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We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

Quasi-2D van der Waals ferromagnet Fe$_4$GeTe$_2$, featuring the simultaneous presence of high Curie temperature ($T_\mathrm{C}$ $\sim 270$ K) and a spin-reorientation transition at $T_\mathrm{SR}$ $\sim 110$ K, is a rare system where…

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

Materials Science · Physics 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch

Two-dimensional (2D) van der Waals (vdW) magnets with spin-phonon coupling are crucial for next-generation spintronics. Among them, Fe3GaTe2 has attracted widespread attention due to above-room-temperature intrinsic ferromagnetism and large…

Materials Science · Physics 2024-12-02 Gaojie Zhang , Hao Wu , Li Yang , Wen Jin , Bichen Xiao , Wenfeng Zhang , Haixin Chang

The vibrational properties of ferrimagnetic $\mathrm{Mn_3Si_{2}Te_6}$ single crystals are investigated using Raman spectroscopy and density functional theory calculations. Eighteen Raman-active modes are identified, fourteen of which are…

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

Materials Science · Physics 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

Antiferromagnetic materials with strong spin-phonon coupling have the potential for spintronic applications. Here, we report the structural, magnetic, and vibrational properties of 12R-BaTi0.4Mn0.6O3. Temperature-dependent magnetization…

Materials Science · Physics 2021-10-27 Bommareddy Poojitha , Anjali Rathore , Surajit Saha

Materials having strong coupling between different degrees of freedom such as spin, lattice, orbital, and charge are of immense interest due to their potential device applications. Here, we have stabilized the 9R phase of BaMnO3, by Sr (Ti)…

Materials Science · Physics 2021-10-27 Bommareddy Poojitha , Anjali Rathore , Surajit Saha

The manipulation of spin-phonon coupling in both formations and explorations of magnetism in two-dimensional van der Waals ferromagnetic semiconductors facilitates unprecedented prospects for spintronics devices. The interlayer engineering…

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

Electronic structure near Fermi level of Pr2CoFeO6 (at 300 K) was investigated by X-ray photoemission spectroscopy (XPS) technique. All three cations, i.e., Pr, Co and Fe were found to be trivalent in nature. XPS analysis also suggested the…

Strongly Correlated Electrons · Physics 2019-05-22 Arkadeb Pal , Surajit Ghosh , Amish G. Joshi , P. K. Gupta , P. Prakash , Amitabh Das , A. K. Ghosh , Sandip Chatterjee

The temperature dependence of eigenfrequencies and intensities of the IR active modes has been investigated for the antiferromagnetic chromium spinel compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy for…

Strongly Correlated Electrons · Physics 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

We report on infrared, Raman, magnetic susceptibility, and specific heat measurements on CdCr2O4 and ZnCr2O4 single crystals. We estimate the nearest-neighbor and next-nearest neighbor exchange constants from the magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2010-02-03 Ch. Kant , J. Deisenhofer , T. Rudolf , F. Mayr , F. Schrettle , A. Loidl , V. Gnezdilov , D. Wulferding , P. Lemmens , V. Tsurkan

The layered van der Waals Fe$_5$GeTe$_2$ (F5GT) compound exhibits room-temperature ferromagnetism, making it a promising candidate for technological applications. In our study, combined temperature, wavelength, and polarization-dependent…

Materials Science · Physics 2026-05-14 Smrutiranjan Mekap , Andrzej Ptok , Jyoti Saini , Changgu Lee , Subhasis Ghosh , Anushree Roy

Infrared reflectivity spectra of cubic SrMnO$_{3}$ ceramics reveal 18 % stiffening of the lowest-frequency phonon below the antiferromagnetic phase transition occurring at T$_{N}$ = 233 K. Such a large temperature change of the polar phonon…

Inelastic light scattering studies on single crystal of electron-doped Ca(Fe0.95Co0.05)2As2 superconductor, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at TSM ~ 140 K and superconducting…

Single crystals of quasi-2D chromium telluride system represented by Cr1+xTe2 (x = 0.22), which crystallizes in the trigonal structure with the c-axis as the growth direction, are synthesized by the flux method. The magnetization…

Strongly Correlated Electrons · Physics 2025-07-21 Gayathri V , Sathishkumar M , Sandip Kumar Kuila , Vikash Kumar , Abhidev B , Reshna Elsa Philip , Partha Pratim Jana , Soham Manni

We have studied polarized Raman spectra of (TMTSF)2PF6 single crystals in the wide spectral and temperature range using different laser energies. We observed and assigned 23 Raman active modes. The carbon C=C in-phase and out-of-phase…

Strongly Correlated Electrons · Physics 2007-05-23 Z. V. Popovic , V. A. Ivanov , O. P. Khoung , T. Nakamura , G. Saito , V. V. Moshchalkov

Temperature dependent Raman scattering measurements have been performed to explore unusual coupling between magnetism and crystal structure in doped pyrochlore iridate Y$_2$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$ with $x$ = 0.0, 0.05 and 0.2. The…

Strongly Correlated Electrons · Physics 2019-02-20 Harish Kumar , V. G. Sathe , A. K. Pramanik

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh
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