated image generation as next-token prediction, demonstrating remarkable potential and emerging as strong competitors to diffusion models. However, control-to-image generation, akin to ControlNet,…

Computer Vision and Pattern Recognition · Computer Science 2025-03-11 Zongming Li , Tianheng Cheng , Shoufa Chen , Peize Sun , Haocheng Shen , Longjin Ran , Xiaoxin Chen , Wenyu Liu , Xinggang Wang

Inspired by the remarkable success of autoregressive models in language modeling, this paradigm has been widely adopted in visual generation. However, the sequential token-by-token decoding mechanism inherent in traditional autoregressive…

Computer Vision and Pattern Recognition · Computer Science 2026-01-01 Siyang Wang , Hanting Li , Wei Li , Jie Hu , Xinghao Chen , Feng Zhao

Autoregressive (AR) models have achieved remarkable success in natural language and image generation, but their application to 3D shape modeling remains largely unexplored. Unlike diffusion models, AR models enable more efficient and…

Computer Vision and Pattern Recognition · Computer Science 2026-01-12 Tejaswini Medi , Arianna Rampini , Pradyumna Reddy , Pradeep Kumar Jayaraman , Margret Keuper

Machine learning has the potential to automate molecular design and drastically accelerate the discovery of new functional compounds. Towards this goal, generative models and reinforcement learning (RL) using string and graph…

Machine Learning · Computer Science 2022-02-02 Daniel Flam-Shepherd , Alexander Zhigalin , Alán Aspuru-Guzik

Autoregressive visual generation has garnered increasing attention due to its scalability and compatibility with other modalities compared with diffusion models. Most existing methods construct visual sequences as spatial patches for…

Computer Vision and Pattern Recognition · Computer Science 2025-06-13 Yuanhui Huang , Weiliang Chen , Wenzhao Zheng , Yueqi Duan , Jie Zhou , Jiwen Lu

The application of language models (LMs) to molecular structure generation using line notations such as SMILES and SELFIES has been well-established in the field of cheminformatics. However, extending these models to generate 3D molecular…

Machine Learning · Computer Science 2024-12-03 Kaiyuan Gao , Yusong Wang , Haoxiang Guan , Zun Wang , Qizhi Pei , John E. Hopcroft , Kun He , Lijun Wu

Molecule generation is a very important practical problem, with uses in drug discovery and material design, and AI methods promise to provide useful solutions. However, existing methods for molecule generation focus either on 2D graph…

Machine Learning · Computer Science 2024-02-07 Chenqing Hua , Sitao Luan , Minkai Xu , Rex Ying , Jie Fu , Stefano Ermon , Doina Precup

Shape-based virtual screening is widely employed in ligand-based drug design to search chemical libraries for molecules with similar 3D shapes yet novel 2D chemical structures compared to known ligands. 3D deep generative models have the…

Chemical Physics · Physics 2022-10-12 Keir Adams , Connor W. Coley

State-of-the-art models for 3D molecular generation are based on significant inductive biases, SE(3), permutation equivariance to respect symmetry and graph message-passing networks to capture local chemistry, yet the generated molecules…

Machine Learning · Computer Science 2025-07-02 Carlos Vonessen , Charles Harris , Miruna Cretu , Pietro Liò

Autoregressive Model (AR) has shown remarkable success in conditional image generation. However, these approaches for multiple reference generation struggle with decoupling different reference identities. In this work, we propose the…

Computer Vision and Pattern Recognition · Computer Science 2025-10-21 Haiyue Sun , Qingdong He , Jinlong Peng , Peng Tang , Jiangning Zhang , Junwei Zhu , Xiaobin Hu , Shuicheng Yan

Autoregressive models have demonstrated remarkable success across various fields, from large language models (LLMs) to large multimodal models (LMMs) and 2D content generation, moving closer to artificial general intelligence (AGI). Despite…

Computer Vision and Pattern Recognition · Computer Science 2025-03-25 Yongwei Chen , Yushi Lan , Shangchen Zhou , Tengfei Wang , Xingang Pan

Autoregressive models (ARMs) have become the workhorse for sequence generation tasks, since many problems can be modeled as next-token prediction. While there appears to be a natural ordering for text (i.e., left-to-right), for many data…

Machine Learning · Computer Science 2025-07-15 Zhe Wang , Jiaxin Shi , Nicolas Heess , Arthur Gretton , Michalis K. Titsias

We consider molecule generation in 3D space using language models (LMs), which requires discrete tokenization of 3D molecular geometries. Although tokenization of molecular graphs exists, that for 3D geometries is largely unexplored. Here,…

Artificial Intelligence · Computer Science 2024-08-20 Xiner Li , Limei Wang , Youzhi Luo , Carl Edwards , Shurui Gui , Yuchao Lin , Heng Ji , Shuiwang Ji

Autoregressive (AR) image generators offer a language-model-friendly approach to image generation by predicting discrete image tokens in a causal sequence. However, unlike diffusion models, AR models lack a mechanism to refine previous…

Computer Vision and Pattern Recognition · Computer Science 2026-01-29 Cheng Cheng , Lin Song , Di An , Yicheng Xiao , Xuchong Zhang , Hongbin Sun , Ying Shan
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