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High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

In this paper we discuss a method for nondestructive measurements of the longitudinal profile of sub-picosecond electron bunches for X-Ray Free Electron Lasers (XFELs). The method is based on the detection of the Coherent Synchrotron…

Accelerator Physics · Physics 2007-05-23 G. A. Geloni , E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…

Computational Physics · Physics 2026-05-19 Zhenjiang Zhao , Zhihua Zheng , Zhiyi Xu , Xing Ran , Xiaolong Yao , Fangping Ouyang

High harmonic generation by relativistically intense laser pulses from overdense plasma layers is surveyed. High harmonics are generated in form of (sub-)attosecond pulses when the plasma surface rebounds towards the observer with…

Plasma Physics · Physics 2011-11-18 Daniel an der Brügge , Alexander Pukhov

A new method to generate short wavelength Free Electron Laser output with modulated polarisation at attosecond timescales is presented. Simulations demonstrate polarisation switching timescales that are four orders of magnitude faster than…

Accelerator Physics · Physics 2021-01-20 J. Morgan , B. W. J. McNeil

We present a model for quasi-phase matching (QPM) in high-order harmonic generation (HHG). Using a one-dimensional description, we analyze the time-dependent, ultrafast wave-vector balance to calculate the on-axis harmonic output versus…

Acting as a highly nonlinear response to the strong laser field, high harmonic generation (HHG) naturally contains the fingerprints of atomic and electronic properties of materials. Electronic properties of a solid such as band structure…

Materials Science · Physics 2023-04-20 Shi-Qi Hu , Hui Zhao , Xin-Bao Liu , Da-Qiang Chen , Sheng Meng

Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials…

Quantum Physics · Physics 2021-01-27 Valerio Di Giulio , F. Javier García de Abajo

High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require…

A technique is proposed to generate attosecond pulse trains of radiation from a Free-Electron Laser amplifier. The optics-free technique synthesises a comb of longitudinal modes by applying a series of spatio-temporal shifts between the…

Optics · Physics 2008-11-26 N. R. Thompson , B. W. J. McNeil

Harmonic generation from solid surfaces is a promising tool for producing high energy attosecond pulses. We report shaping of the harmonic spectrum to achieve the bandwidth necessary for attosecond pulse generation. The shaping is…

Plasma Physics · Physics 2019-03-27 A. Seyen , R. Kohn , U. Bovensiepen , D. von der Linde , A. Tarasevitch

We make a systematic study of high-order harmonic generation (HHG) in a He$^+$-like model ion when the initial states are prepared as a coherent superposition of the ground state and an excited state. It is found that, according to the…

Atomic Physics · Physics 2009-11-11 Bingbing Wang , Taiwang Cheng , Xiaofeng Li , Panming Fu , Shigang Chen , Jie Liu

In this paper we propose a new method for measurements of the longitudinal profile of 100 femtosecond electron bunches for X-ray Free Electron Lasers (XFELs). The method is simply the combination of two well-known techniques, which where…

Accelerator Physics · Physics 2009-11-10 E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

Various scientific and industrial researches such as spectroscopy and advanced nano-technologies have been demanding high flux and fully coherent EUV and X-ray radiation. These demands can be commendably satisfied with a MHz-level…

Accelerator Physics · Physics 2024-04-29 Xiaofan Wang , Chao Feng , Bart Faatz , Weiqing Zhang , Zhentang Zhao

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

Attosecond pulses from X-ray free-electron laser (XFEL) have opened new opportunities for probing ultrafast electronic dynamics on the Angstrom--attosecond spatiotemporal scale. Most attosecond XFEL concepts rely on generating an ultrashort…

Accelerator Physics · Physics 2026-04-22 Chenzhi Xu , Jiawei Yan , Ye Chen , Winfried Decking , Marc Guetg , Tianyun Long , Bingyang Yan , Haixiao Deng

The interaction between relativistic electron beams and intense laser fields has been extensively studied for generating high-energy radiation. However, achieving coherent radiation from such interactions needs to precisely control the…

Plasma Physics · Physics 2025-09-01 H. Peng , T. W. Huang , C. N. Wu , K. Jiang , R. Li , C. Riconda , S. Weber , C. T. Zhou

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang