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A unitary coupled-cluster (UCC) form for the wavefunction in the variational quantum eigensolver has been suggested as a systematic way to go beyond the mean-field approximation and include electron correlation in solving quantum chemistry…

Quantum Physics · Physics 2018-09-12 Ilya G. Ryabinkin , Tzu-Ching Yen , Scott N. Genin , Artur F. Izmaylov

Computing-in-Memory (CIM) macros have gained popularity for deep learning acceleration due to their highly parallel computation and low power consumption. However, limited macro size and ADC precision introduce throughput and accuracy…

Hardware Architecture · Computer Science 2026-05-01 Ming-Han Lin , Tian-Sheuan Chang

The Compact Muon Solenoid (CMS) experiment at the Large Hadron Collider (LHC) is one of the largest data producers in the scientific world, with standard data products centrally produced, and then used by often competing teams within the…

Distributed, Parallel, and Cluster Computing · Computer Science 2022-12-20 Igor Sfiligoi , Frank Würthwein , Diego Davila

To facilitate rational molecular and materials design, this research proposes an integrated computational framework that combines stochastic simulation, ab initio quantum chemistry, and molecular docking. The suggested workflow allows…

Materials Science · Physics 2026-01-08 Md Rakibul Karim Akanda , Michael P. Richard

We introduce a parallel, GPU-accelerated implementation of the iterative qubit coupled cluster (iQCC) method that overcomes the exponential growth of the transformed Hamiltonian -- the principal bottleneck for classical emulation of quantum…

Quantum Physics · Physics 2026-03-11 Seyyed Mehdi Hosseini Jenab , Brandon Henderson , Scott N. Genin

The study of strongly correlated electron systems remains a fundamental challenge in condensed matter physics, particularly in two-dimensional (2D) systems hosting various exotic phases of matter including quantum spin liquids,…

Strongly Correlated Electrons · Physics 2025-07-01 Hui-Ke Jin , Rong-Yang Sun , Hong-Hao Tu , Yi Zhou

Traditional atomistic machine learning (ML) models serve as surrogates for quantum mechanical (QM) properties, predicting quantities such as dipole moments and polarizabilities, directly from compositions and geometries of atomic…

In a new effort to make our research transparent and reproducible by others, we developed a workflow to run and share computational studies on the public cloud Microsoft Azure. It uses Docker containers to create an image of the application…

Computational Engineering, Finance, and Science · Computer Science 2020-07-24 Olivier Mesnard , Lorena A. Barba

The trend of massive connectivity pushes forward the explosive growth of end devices. The emergence of various applications has prompted a demand for pervasive connectivity and more efficient computing paradigms. On the other hand, the lack…

Signal Processing · Electrical Eng. & Systems 2024-11-12 Zelin Ji , Zhijin Qin

Determining ground state energies of quantum systems by hybrid classical/quantum methods has emerged as a promising candidate application for near-term quantum computational resources. Short of large-scale fault-tolerant quantum computers,…

Quantum Physics · Physics 2016-10-25 Nicholas C. Rubin

Quantum computing has emerged as a promising platform for simulating strongly correlated systems in chemistry, for which the standard quantum chemistry methods are either qualitatively inaccurate or too expensive. However, due to the…

Chemical Physics · Physics 2024-05-06 Max Rossmannek , Fabijan Pavošević , Angel Rubio , Ivano Tavernelli

We developed a general framework for hybrid quantum-classical computing of molecular and periodic embedding approaches based on an orbital space separation of the fragment and environment degrees of freedom. We demonstrate its potential by…

Chemical Physics · Physics 2024-12-23 Stefano Battaglia , Max Rossmannek , Vladimir V. Rybkin , Ivano Tavernelli , Jürg Hutter

Meeting the strict Quality of Service (QoS) requirements of terminals has imposed a signiffcant challenge on Multiaccess Edge Computing (MEC) systems, due to the limited multidimensional resources. To address this challenge, we propose a…

Networking and Internet Architecture · Computer Science 2024-04-29 Qianqian Liu , Haixia Zhang , Xin Zhang , Dongfeng Yuan

We demonstrate the first end-to-end integration of high-performance computing (HPC), reliable quantum computing, and AI in a case study on catalytic reactions producing chiral molecules. We present a hybrid computation workflow to determine…

An accurate description of strong correlation is quintessential for the exploration of emerging chemical phenomena. While near-term variational quantum algorithms provide a theoretically scalable framework for quantum chemical problems, the…

Quantum Physics · Physics 2025-10-20 Arpan Choudhury , Sonaldeep Halder , Rahul Maitra , Debashree Ghosh

Machine learning (ML) plays an important role in quantum chemistry, providing fast-to-evaluate predictive models for various properties of molecules. However, most existing ML models for molecular electronic properties use density…

Chemical Physics · Physics 2024-06-26 Hao Tang , Brian Xiao , Wenhao He , Pero Subasic , Avetik R. Harutyunyan , Yao Wang , Fang Liu , Haowei Xu , Ju Li

In this paper, we aim to address the challenge of hybrid mobile edge-quantum computing (MEQC) for sustainable task offloading scheduling in mobile networks. We develop cost-effective designs for both task offloading mode selection and…

Systems and Control · Electrical Eng. & Systems 2023-06-27 Ziqiang Ye , Yulan Gao , Yue Xiao , Minrui Xu , Han Yu , Dusit Niyato

Automatic decision-making approaches, such as reinforcement learning (RL), have been applied to (partially) solve the resource allocation problem adaptively in the cloud computing system. However, a complete cloud resource allocation…

Distributed, Parallel, and Cluster Computing · Computer Science 2017-08-15 Ning Liu , Zhe Li , Zhiyuan Xu , Jielong Xu , Sheng Lin , Qinru Qiu , Jian Tang , Yanzhi Wang

Quantum computers have the potential to simulate chemical systems beyond the capability of classical computers. Recent developments in hybrid quantum-classical approaches enable the determinations of the ground or low energy states of…

Quantum Physics · Physics 2021-12-06 Chee-Kong Lee , Jonathan Wei Zhong Lau , Liang Shi , Leong Chuan Kwek

In this work we investigate methods to improve the efficiency and scalability of quantum algorithms for quantum chemistry applications. We propose a transformation of the electronic structure Hamiltonian in the second quantization framework…

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