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We have performed elastic and inelastic neutron experiments on single crystal samples of the coordination polymer compound CuF2(H2O)2(pyz) (pyz=pyrazine) to study the magnetic structure and excitations. The elastic neutron diffraction…

The space- and time-dependent response of many-body quantum systems is the most informative aspect of their emergent behaviour. The dynamical structure factor, experimentally measurable using neutron scattering, can map this response in…

Strongly Correlated Electrons · Physics 2013-09-27 B. Lake , D. A. Tennant , J. -S. Caux , T. Barthel , U. Schollwöck , S. E. Nagler , C. D. Frost

We present a systematic analysis on the basis of ab initio calculations and many-body perturbation theory for clarifying the dominant fluctuation in complex charge-spin-orbital coupled systems. For a tight-binding multiband model obtained…

Strongly Correlated Electrons · Physics 2015-06-23 Amane Uehara , Hiroshi Shinaoka , Yukitoshi Motome

Magnetization, magnetocaloric, calorimetric, neutron and X-ray diffraction and inelastic neutron scattering measurements are performed on single crystals of BaCdVO(PO$_4$)$_2$. The low-temperature crystal structure is found to be of a lower…

Strongly Correlated Electrons · Physics 2019-11-07 V. K. Bhartiya , K. Yu. Povarov , D. Blosser , S. Bettler , Z. Yan , S. Gvasaliya , S. Raymond , E. Ressouche , K. Beauvois , J. Xu , F. Yokaichiya , A. Zheludev

The coupling of spin and orbital degrees of freedom in the trilayer Sr4Ru3O10 sets a long-standing puzzle, due to the peculiar anisotropic coexistence of out-of-plane ferromagnetism and in-plane metamagnetism. Recently, the induced magnetic…

Strongly Correlated Electrons · Physics 2019-10-09 Filomena Forte , Lucia Capogna , Veronica Granata , Rosalba Fittipaldi , Antonio Vecchione , Mario Cuoco

Dispersionless electronic bands lead to an extremely high density of states and suppressed kinetic energy, thereby increasing electronic correlations and instabilities that can shape emergent ordered states, such as excitonic,…

We have studied the static and dynamic magnetic properties of two-dimensional (2D) and quasi-two-dimensional, spin-S, quantum Heisenberg antiferromagnets (QHAF) diluted with spinless vacancies. Using spin-wave theory and T-matrix…

Strongly Correlated Electrons · Physics 2009-11-07 A. L. Chernyshev , Y. C. Chen , A. H. Castro Neto

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin

Recent neutron scattering experiments on the spin-1/2 kagome lattice antiferromagnet ZnCu3(OH)6Cl2 (Herbertsmithite) provide the first evidence of fractionalized excitations in a quantum spin liquid state in two spatial dimensions. In…

Strongly Correlated Electrons · Physics 2014-04-03 Matthias Punk , Debanjan Chowdhury , Subir Sachdev

Nd2Ir2O7 is a correlated semimetal with the pyrochlore structure, in which competing spin-orbit coupling and electron-electron interactions are believed to induce a time-reversal symmetry broken Weyl semimetal phase characterized by pairs…

Strongly Correlated Electrons · Physics 2020-11-02 K. Wang , B. Xu , C. W. Rischau , N. Bachar , B. Michon , J. Teyssier , Y. Qiu , T. Ohtsuki , Bing Cheng , N. P. Armitage , S. Nakatsuji , D. van der Marel

Emergent $U(1)$ gauge theories and artificial photons in frustrated magnets are outstanding examples of many-body collective phenomena. The classical and quantum regimes of these systems provide platforms for classical and quantum spin…

Strongly Correlated Electrons · Physics 2023-01-26 Emily Z. Zhang , Finn Lasse Buessen , Yong Baek Kim

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

Pinch point singularities, associated with flat band magnetic excitations, are tell-tale signatures of Coulomb spin liquids. While their properties in the presence of quantum fluctuations have been widely studied, the fate of the…

We report a comprehensive inelastic neutron-scattering study of the frustrated pyrochlore antiferromagnet MgCr2O4 in its cooperative paramagnetic regime. Theoretical modeling yields a microscopic Heisenberg model with exchange interactions…

Partially-ordered magnets are distinct from both spin liquids and conventional ordered magnets because order and disorder coexist in the same magnetic phase. Here, we determine the nature of partial order in the canonical frustrated…

The frustrated magnet Bi2Fe4O9 has been reported to exhibit complex spin dynamics coexisting with conventional spin wave excitations. The magnetic Fe3+ (S = 5/2) ions are arranged into a distorted two-dimensional Cairo pentagonal lattice…

We discuss the magnetic properties of a Sm$_{2}$Mo$_{2}$O$_{7}$ single crystal as investigated by means of different experimental techniques. In the literature, a conventional itinerant ferromagnetic state is reported for the Mo$^{4+}$…

Strongly Correlated Electrons · Physics 2014-08-13 G. Prando , P. Carretta , A. U. B. Wolter , R. Saint-Martin , A. Revcolevschi , B. Büchner

We present magnetic susceptibility, heat capacity, and neutron diffraction measurements of polycrystalline Nd2Ru2O7 down to 0.4 K. Three anomalies in the magnetic susceptibility measurements at 146, 21 and 1.8 K are associated with an…

Strongly Correlated Electrons · Physics 2018-07-31 S. T. Ku , Dinesh Kumar , M. R. Lees , W-T. Lee , R. Aldus , A. Studer , P. Imperia , S. Asai , T. Masuda , S. W. Chen , J. M. Chen , L. J. Chang

Using Raman scattering spectroscopy, we uncover a complex magnetic behavior of Nd$_2$Ir$_2$O$_7$ , which stands out among magnetic pyrochlores by the lowest temperature of the all-in-all-out (AIAO) Ir moments ordering…

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian