Related papers: Fast and compact time-resolved spectroscopy enable…
A key challenge for quantum science and technology is to realise large-scale, precisely controllable, practical systems for non-classical secured communications, metrology and ultimately meaningful quantum simulation and computation.…
Fast (sub-second) spectroscopy with high spectral resolution is of vital importance for revealing quantum chemistry kinetics of complex chemical and biological reactions. Fourier transform (FT) spectrometers can achieve high spectral…
We present homogeneous quantum cascade lasers (QCLs) emitting around 3 THz which display bandwidths up to 950 GHz with a single stable beatnote. Devices are spontaneously operating in a harmonic comb state, and when in a dense mode regime…
Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…
Here we show how time-resolved broadband optical spectroscopy can be used to quantify, with femtometer resolution, the oscillation amplitudes of coherent phonons through a displacive model without free tuning parameters, except an overall…
Optical frequency combs are utilized in a wide range of optical applications, including atomic clocks, interferometers, and various sensing technologies. They are often generated via four-wave mixing in chip-integrated microring resonators,…
An optical frequency comb comprises a cluster of equally spaced, phase-locked spectral lines. Replacing these classical components with correlated quantum light gives rise to cluster quantum frequency combs, providing abundant quantum…
Optical frequency combs have revolutionized the field of frequency metrology within the last decade and have become enabling tools for atomic clocks, gas sensing and astrophysical spectrometer calibration. The rapidly increasing number of…
Supercontinuum generation using chip-integrated photonic waveguides is a powerful approach for spectrally broadening pulsed laser sources with very low pulse energies and compact form factors. When pumped with a mode-locked laser frequency…
We demonstrate a simple system for dual-comb spectroscopy based on two inherently coherent optical frequency combs generated via seeded parametric down-conversion. The inbuilt coherence is established by making the two combs share a common…
We propose a direct and real-time ranging scheme using an optical frequency combs, able to compensate optically for index of refraction variations due to atmospheric parameters. This scheme could be useful for applications requiring…
Dual THz comb spectroscopy has the potential to be used as universal THz spectroscopy with high spectral resolution, high spectral accuracy, and broad spectral coverage; however, the requirement for dual stabilized femtosecond lasers…
We propose an implementation scheme for the continuous-time quantum walk using a diatomic molecule and an optical frequency comb. We show an analogy between the quantum walk and the cascade rotational transitions induced by the optical…
Due to their rich level structure, molecules are well-suited for probing time variation of fundamental constants, precisely measuring parity violation and time-reversal non-invariance effects, studying quantum mechanical aspects of chemical…
Spectral shaping is critical to many fields of science. In astronomy for example, the detection of exoplanets via the Doppler effect hinges on the ability to calibrate a high resolution spectrograph. Laser frequency combs can be used for…
Frequency-modulated (FM) combs are produced by mode-locked lasers in which the electric field has a linearly chirped frequency and nearly constant amplitude. This regime of operation occurs naturally in certain laser systems and constitutes…
We present a detailed description of the design, construction, and performance of high-power ultrafast Yb:fiber laser frequency combs in operation in our laboratory. We discuss two such laser systems: an 87 MHz, 9 W, 85 fs laser operating…
Dual comb spectroscopy (DCS) is a powerful technique for broadband spectroscopy with high precision and fast data acquisition. High-frequency resolution requires long data acquisition times, limiting the temporal resolution in time-resolved…
Optical frequency comb, with precisely controlled spectral lines spanning a broad range, has been the key enabling technology for many scientific breakthroughs. In addition to the traditional implementation based on modelocked lasers,…
Laser frequency combs are fast becoming critical to reaching the highest radial velocity precisions. One shortcoming is the highly variable brightness of the comb lines across the spectrum (up to 4-5 orders of magnitude). This can result in…