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High intensity THz lasers allow for the coherent excitation of individual phonon modes. The ultrafast control of emergent magnetism by means of phonons opens up new tuning mechanisms for functional materials. While theoretically predicted…

Materials Science · Physics 2024-07-08 R. Matthias Geilhufe , Wolfram Hergert

Altermagnetism refers to a wide class of magnetic orders featuring magnetic sublattices with opposite spins related by rotational symmetries, resulting in non-trivial spin splitting and magnetic multipoles. However, the direct observation…

Spin-phonon coupling and magnetodielectric effects of ZnCr2Se4 were investigated by means of infrared (IR) spectroscopy as a function of temperature and magnetic field. ZnCr2Se4 is dominated by ferromagnetic exchange but undergoes…

Strongly Correlated Electrons · Physics 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

Utilizing magnetic susceptibility, specific heat, thermal expansion and IR spectroscopy we provide experimental evidence that the two subsequent antiferromagnetic transitions in ZnCr_2S_4 at T_N1 = 15 K and T_N2= 8 K are accompanied by…

Strongly Correlated Electrons · Physics 2009-11-11 J. Hemberger , T. Rudolf , H. -A. Krug von Nidda , F. Mayr , A. Pimenov , V. Tsurkan , A. Loidl

We report the direct observation of a "resonance" mode in the lowest-energy optic phonon very near the zone center around (111) in the multiferroic BiFeO$_3$ using neutron scattering methods. The phonon scattering intensity is enhanced when…

We investigate spin dynamics in the antiferromagnetic (AFM) multiferroic TbMnO3 using optical- pump, terahertz (THz)-probe spectroscopy. Photoexcitation results in a broadband THz transmission change, with an onset time of 25 ps at 6 K that…

Strongly Correlated Electrons · Physics 2016-12-21 P. Bowlan , S. A. Trugman , X. Wang , Y. M. Dai , S. -W. Cheong , E. D. Bauer , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

Compressively strained epitaxial (001) EuTiO3 thin films of tetragonal symmetry have been deposited on (001) (LaAlO3)_0.29-(SrAl_{1/2}Ta_{1/2}O3)_0.71 (LSAT) substrates by reactive molecular-beam epitaxy. Enhancement of the Neel temperature…

Ultrafast light-matter interactions inspire potential functionalities in picosecond optoelectronic applications. However, achieving directional carrier dynamics in metals remains challenging due to strong carrier scattering within a…

Materials Science · Physics 2025-02-14 S. G. Jeong , I. H. Choi , S. Lee , J. Y. Oh , S. Nair , J. H. Lee , C. Kim , A. Seo , W. S. Choi , T. Low , J. S. Lee , B. Jalan

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

Materials Science · Physics 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~…

Strongly Correlated Electrons · Physics 2015-05-28 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , G. Karapetrov , R. Hott , R. Heid , K. -P. Bohnen , A. Alatas

We study THz-driven spin dynamics in thin CoPt films with perpendicular magnetic anisotropy. Femtosecond magneto-optical Kerr effect measurements show that demagnetization amplitude of about $1\%$ can be achieved with a peak THz electric…

Mesoscale and Nanoscale Physics · Physics 2018-03-14 Debanjan Polley , Matteo Pancaldi , Matthias Hudl , Paolo Vavassori , Sergei Urazhdin , Stefano Bonetti

Understanding spin-lattice interactions in antiferromagnets is one of the most fundamental issues at the core of the recently emerging and booming fields of antiferromagnetic spintronics and magnonics. Recently, coherent nonlinear…

Transient reflectivity traces measured for nanometer-sized films of the topological insulator Bi2Se3 revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort laser pulses of 1.51 eV photon…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh

MnO thin films with various thicknesses and strains were grown on MgO substrates by pulsed laser deposition, then characterized using x-ray diffraction and infrared reflectance spectroscopy. Films grown on (001)-oriented MgO substrates…

Strongly Correlated Electrons · Physics 2020-01-20 Alireza Kashir , Veronica Goian , Oliva Pacherova , Yoon Hee Jeong , Gil-Ho Lee , Stanislav Kamba

Exciting atomic oscillations with light is a powerful technique to control the electronic properties of materials, leading to remarkable phenomena such as light-induced superconductivity and ultrafast insulator to metal transitions. Here we…

Strongly Correlated Electrons · Physics 2021-05-13 D. Afanasiev , J. R. Hortensius , B. A. Ivanov , A. Sasani , E. Bousquet , Y. M. Blanter , R. V. Mikhaylovskiy , A. V. Kimel , A. D. Caviglia

Excitation of coherent high-frequency magnons (quanta of spin waves) is critical to the development of high-speed magnonic devices. Here we computationally demonstrate the excitation of coherent sub-terahertz (THz) magnons in ferromagnetic…

Applied Physics · Physics 2022-06-22 Shihao Zhuang , Jia-Mian Hu

Magnetophononics, the modulation of magnetic interactions by driving infrared-active lattice excitations, is emerging as a key mechanism for the ultrafast dynamical control of both semiclassical and quantum spin systems by coherent light.…

Strongly Correlated Electrons · Physics 2023-05-15 M. Yarmohammadi , M. Krebs , G. S. Uhrig , B. Normand

We explore the phonon dynamics of thin films of the topological insulator material Bi2Se2Te using ultrafast pump-probe spectroscopy. The time resolved differential reflectivity of the films exhibit fast and slow oscillations. We have given…

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The…

Strongly Correlated Electrons · Physics 2019-04-23 Kousik Samanta , Danilo Rigitano , Pascoal Jose Giglio Pagliuso , Eduardo Granado