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Selective control of light is essential for optical science and technology with numerous applications. Nanophotonic waveguides and integrated couplers have been developed to achieve selective coupling and spatial control of an optical beam…

We study the two-step spin crossover in a double-layered elastic model based on transition metal complexes each taking high spin (HS) and low spin (LS) states. Here, only the simplest elastic interactions between adjacent molecules are…

Materials Science · Physics 2017-11-15 Daisuke Taniguchi , Jun Okabayashi , Chisa Hotta

In spin crossover materials, an abrupt phase transition between a low spin state and a high spin state can be driven by temperature, pressure or by light irradiation. Of a special relevance are Fe(II) based coordination polymers where, in…

We have observed an electronic energy level crossing in a molecular nanomagnet (MNM) using muon-spin relaxation. This effect, not observed previously despite several muon studies of MNM systems, provides further evidence that the spin…

Strongly Correlated Electrons · Physics 2015-05-27 T. Lancaster , J. S. Moeller , S. J. Blundell , F. L. Pratt , P. J. Baker , T. Guidi , G. A. Timco , R. E. P. Winpenny

On the spin-valve-like ferromagnet/spin glass/ferromagnet (FM/SG/FM) structure, the tunneling current is dominated by resistance switch (RS) instead of the local density of states according to the conventional tunneling theory. Here we show…

Using the Landau-Ginzburg-Devonshire approach, we study light-induced phase transitions, evolution of polar state and domain morphology in photo-ferroelectric nanoparticles (NPs). Light exposure increases the free carrier density near the…

We study and actively control the coherent properties of Surface Plasmon Polaritons (SPPs) optically exited on a nano-hole array. Amplitude and phase of the optical excitation are externally controlled via a digital spatial light modulator…

Optics · Physics 2013-04-05 B. Gjonaj , J. Aulbach , P. M. Johnson , A. P. Mosk , L. Kuipers , A. Lagendijk

We show, both theoretically and experimentally, that high-numerical-aperture (NA) optical microscopy is accompanied by strong spin-orbit interaction of light, which translates fine infomation about the specimen to the polarization degrees…

Self-assembled functionalized nano particles are at the focus of a number of potential applications, in particular for molecular scale electronics devices. Here we perform experiments of self-assembly of 10 nm Au nano particles (NPs),…

Mesoscale and Nanoscale Physics · Physics 2015-09-15 Yannick Viero , Guillaume Copie , David Guerin , Christophe Krzeminski , Dominique Vuillaume , Stephane Lenfant , Fabrizio Cleri

Light-matter interactions are frequently perceived as predominantly influenced by the electric optical field, with the magnetic component of light often overlooked. Nonetheless, the magnetic aspect plays a pivotal role in various optical…

Pressure-induced phase transitions of spin-crossover materials were simulated by a Monte Carlo simulation in the constant pressure ensemble for the first time. Here, as the origin of the cooperative interaction, we adopt elastic interaction…

Materials Science · Physics 2008-04-09 Yusuke Konishi , Hiroko Tokoro , Masamichi Nishino , Seiji Miyashita

We present a detailed theoretical study of the recent proposal for selective nanomanipulation of nanometric particles above a substrate using near-field optical forces [Chaumet {\it et al.} Phys. Rev. Lett. {\bf 88}, 123601 (2002)].…

Optics · Physics 2009-11-10 Patrick C. Chaumet , Adel Rahmani , Manuel Nieto-Vesperinas

Molecular spin crossover switches are the objects of intense theoretical and experimental studies in recent years. This interest is due to the fact that these systems allow one to control their spin state by applying an external photo-,…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 Oleg V. Farberovich , Victoria L. Mazalova , Valeri S. Stepanyuk

We investigate dissipative phase transitions in an open central spin system. In our model the central spin interacts coherently with the surrounding many-particle spin environment and is subject to coherent driving and dissipation. We…

Manipulating the spin polarization of electron beams using light is highly desirable but exceedingly challenging, as the approaches proposed in previous studies using free-space light usually require enormous laser intensities. Here, we…

Optics · Physics 2022-06-22 Deng Pan , Hongxing Xu

We investigate the signature of magnetic surface anisotropy in nanoparticles in their spin-flip neutron scattering cross section. Taking into account the isotropic exchange interaction, an external magnetic field, a uniaxial or cubic…

Materials Science · Physics 2023-11-13 Michael P. Adams , Evelyn Pratami Sinaga , Hamid Kachkachi , Andreas Michels

Nanosphere-on-mirror plasmonic antennas, each having a monolayer graphene or MoS2 sheet in the gap, were pumped with a femtosecond laser. Abrupt turnings in the scattering linewidth and peak intensity trends as the laser power changed were…

Optics · Physics 2020-12-24 Tian Yang , Hui Yi , Xiaodan Wang , Yichen Miao , Cheng Chen , Jing Long , Xiangyang Kong , Lin Wu

Spin crossover molecules have recently emerged as a family of compounds potentially useful for implementing molecular spintronics devices. The calculations of the electronic properties of such molecules is a formidable theoretical challenge…

Materials Science · Physics 2015-06-04 Andrea Droghetti , Dario Alfe' , Stefano Sanvito

Spin-polarized scanning tunneling microscopy has been applied to study non-collinear spin textures of a Mn monolayer on a four-fold symmetric W(001) substrate revealing a zero-field spin spiral ground state and two different types of…

Mesoscale and Nanoscale Physics · Physics 2022-06-15 Reiner Brüning , André Kubetzka , Kirsten von Bergmann , Elena Y. Vedmedenko , Roland Wiesendanger

Electronic spin superposition states enable nanoscale sensing through their sensitivity to the local environment, yet their sensitivity to vibrational motion also limits their coherence times. In molecular spin systems, chemical tunability…

Quantum Physics · Physics 2026-02-04 Stefan H. Lohaus , Kay T. Xia , Yongqiang Cheng , Ryan G. Hadt