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Defects in two-dimensional transition metal dichalcogenides (TMDCs) broadly affect their optical and electronic properties. Directly capturing the ultrafast processes of exciton trapping and defect-bound exciton formation is crucial for…

Non-volatile resistive switching, also known as memristor effect in two terminal devices, has emerged as one of the most important components in the ongoing development of high-density information storage, brain-inspired computing, and…

Mesoscale and Nanoscale Physics · Physics 2020-02-06 Saban M. Hus , Ruijing Ge , Po-An Chen , Meng-Hsueh Chiang , Gavin E. Donnelly , Wonhee Ko , Fumin Huang , Liangbo Liang , An-Ping Li , Deji Akinwande

Large chemical tunability and strong light-matter interactions make colloidal transition metal dichalcogenide (TMD) nanostructures particularly suitable for light-emitting applications. However, ultrafast exciton decay and quenched…

The weakly screened electron-hole interactions in an atomically thin semiconductor not only downshift its excitation spectrum from a quasiparticle one, but also redistribute excitation energies and wavefunction characters with profound…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Yuanxi Wang , Bruno R. Carvalho , Vincent H. Crespi

Semiconducting monolayer of 2D material are able to concatenate multiple interesting properties into a single component. Here, by combining opto-mechanical and electronic measurements, we demonstrate the presence of a partial 2H-1T phase…

The new generation of two-dimensional (2D) materials has shown a broad range of applications for optical and electronic devices. Understanding the properties of these materials when integrated with the more traditional three-dimensional…

Strain engineering is a powerful tool for tuning physical properties of 2D materials, including monolayer transition metal dichalcogenides (TMD) -- direct bandgap semiconductors with strong excitonic response. Here, we demonstrate an…

Hexagonal boron nitride (hBN) has emerged as a promising material platform for nanophotonics and quantum sensing, hosting optically-active defects with exceptional properties such as high brightness and large spectral tuning. However,…

We calculate the excitation spectrum of single-layer MoS$_2$ at several hydrogen coverages by using a method based on first-principles Density-Matrix Time-Dependent Density-Functional Theory (TDDFT). Our results show that the fully…

Materials Science · Physics 2020-12-30 Naseem Ud Din , Volodymyr Turkowski , Talat S. Rahman

Engineering and probing excitonic properties at the nanoscale remains a central challenge in quantum photonics and optoelectronics. While exciton confinement via electrical control and strain engineering has been demonstrated in 2D…

Mesoscale and Nanoscale Physics · Physics 2025-09-03 Yueh-Chun Wu , Bogdan Dryzhakov , Huan Zhao , Ivan Vlassiouk , Kyle Kelley , Takashi Taniguchi , Kenji Watanabe , Jun Yan , Benjamin Lawrie

The excitonic radiative recombination of intercalated Cl2 molecules for two different polytypes 2H-MoS2 and 3R-MoS2 layered crystals are presented. The structure of the excitonic emission is unique and provides a robust experimental…

Materials Science · Physics 2014-11-17 S. Anghel , Yu. Chumakov , V. Kravtsov , A. Mitioglu , P. Plochocka , K. Sushkevich , G. Volodina , A. Colev , L. Kulyuk

Defects play a key role in determining the properties of most materials and, because they tend to be highly localized, characterizing them at the single-defect level is particularly important. Scanning tunneling microscopy (STM) has a…

By using first-principles calculations, we investigated the monolayer $ReS_2$ with vacancies under strain engineering, specifically focusing on its energy of formation, band gap, electron density of states, effective mass and optical…

Materials Science · Physics 2016-11-28 Y. M. Min , L. Z. Liu

Spatially resolved EELS has been performed at diffuse interfaces between MoS$_2$ and MoSe$_2$ single layers. With a monochromated electron source (20 meV) we have successfully probed excitons near the interface by obtaining the low loss…

Mesoscale and Nanoscale Physics · Physics 2019-06-25 Luiz H. G. Tizei , Yung-Chang Lin , Masaki Mukai , Hidetaka Sawada , Ang-Yu Lu , Lain-Jong Li , Koji Kimoto , Kazu Suenaga

Transition metal dichalcogenides layered nano-crystals are emerging as promising candidates for next-generation optoelectronic and quantum devices. In such systems, the interaction between excitonic states and atomic vibrations is crucial…

Mesoscale and Nanoscale Physics · Physics 2023-12-29 Jianbo Hu , Yang Xiang , Beatrice Matilde Ferrari , Emilio Scalise , Giovanni Maria Vanacore

Transition metal dichalcogenides (TMDs) attract significant attention as potential building blocks in next-generation electronic devices. On the other hand, a comprehensive understanding of how various defects affect local electronic…

Materials Science · Physics 2026-04-28 Joshua R. Evans , Diego A. Garibay , Aiden N. Kuhls , Mehmet Z. Baykara

Two dimensional materials and their heterostructures constitute a promising platform to study correlated electronic states as well as many body physics of excitons. Here, we present experiments that unite these hitherto separate efforts and…

Mesoscale and Nanoscale Physics · Physics 2020-05-12 Yuya Shimazaki , Ido Schwartz , Kenji Watanabe , Takashi Taniguchi , Martin Kroner , Ataç Imamoğlu

Monolayer transition metal dichalcogenide (TMD) semiconductors such as MoSe$_2$ host strongly bound excitons which are known to exhibit a strong resonant third-order nonlinear response. Although there have been numerous studies of the…

Achieving localized light emission from monolayer two-dimensional (2D) transition metal dichalcogenides (TMDs) embedded in the matrix of another TMD has been theoretically proposed but not experimentally proven. In this study, we used…

Optically addressable spins in materials are important platforms for quantum technologies, such as repeaters and sensors. Identification of such systems in two-dimensional (2d) layered materials offers advantages over their bulk…