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Nitrogen vacancy (NV) centers in diamond have been used as ultrasensitive magnetometers to perform nuclear magnetic resonance (NMR) spectroscopy of statistically polarized samples at 1 - 100 nm length scales. However, the spectral linewidth…

We present nanoscale NMR measurements performed with nitrogen-vacancy (NV) centers located down to about 2 nm from the diamond surface. NV centers were created by shallow ion implantation followed by a slow, nanometer-by-nanometer removal…

Mesoscale and Nanoscale Physics · Physics 2014-01-24 M. Loretz , S. Pezzagna , J. Meijer , C. L. Degen

We investigate nuclear spin hyperpolarization from nitrogen vacancy centers in isotopically enriched diamonds with $^{13}$C concentrations up to 100%. $^{13}$C enrichment leads to hyperfine structure of the nitrogen vacancy electron spin…

Here we propose and analyse in detail protocols that can achieve rapid hyperpolarization of 13C nuclear spins in randomly oriented ensembles of nanodiamonds at room temperature. Our protocols exploit a combination of optical polarization of…

Quantum Physics · Physics 2015-11-25 Q. Chen , I. Schwarz , F. Jelezko , A. Retzker , M. B. Plenio

Nuclear magnetic resonance imaging (MRI) at the atomic scale offers exciting prospects for determining the structure and function of individual molecules and proteins. Quantum defects in diamond have recently emerged as a promising platform…

Quantum Physics · Physics 2022-04-06 K. S. Cujia , K. Herb , J. Zopes , J. M. Abendroth , C. L. Degen

Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high…

Quantum Physics · Physics 2024-09-06 Zhiyi Hu , Fengjian Jiang , Jingyan He , Yulin Dai , Ya Wang , Nanyang Xu , Jiangfeng Du

The nitrogen-vacancy (N-V) center in diamond is a promising atomic-scale system for solid-state quantum information processing. Its spin-dependent photoluminescence has enabled sensitive measurements on single N-V centers, such as: electron…

Other Condensed Matter · Physics 2015-06-25 R. J. Epstein , F. M. Mendoza , Y. K. Kato , D. D. Awschalom

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) spectroscopy of bulk quantum materials have provided insight into phenomena such as quantum phase criticality, magnetism, and superconductivity. With the emergence of…

Nitrogen-vacancy (NV) center in diamond was found to be a powerful tool for various sensing applications. The main work horse of this center so far has been optically detected electron resonance. Utilization of the nuclear spin has the…

We present high-resolution optically detected magnetic resonance (ODMR) spectroscopy on single nitrogen-vacancy (NV) center spins in diamond at and around zero magnetic field. The experimentally observed transitions depend sensitively on…

Mesoscale and Nanoscale Physics · Physics 2019-11-22 Johannes Kölbl , Mark Kasperczyk , Beat Bürgler , Arne Barfuss , Patrick Maletinsky

The nuclear spin in the vicinity of a nitrogen-vacancy (NV) center possesses of long coherence time and convenient manipulation assisted by the strong hyperfine interaction with the NV center. It is suggested for the subsequent quantum…

Quantum Physics · Physics 2018-04-18 Yang-Yang Wang , Jing Qiu , Ying-Qi Chu , Mei Zhang , Jianming Cai , Qing Ai , Fu-Guo Deng

Using pulsed photoionization the coherent spin manipulation and echo formation of ensembles of NV- centers in diamond are detected electrically realizing contrasts of up to 17 %. The underlying spin-dependent ionization dynamics are…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Florian M. Hrubesch , Georg Braunbeck , Martin Stutzmann , Friedemann Reinhard , Martin S. Brandt

The nitrogen-vacancy (NV) centre, as a promising candidate solid state system of quantum information processing, its electron spin coherence is influenced by the magnetic field fluctuations due to the local environment. In pure diamonds,…

Mesoscale and Nanoscale Physics · Physics 2011-04-08 Nan Zhao , Jian-Liang Hu , Sai-Wah Ho , Tsz-Kai Wen , R. B. Liu

Nuclear spins in the proximity of electronic spin defects in solids are promising platforms for quantum information processing due to their ability to preserve quantum states for a remarkably long time. Here we report a comprehensive study…

Quantum Physics · Physics 2023-10-03 Mykyta Onizhuk , Giulia Galli

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

The nitrogen-vacancy (NV) center has enabled widespread study of nanoscale nuclear magnetic resonance (NMR) spectroscopy at low magnetic fields. NMR spectroscopy at high magnetic fields significantly improves the technique's spectral…

Mesoscale and Nanoscale Physics · Physics 2021-09-15 Benjamin Fortman , Laura Mugica-Sanchez , Noah Tischler , Cooper Selco , Yuxiao Hang , Karoly Holczer , Susumu Takahashi

A nitrogen-vacancy (NV) center in diamond is a promising sensor for nanoscale magnetic sensing. Here we report electron spin resonance (ESR) spectroscopy using a single NV center in diamond. First, using a 230 GHz ESR spectrometer, we…

Mesoscale and Nanoscale Physics · Physics 2016-10-05 Chathuranga Abeywardana , Viktor Stepanov , Franklin H. Cho , Susumu Takahashi

The long-lived electronic spin of the nitrogen-vacancy (NV) center in diamond is a promising quantum sensor for detecting nanoscopic magnetic and electric fields in a variety of experimental conditions. Nevertheless, an outstanding…

We propose a sensitive and stable three-axis gyroscope in diamond. We achieve high sensitivity by exploiting the long coherence time of the N14 nuclear spin associated with the Nitrogen-Vacancy center in diamond, and the efficient…

Quantum Physics · Physics 2015-11-25 Ashok Ajoy , Paola Cappellaro
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