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Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

Strongly Correlated Electrons · Physics 2021-09-15 Li Ern Chern , Yong Baek Kim

Spin-$1/2$ kagome antiferromagnets are leading candidates for realizing quantum spin liquid (QSL) ground states. While QSL ground states are predicted for the pure Heisenberg model, understanding the robustness of the QSL to additional…

Strongly Correlated Electrons · Physics 2026-02-16 Shengtao Jiang , Arthur C. Campello , Wei He , Jiajia Wen , Daniel M. Pajerowski , Young S. Lee , Hong-Chen Jiang

We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

Strongly Correlated Electrons · Physics 2020-04-29 Ying Li , A. Pustogow , M. Bories , P. Puphal , C. Krellner , M. Dressel , Roser Valenti

Recent neutron scattering experiments on the spin-1/2 kagome lattice antiferromagnet ZnCu3(OH)6Cl2 (Herbertsmithite) provide the first evidence of fractionalized excitations in a quantum spin liquid state in two spatial dimensions. In…

Strongly Correlated Electrons · Physics 2014-04-03 Matthias Punk , Debanjan Chowdhury , Subir Sachdev

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

We report 17O NMR measurements in the S=1/2 Cu2+ kagome antiferromagnet Herbertsmithite ZnCu3(OH)6Cl2 down to 45mK in magnetic fields ranging from 2T to 12T. While Herbertsmithite displays a gapless spin-liquid behavior in zero field, we…

Strongly Correlated Electrons · Physics 2013-09-09 M. Jeong , F. Bert , P. Mendels , F. Duc , J. C. Trombe , M. A. de Vries , A. Harrison

Motivated by recent experimental observations of Kondo resonances in cobalt atoms on single layer 1T-TaSe$_{2}$, we theoretically investigate the effect of coupling a U(1) quantum spin liquid with a spinon Fermi surface to a lattice of…

Strongly Correlated Electrons · Physics 2024-04-01 Xia-Ming Zheng , Mehdi Kargarian

Quantum spin liquids are exotic many-body states featured with long-range entanglement and fractional anyon quasiparticles. Quantum phase transitions of spin liquids are particularly interesting problems related with novel phenomena of…

Strongly Correlated Electrons · Physics 2024-07-19 Kyusung Hwang

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…

Localized magnetic moments with crystal-field doublet or pseudo-spin 1/2 may arise in correlated insulators with even number of electrons and strong spin-orbit coupling. Such a non-Kramers pseudo-spin 1/2 is the consequence of crystalline…

Strongly Correlated Electrons · Physics 2013-11-13 Robert Schaffer , Subhro Bhattacharjee , Yong Baek Kim

Based on large-scale quantum Monte Carlo simulations, we examine the dynamical spin structure factor of the Balents-Fisher-Girvin kagome lattice quantum spin-$1/2$ model, which is known to harbor an extended $Z_2$ quantum spin liquid phase.…

Strongly Correlated Electrons · Physics 2018-08-27 Jonas Becker , Stefan Wessel

Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel…

Strongly Correlated Electrons · Physics 2017-01-06 A. Zorko , M. Herak , M. Gomilšek , J. van Tol , M. Velázquez , P. Khuntia , F. Bert , P. Mendels

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

Strongly Correlated Electrons · Physics 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

By means of quantum Monte Carlo simulations, combined with a stochastic analytic continuation, we examine the spin dynamics of the spin-1/2 planar (XY) ferromagnet on the kagome lattice with additional four-site ring exchange terms. Such…

Strongly Correlated Electrons · Physics 2019-12-25 Jonas Becker , Stefan Wessel

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

Strongly Correlated Electrons · Physics 2024-08-21 Hidekazu Tanaka

The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with non-negligible Dzyaloshinskii-Moriya interaction~(DMI). A well established phase transition to the $\mathbf…

Strongly Correlated Electrons · Physics 2017-07-04 Laura Messio , Samuel Bieri , Claire Lhuillier , Bernard Bernu
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